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2004 Fiscal Year Final Research Report Summary

Studies on shape resonance dynamics by photoelectron angular distribution measurements from oriented molecules

Research Project

Project/Area Number 14340126
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 物理学一般
Research InstitutionHigh Energy Accelerator Research Organization (2004)
The High Energy Accelerator Research Organization (2002-2003)

Principal Investigator

YAGISHITA Akira  High energy accelerator research organization, Institute of materials structure science, Prof., 物質構造科学研究所, 教授 (80157966)

Co-Investigator(Kenkyū-buntansha) TAKAHASHI Masahiko  Tohoku Univ, Institute of Multidisciplinary Research for Advanced Materials, Associate Prof., 多元物質科学研究所, 助教授 (80241579)
ADACHI Jun-ichi  High energy accelerator research organization, Institute of materials structure science, Res. Associate, 物質構造科学研究所, 助手 (10322629)
Project Period (FY) 2002 – 2004
Keywordsvelocity imaging / angular correlation / inversion symmetry / dissociation channel / triple coincidence / core-hole / 反転対称性 / 分子の構造変形
Research Abstract

We have successfully designed and constructed a new apparatus of coincidence velocity imaging spectrometer for the study of angular correlations between photoelectrons and photofragments.
Using this apparatus, we have measured momentum correlation patterns between O1s photoelectrons and photofragments of CO^+ and O^+ at the photon energy above the ionization threshold of O1s of CO_2 molecules. And we have found that the O1s photoelectron angular distribution pattern violate the inversion symmetry.
We have also succeeded in measuring the C1s photoelectron angular distribution patterns of C_2H_2 molecules for each dissociation channel by the triple coincidence. For asymmetric dissociation channels, the C 1s photoelectron angular distribution patterns violate the inversion symmetry. This implies that the core-hole memory is preserved in the photofragments.

  • Research Products

    (26 results)

All 2005 2004 2003 2002 Other

All Journal Article (26 results)

  • [Journal Article] Inner-shell photoelectron angular distributions from fixed-in-space OCS molecules2005

    • Author(s)
      A.V.Golovin
    • Journal Title

      J.Phys.B ; At.Mol.Opt.Phys. 38

      Pages: L63-L68

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Photoelectron angular distributions from fixed-in-space molecules2005

    • Author(s)
      A.Yagishita
    • Journal Title

      Journal of Electron Spectroscopy and Relat.Phenom. 142

      Pages: 295-312

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Symmetry-resolved soft x-ray absorption spectroscopy ; its application to simple molecules2005

    • Author(s)
      J.Adachi
    • Journal Title

      J.Phys.B ; At.Mol.Opt.Phys. 38(in press)

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Inner-shell photoelectron angular distributions from fixed-in-space OCS molecules2005

    • Author(s)
      A.V.Golovin, J.Adachi, S.Motoki, M.Takahashi, A.Yagishita
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys 38

      Pages: L63-L68

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Photoelectron angular distributions from fixed-in-space molecules2005

    • Author(s)
      A.Yagishita, H.Hosaka, J.Adachi
    • Journal Title

      Journal of Electron Spectroscopy and Relat. Phenom. 142

      Pages: 295-312

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Multiplet-specific N 1s photoelectron angular distributions from the fixed-in-space NO molecules2004

    • Author(s)
      K.Hosaka
    • Journal Title

      J.Phys.B ; At.Mol.Opt.Phys. 37

      Pages: L47-L55

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Angular distributions of vibrationally-resolved C 1s photoelectrons from fixed-in-space CO molecules : vibrational effect in the shape-resonant C 1s photoionization of CO2004

    • Author(s)
      J.Adachi
    • Journal Title

      Journal of Electron Spectroscopy and Relat.Phenom. 137

      Pages: 243-248

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Multiple photoionization following 3d_<5/2>-shell threshold ionization of Xe2004

    • Author(s)
      T.Matsui
    • Journal Title

      J.Phys.B ; At.Mol.Opt.Phys. 37

      Pages: 3745-3752

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] O K-shell photoemission of the CO molecule : comparison between theory and experiment2004

    • Author(s)
      N.A.Cherepkov
    • Journal Title

      J.Phys.B ; At.Mol.Opt.Phys. 37

      Pages: 4803-4815

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Multiplet-specific N 1s photoelectron angular distributions from the fixed-in-space NO molecules2004

    • Author(s)
      K.Hosaka, J.Adachi, M.Takahashi, A.Yagishita, P.Lin, R.R.Lucchese
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 37

      Pages: L47-L55

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Angular distributions of vibrationally-resolved C 1s photoelectrons from fixed-in-space CO molecules : vibrational effect in the shape-resonant C 1s photoionization of CO2004

