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2003 Fiscal Year Final Research Report Summary

Anomalous Magnetism of Strongly Correlated 5f Electron Compounds

Research Project

Project/Area Number 13440103
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionHokkaido University

Principal Investigator

AMITSUKA Hiroshi  Hokkaido Univ., Grad. School of Sci., Asso. Prof., 大学院・理学研究科, 助教授 (40212576)

Co-Investigator(Kenkyū-buntansha) TENYA Kenichi  Hokkaido Univ., Grad. School of Sci., Inst., 大学院・理学研究科, 助手 (70261279)
Project Period (FY) 2001 – 2003
KeywordsStrongly Correlated Electron Systems / Heavy Fermion Systems / 5f Election Compounds / Uranium Compounds / Kondo Effects / Hidden Order / Antiferromagnetism / Pressure Effects
Research Abstract

Low-temperature 5f electronic States of URu_2Si_2 and related compounds were intensively investigated by using various experimental techniques including high-pressure and ultra-high-field measurements. Main results obtained are listed as follows : 1. It was found through neutron-scattering, NMR and μSR measurements that applying hydrostatic pressure induces a first-order phase transition from unknown "hidden order (HO)" to antiferromagnetic (AF) order in URu_2Si_2. The pressure variations of the AF volume fraction revealed that weak antiferromagnetism the long-standing issue of this system, is ascribed to the inhomogeneous AF clusters of 〜 1% volume fraction. 2. It was further found that the uniaxial stress applied along the tetragonal basal plane can induce the AF phase. This strongly suggests that the c/a ratio is a relevant parameter to control the two-phase competition. 3. Another evidence for the c/a-ratio hypothesis was obtained from Rh doping experiments. The relationship between magnetic excitations and the two-phase competition was also studied by using the Rh dope systems. 4. A precise B-T-x phase diagram for U(Ru_<1-x>Rh_x)_2Si_2 (x < 0.05) was obtained for the first time The relationship between the low-field HO-AF competing state and the high-field unknown order states was clarified. 5. A high-precision magnetometer operational at very low temperature (T > 40mK) and under high pressure (P < 1.5GPa) was developed. From the careful magnetization measurements using this apparatus, the influence of the inhomogeneous AF evolution on the superconductivity was clarified. Some of the results of the present research protect were selected as invited talks for major international conferences such as "The 23rd International Conference on Low Temperature Physics (LT23) August 20-23, 2002 (Hiroshima, Japan)" and "The Match 2003 Meeting of the American Physical Society, March 3-7, 2003 (Austin, USA)"

  • Research Products

    (52 results)

All Other

All Publications (52 results)

