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2002 Fiscal Year Final Research Report Summary

Development of magnetoresistance sensing materials consisting of granulan materials with micro-patterned soft magnetic alloy films

Research Project

Project/Area Number 12555183
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section展開研究
Research Field Structural/Functional materials
Research InstitutionTohoku University

Principal Investigator

TAKANASHI Koki  Institute for Materials Research, Professor, 金属材料研究所, 教授 (00187981)

Co-Investigator(Kenkyū-buntansha) KOBAYASHI Nobukiyo  The Research Institute for Electric and Magnetic Materials Researcher, 研究員 (70205475)
SHIMA Toshiyuki  Institute for Materials Research, Research Associate, 金属材料研究所, 助手 (50261508)
MITANI Seiji  Institute for Materials Research, Associate Professor, 金属材料研究所, 助教授 (20250813)
OHNUMA Shigehiro  The Research Institute for Electric and Magnetic Materials, Principal Researcher, 主任研究員 (50142633)
Project Period (FY) 2000 – 2002
Keywordsgranular film / soft magnetic film / micro fabrication / tunnel effect / magnetoresistance / magnetization process / magnetoresistance device / magnetic sensor
Research Abstract

Currently, magnetic sensors have been important devices, and are actually used for many systems and purposes. Magnetic granular thin film is one of most important materials applicable to magnetic sensors because it can be made easily by a conventional sputtering technique. Furthermore, excellent field-sensitivity has been achieved in granular-in-gap (GIG) structures in which magnetic granular film is put in a lateral gap between a couple of soft magnetic alloy electrodes.
In this study, we have investigated on (i) optimization of GIG structures, (ii) development of new structures for high field-sensitivity, (iii) development of new magnetic granular materials with large magnetoresistance, (iv) mechanism of the high field-sensitivity in GIG structures,(v) related magnetoresistance effects in GIG structures and (vi) development of actual GIG devices. By optimizing GIG structures, the magnitude and field-sensitivity of tunnel magnetoresistance are improved. This result is useful for preparing actual GIG devices. Concerning new materials, the largest room-temperature magnetoresistance has been found in CoFe-fluoride granular films, indicating that fluoride is a good barrier material for tunnel magnetoresistance. As a related magnetoresistance effect, enhanced magnetoresistance due to spin dependent single electron tunneling is observed at low temperatures in nanometer-sized GIG structures. Additionally, optimization of the electrical circuit for GIG sensors has been performed.

  • Research Products

    (34 results)

All Other

All Publications (34 results)