    • Author(s)
      J.Adachi, K.Hosaka, S.Furuya, K.Soejima, M.Takahashi, A.Yagishita, S.K.Semenov, N.A.Cherepkov
    • Journal Title

      Journal of Electron Spectroscopy and Relat. Phenom. 137

      Pages: 243-248

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Multiple photoionization following 3d_<5/2>-shell threshold ionization of Xe.2004

    • Author(s)
      T.Matsui, H.Yoshiki, K.Tsukamoto, S.Kawakita, E.Murakami, J.Adachi, A.Yagishita, Y.Morioka, T.Hayaishi
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 37

      Pages: 3745-3752

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] O K-shell photoemission of the CO molecule : comparison between theory and experiment2004

    • Author(s)
      N.A.Cherepkov, S.K.Semenov, A.V.Golovin, J.Adachi, A.Yagishita
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 37

      Pages: 4803-4815

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Shape-Resonance-Enhanced Vibrational Effects in the Angular Distributions of C 1s Photoelectrons from Fixed-in-Space CO Molecules2003

    • Author(s)
      J.Adachi
    • Journal Title

      Phys.Rev.Lett. 91

      Pages: 163001-1-163001-4

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] N 1s photoionization cross sections of nitric oxide molecules in the shape resonance region2003

    • Author(s)
      K.Hosaka
    • Journal Title

      J.Phys.B ; At.Mol.Opt.Phys. 36

      Pages: 4617-4629

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Shape-Resonance-Enhanced Vibrational Effects in the Angular Distributions of C 1s Photoelectrons from Fixed-in-Space CO Molecules2003

    • Author(s)
      J.Adachi, K.Hosaka, S.Furuya, K.Soejima, M.Takahashi, A.Yagishita, S.K.Semenov, N.A.Cherepkov
    • Journal Title

      Phys. Rev. Lett. 91

      Pages: 163001-1-4

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] N 1s photoionization cross sections of nitric oxide molecules in the shape resonance region2003

    • Author(s)
      K.Hosaka, J.Adachi, M.Takahashi, A.Yagishita
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 36

      Pages: 4617-4629

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Double photoionization of helium at an excess energy of 60 eV using left-and right-elliptically-polarized light2002

    • Author(s)
      S.A.Collins
    • Journal Title

      Phys.Rev.A 65

      Pages: 052717-1-052717-8

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Cascade processes after 3p-shell threshold photoionization of Kr2002

    • Author(s)
      T.Matsui
    • Journal Title

      J.Phys.B : At.Mol.Opt.Phys. 35

      Pages: 3069-3075

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Complete photoionization experiment in the region of the 2□_g□ □_u shape resonance of the N_2 molecule2002

    • Author(s)
      S.Motoki
    • Journal Title

      J.Phys.B : At.Mol.Opt.Phys. 35

      Pages: 3801-3819

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Characterization of □_u shape resonance in the C 1s ionization continuum of CO_2 molecules.2002

    • Author(s)
      J.Adachi
    • Journal Title

      J.Phys.B : At.Mol.Opt.Phys. 35

      Pages: 5023-5033

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Double photoionization of helium at an excess energy of 60 eV using left-and right-elliptically-polarized light2002

    • Author(s)
      S.A.Collins, S.Cvejanovic, C.Dawson, T.J.Reddish, D.P.Seccombe, A.Huetz, L.Malegat, P.Selles, A.K.Kazansky, A.Danjo, K.Soejima, K.Okuno, A.Yagishita
    • Journal Title

      Phys. Rev. A 65

      Pages: 052717-1-8

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Cascade processes after 3p-shell threshold photoionization of Kr.2002

    • Author(s)
      T.Matsui, H.Yoshii, A.Higurashi, E.Murakami, T.Aoto, T.Onuma, Y.Morioka, A.Yagishita, T.Hayaishi
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 35

      Pages: 3069-3075

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Complete photoionization experiment in the region of the 2□_g□ □_u shape resonance of the N_2 molecule2002

    • Author(s)
      S.Motoki, J.Adachi, K, Ito, K.Ishii, K.Soejima, A.Yagishita, S.K.Semenov, N.A.Cherepkov
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 35

      Pages: 3801-3819

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Characterization of of □_u shape resonance in the C 1s ionization continuum of CO_2 molecules2002

    • Author(s)
      J.Adachi, S.Motoki, N.A.Cherepkov, A.Yagishita
    • Journal Title

      J. Phys. B ; At. Mol. Opt. Phys. 35

      Pages: 5023-5033

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Symmetry-resolved soft x-ray absorption spectroscopy ; its application to simple molecules

    • Author(s)
      J.Adachi, N.Kosugi, A.Yagishita
    • Journal Title

      J. Phys. B; At. Mol. Opt. Phys (in press)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2006-07-11  

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