  • [Publications] K.Matsuda: "Spatially Inhomogeneous Development of Antiferromagnetism in URu_2Si_2 : Evidence from ^<29>Si NMR under Pressure"Physical Review Letters. 87. 87203-1-87203-4 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Tayama: "Antiferro-Quadrupolar Ordering and Multipole Interactions in PrPb_3"Journal of the Physical Society of Japan. 70. 248-258 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Nagata: "Antiferromagnetic Ordering in the Spin Ladder Compound : Sr_<14-x>Ca_xCu_<24>O_<41>"Journal of the Physical Society of Japan. 70. 2419-2424 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yokoyama: "Anomalous Fermi Liquid Behavior of the Dilute Uranium Alloys La_<1-x>U_xRu_2Si_2 (x【less than or equal】0.07)"Journal of the Physical Society of Japan. 71. 3037-3042 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yokoyama: "Effects of Uniaxial Stress on Antiferromagnetic Moment in the Heavy Electron Compound URu_2Si_2"Journal of the Physical Society of Japan. 71 Suppl.. 264-266 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Amitsuka: "Low-Temperature Magnetization Study on the Non-Kramers Cubic System Pr_3Pd_<20>Ge_6"Journal of the Physical Society of Japan. 71 Suppl.. 124-126 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Sakakibara: "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in Ce_xLa_<1-x>B_6"Journal of the Physical Society of Japan. 71 Suppl.. 48-51 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Sakakibara: "Multipole Ordering in f Electron Systems"Journal of Physics and Chemistry of Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] P.Gegenwart: "Magnetic-Field Induced Quantum Critical Point in YbRh_2Si_2"Physical Review Letters. 89. 056402-1-056402-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] F.Kromer: "Magnetic Field Response in (U,Th)Be_<13>"Journal of Low Temperature Physics. 126. 815-833 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Matsuhira: "Low-Temperature Magnetic Properties of Pyrochlore Stannates"Journal of the Physical Society of Japan. 71. 1576-1582 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Matsuda: "^<29>Si NMR Study of URu_2Si_2 under Pressure"Physica B. 312-313. 504-505 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yokoyama: "Thorium Dilution Effects of the Heavy Electron Compound URu_2Si_2"Physica B. 312-313. 498-500 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Amitsuka: "Hidden Order and Weak Antiferromagnetism in URu_2Si_2"Physica B. 312-313. 390-396 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Sakakibara: "Magnetic Susceptibility of Ce_<0.75>La_<0.25>B_6 under Uniaxial Pressure"Physica B. 312-313. 194-196 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Matsuda: "The Appearance of Homogeneous Antiferromagnetism in URu_2Si_2 under High Pressure : a ^<29>Si Nuclear Magnetic Resonance Study"Journal of Physics : Condensed Matter. 15. 2363-2373 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] D.Kaczorowski: "Possible Heavy-Fermion Behavior in a Heusler-Type Compound YbPd_2Sb"Acta Physica Polonica B. 34. 1253-1256 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] P.Gegenwart: "Divergence of the Heavy Quasiparticle Mass at the Antiferromagnetic Quantum Critical Point in YbRh_2Si_2"Acta Physica Polonica B. 34. 323-334 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Oeschler: "UBe_<13> : Prototype of a Non-Fermi-Liquid Superconductor"Acta Physica Polonica B. 34. 255-274 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Amitsuka: "Inhomogeneous Magnetism in URu_2Si_2 Studied by Muon Spin Relaxation under High Pressure"Physica B. 326. 418-421 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] R.Giri: "Magnetic Properties of Sm-Based Filled Skutterudite Phosphides"Physica B. 329-333. 458-459 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Amitsuka: "Inhomogeneous Magnetism and Hidden Order in URu_2Si_2"Physica B. 329-333. 452-455 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yokoyama: "Nonequilibrium Antiferromagnetic State in the Heavy Electron Compound URu_2Si_2"Acta Physica Polonica B. 34. 1067-1070 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Kuwahara: "High Pressure X-Ray Diffraction Study of URu_2Si_2"Acta Physica Polonica B. 34. 4307-4310 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Tenya: "Low Temperature Magnetization of the Skutterudite Superconductor PrOs_4Sb_<12>"Acta Physica Polonica B. 34. 995-998 (2003)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yokoyama: "Neutron Scattering Study on Competition between Hidden Order and Antiferromagnetism in U(Ru_<1-x>Rh_x)_2Si_2 (x【less than or equal】0.05)"Journal of the Physical Society of Japan. 73. 