  • [Publications] K.Yakushiji: "Composition dependence of particle size distribution and giant magnetoresistance in Co-Al-O granular films"J. Magn. Magn. Mater.. 212. 75-81 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 薬師寺 啓: "集束イオンビーム加工によるCo-Al-Oグラニュラー細線の作製と磁気抵抗効果"日本応用磁気学会誌. 24. 567-570 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 小林 伸聖: "金属-フッ化物系ナノグラニュラー薄膜のトンネル型巨大磁気抵抗効果"日本応用磁気学会誌. 24. 571-574 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 大沼 繁弘: "高B_sとρを有する(Fe, Co)-酸化物系膜の軟磁気特性"日本応用磁気学会誌. 24. 691-694 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Yakushiji: "Enhanced tunnel magnetoresistance in granular nanobridges"Appl. Phys. Lett.. 78. 515-517 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mitani: "Study on spin dependent tunneling and Coulomb blockade in granular systems with restricted tunneling paths"Mater. Sci. Eng. B. 84. 120-125 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Yakushiji: "Tunnel magnetoresistance oscillations in current perpendicular to plane geometry of CoAlO granular films"J. Appl. Phys.. 91. 7038-7040 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mitani: "Structure and tunnel magnetoresisitance in Fe/MgF_2/Co junctions with an oxide seed layer on an Fe bottom electrode"J. Appl. Phys.. 91. 7200-7202 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Yakushiji: "Tunnel magnetoresistance oscillations associated with Coulomb staircases in insulating granular systems"J. Phys. D: Appl. Phys.. 35. 2422-2426 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 森山 貴広: "Fe/MgO/MgF_2/Co接合のトンネル磁気抵抗効果"日本応用磁気学会誌. 26. 405-409 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Tanaka: "High-angle annular dark-field scanning transmission electron microscopy and electron energy-loss spectroscopy of nano-granular Co-Al-O alloys"Scripta Materialia. 48. 909-914 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 小林 伸聖: "金属-フッ化物系ナノグラニュラー膜のトンネル磁気 抗効果とGIG化による磁界感度の改善"日本応用磁気学会誌. 25. 779-782 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Kobayashi: "(Fe-Ca)-(Mg-fluoride) insulating nanogranular system with enhanced tunnel-type giant magnetoresistance"J. Appl. Phys.. 90. 4159-4162 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mitani: "Fe/MgO/FeCo(100) epitaxial magnetic tunnel junctions prepared by using in situ plasma oxidation"J. Appl. Phys.. (in press). (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 藤森 啓安: "人工微小構造制御によるスピン依存物性と新機能性材料"学術月報. 53. 33-36 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 小林 伸聖: "ナノグラニュラーインギャップ(GIG)膜による磁気 抵抗効果の高感度化"まてりあ. 41. 561-565 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 薬師寺 啓: "磁性グラニュラー薄膜を用いた人工微小構造におけるスピン依存単電子トンネル現象"日本応用磁気学会誌. 27. 111-117 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K. Yakushiji: "Composition dependence of particle size distribution and magnetoresistance in Co-Al-O granular films"J. Magn. Magn. Mater.. 212. 75-81 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Yakushiji: "Fabrication and magnetoresistance of Co-AN-0 granular wires by focused ion beam etching"J. Magn. Soc. Jpn. 24(2-4). 567-570 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N. Kobayashi: "Tunnel magnetoresistance in metal-fluoride nanogranular thin films"J. Magn., S0C. Jpn. 24(24). 571-574 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S . Ohnuma: "Soft magnetic properties of (Fe, Co)-oxide films with high Bs and p"J. Magm. Soc. Jpn. 24(2-4). 691-694 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Yakushiji: "Enhanced tunnel magnetoresistance in granular nanobridges"Appl. Phys. Lett.. 78(4). 515-517 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S. Mitani: "Study on spin dependent tunneling and Coulomb blockade in granular systems with restricted tunneling paths"Mater. Soi. Eng.. B84. 120-125 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Yakushiji: "Tunnel magnetoresistance oscillations in current perpendicular to plane geometry of CoAIO granular thin films"J. Appl. Phys.. 91(10). 7038-7040 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S. Mitani: "Structure and tunnel magnetoresistance in Fe/MgF_2/Co junctions with an oxide seed layer on an Fe bottom electrode"J. Appl. Phys.. 91(10). 7200-7202 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Yakushiji: "Tunnel magnetoresistance oscillations associated with Coulomb staircases in insulating granular systems."J. Phys. D: Appl. Phys.. 35. 2422-2426 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T. Moriyama: "Magnetoresistance in Fe/MgO/MgF_2/Co junctions"J. Magn. Soc. Jpn. 26(4). 405-409 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N. Tanaka: "High-angle annular dark-field scanning transmission electron microscopy and electron energy-loss spectroscopy of nano-granular Co-Al-O alloys"Scripta Materialia. 48. 9O9-914 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N. Kobayashi: "Tunnel magnetoresistance in metal-fluoride nanogranular films and improved field sensitivity in GIG geometry"J. Magn. Soc. Jpn. 25. 779-782 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N. Kobayashi: "(Fe-Co)-(Mg-fluoride) insulating namogranular system with enhanced tunnel-type giant magnetoresistance"J. Appl. Phys.. 90. 4159-4162 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S. Mitani: "Fe/MgO/FeCo(100) epitomical magnetic tunnel junctions prepared by using in-situ plasma oxidation"J. Appl. Phys.. in press..

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H. Fujimori: "Spin dependent properties in microfabricated systems and its application to new functional materials"Gakujutsu Geppou. 53(7). 33-36 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N. Kobayashi: "Improvement of fie[d sensitivity of magnetoresistance in nanogranular-in-gap films"Materia. 41. 561-565 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Yakushiji: "Spin dependent single electron tunneling phenomena in microfabricated granular thin films"J. Magn. Soc. Jpn. 27(3). 111-117 (2003)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2004-04-14  

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