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2002 Fiscal Year Final Research Report Summary

In-Situ X-ray Diffraction Study of Silicate Melt Structure at High Pressures and Temperatures

Research Project

Project/Area Number 12440117
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体地球物理学
Research InstitutionThe University of Tokyo

Principal Investigator

FUNAMORI Nobumasa  The University of Tokyo, Graduate School of Science, Department of Earth and Planetary Science, Associate Professor, 大学院・理学系研究科, 助教授 (70306851)

Project Period (FY) 2000 – 2003
Keywordssilicate melt / high pressure and high temperature / in situ X-ray diffraction
Research Abstract

Our new techniques for studying the structure of liquids at high pressures make it possible to measure the structural changes in (1) elemental liquids with relatively low temperatures, such as liquid Te, liquid Si, and liquid Ge, up to above 20 GPa and (2) silicate melts, such as MgSiO_3 melt and CaSiO_3 melt, up to 6 GPa. Our paper that reports results of (2) in detail may be the first paper of this research field published in an international journal.The abstract of the paper is "We have developed synchrotron X-ray diffraction techniques for studying the structure of silicate melts and have applied them to measuring the structures of MgSiO_3 and CaSiO_3 melts up to 6 GPa. In both melts, it appears that the changes in the local structure around the divalent ions and in the network structure of SiO_4 tetrahedra are the dominant compression mechanisms while a change in the local structure around the Si ion is a secondary mechanism up to at least 6 GPa. The structural changes appear to be larger in CaSiO_3 melt than in MgSiO_3 melt, especially in the vicinity of ambient pressure. These results are consistent with available experimental and theoretical information on MgSiO_3 and CaSiO_3, and explain discrepancies in previous work". We attain some progress in measurements of silicate melt structure at high pressures. However, as shown in the title of the paper, the research is still "exploratory" and requires further development of experimental techniques, for example, to extend the pressure limit.

  • Research Products

    (18 results)

All Other

All Publications (18 results)

  • [Publications] K.Oguri et al.: "Post-garnet transition in a natural pyrope : A multi-anvil study based on in situ X-ray diffraction and transmission electron microscopy"Physics of the Earth and Planetary Interior. 122. 175-186 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Ohtani et al.: "Structure of liquid germanium under pressure"Proceedings of the 17^<th> AIRAPT Conference. 498-501 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Tsuji et al.: "Structure of liquid tellurium at high temperatures"Proceedings of the 17^<th> AIRAPT Conference. 510-513 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Funamori: "Effects of non-hydrostatic stresses on high-pressure and high-temperature X-ray diffraction"Proceedings of ISAM2001. 55-56 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Funamori, K.Tsuji: "Structural transformation of liquid tellurium at high pressures and temperatures"Physical Review B. 65. 014105 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 船守展正: "マルチアンビル装置を用いた高温高圧X線その場観察実験における圧力測定の誤差"高圧力の科学と技術. 12. 153-158 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Funamori, K.Tsuji: "Pressure-induced structural change of liquid silicon"Physical Review Letters. 88. 255058 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Funamori et al.: "Exploratory studies of silicate melt structure at high pressures and temperatures by in situ X-ray diffraction"Journal of Geophysical Research. 109. B03203 (2004)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Tsuji et al.: "Pressure dependence of the structure of liquid group 14 elements"Journal of Physics : Condensed Matter. 16. S989-S996 (2004)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Oguri et al.: "Post-garnet transition in a natural pyrope : A multi-anvil study based on in situ X-ray diffraction and transmission electron microscopy"Physics of the Earth and Planetary Interior. 122. 175-186 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Ohtani et al.: "Structure of liquid germanium under pressure"Proceedings of the 17th AIRAPT Conference, Hawaii. 498-501 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Tsuji et al.: "Structure of liquid tellurium at high temperatures"Proceedings of the 17th AIRAPT Conference, Hawaii. 510-513 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Funamori: "Effects of non-hydrostatic stresses on high-pressure and high-temperature X-ray diffraction"Proceedings of ISAM 2001, Tsukuba. 55-56 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Funamori, K.Tsuji: "Structural transformation of liquid tellurium at high pressures and temperatures"Physical Review B. 65. 014105 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Funamori: "Error sources of pressure and measurements in high-pressure and high-temperature X-ray diffraction studies using multi-anvil apparatus (in Japanese)"The Review of High Pressure Science Technology. 12. 153-158 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Funamori, K.Tsuji: "Pressure-induced structural change of liquid silicon"Physical Review Letters. 88. 255508 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Funamori et al.: "Exploratory studies of silicate melt structure at high pressures and temperatures by in situ X-ray diffraction"Journal of Geophysical Research. 109. B03203 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Tsuji et al.: "Pressure dependence of the structure of liquid group 14 elements"Journal of Physics Condensed Matter. 16. S989-S996 (2004)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2005-04-19  

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