545-548 (2004)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Matsuda: "Spatially Inhomogeneous Development of Antiferromagnetism in URu_2Si_2 : Evidence from ^<29>Si NMR under Pressure"Physical Review Letters. 87. 87203-1-87203-4 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Tayama: "Antiferro-Quadrupolar Ordering and Multipole interactions in PrPb_3"Journal of the Physical Society of Japan. 70. 248-258 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Nagata: "Antiferromagnetic Ordering in the Spin Ladder Compound ; Sr_<14-x>Ca_xCu_<24>O_<41>"Journal of the Physical Society of Japan. 70. 2419-2424 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yokoyama: "Anomalous Fermi Liquid Behavior of the Dilute Uranium Alloys La_<1-x>U_xRu_2Si_2 (x【less than or equal】0.07)"Journal of the Physical Society of Japan. 71. 3037-3042 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yokoyama: "Effects of Uniaxial Stress on Antiferromagnetic Moment in the Heavy Election Compound URu_2Si_2"Journal of the Physical Society of Japan. 71 Suppl. 264-266 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Amitsuka: "Low-Temperature Magnetization Study on the Non-Kramers Cubic System Pr_3Pd_<20>Ge_6"Journal of the Physical Society of Japan. 71 Suppl. 124-126 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Sakakibara: "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in Ce_xLa_<1-x>B_6"Journal of the Physical Society of Japan. 71 Suppl. 48-51 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Sakakibara: "Multipole Ordering to f Election Systems"Journal of Physics and Chemistry of Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] P.Gegenwart: "Magnetic-Field Induced Quantum Critical Point in YbRh_2Si_2"Physical Review Letters. 89. 056402-1-056402-4 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] F.Kromer: "Magnetic Field Response in (U,Th)Be_<13>"Journal of Low Temperature Physics. 126. 815-833 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Matsuhira: "Low-Temperature Magnetic Properties of Pyrochlore Stannates"Journal of the Physical Society of Japan. 71. 1576-1582 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Matsuda: "^<29>Si NMR Study of URu_2Si_2 under Pressure"Physica B. 312-313. 504-505 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yokoyama: "Thorium Dilution Effects of the Heavy Electron Compound URu_2Si_2"Physica B. 312-313. 498-500 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Amitsuka: "Hidden Order and Weak Antiferromagnetism in URu_2Si_2"Physica B. 312-313. 390-396 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Sakakibara: "Magnetic Susceptibility of Ce_<0.75>La_<0.25>B_6 under Uniaxial Pressure"Physica B. 312-313. 194-196 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Matsuda: "The Appearance of Homogeneous Antiferromagnetism in URu_2Si_2 under High Pressure a ^<29>Si Nuclear Magnetic Resonance Study"Journal of Physics : Condensed Matter. 15. 2363-2373 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] D.Kaczorowski: "Possible Heavy-Fermion Behavior in a Heusler-Type Compound YbPd_2Sb"Acta Physica Polonica B. 34. 1253-1256 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] P.Gegenwart: "Divergence of the Heavy Quasiparticle Mass at the Antiferromagnetic Quantum Critical Point in YbRh_2Si_2"Acta Physics Polonica B. 34. 323-334 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Oeschler: "UBe_<13> : Prototype of a Non-Fermi-Liquid Superconductor"Acta Physics Polonica B. 34. 255-274 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Amitsuka: "Inhomogeneous Magnetism in URu_2Si_2 Studied by Muon Spin Relaxation under High Pressure"Physica B. 326. 418-421 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] R.Giri: "Magnetic Properties of Sm-Based Filled Skutterudite Phosphides"Physica B. 329-333. 458-459 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Amitsuka: "Inhomogeneous Magnetism and Hidden Order in URu_2Si_2"Physica B. 329-333. 452-455 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yokoyama: "Nonequilibrium Antiferromagnetic State in the Heavy Electron Compound URu_2Si_2"Acta Physica Polonica B. 34. 1067-1070 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Kuwahara: "High Pressure X-Ray Diffraction Study of URu_2Si_2"Acta Physica Polonica B. 34. 4307-4310 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Tenya: "Low Temperature Magnetization of the Skutterudite Superconductor PrOs_4Sb_<12>"Acta Physica Polonica B. 34. 995-998 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yokoyama: "Neutron Scattering Study on Competition between Hidden Order and Antiferromagnetism in U(Ru_<1-x>Rh_x)_2Si_2 (x【less than or equal】0.05)"Journal of the Physical Society of Japan. 73. 545-548 (2004)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2005-04-19  

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