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2005 Fiscal Year Final Research Report Summary

New Developments in the Theory of Non-Magnetic Ground State and Magnetic-Field-Induced Spin Gap in Low Dimensional Spin Systems

Research Project

Project/Area Number 14540329
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionTokyo Institute of Technology

Principal Investigator

OKAMOTO Kiyomi  Tokyo Institute of Technology, Graduate School of Science and Engineering, Assistant Professor, 大学院・理工学研究科, 助手 (40152342)

Project Period (FY) 2002 – 2005
Keywordslow-dimensional magnets / spin chain / quantum phase transition / spin gap / magnetization plateau / magnetization curve
Research Abstract

By use of analytical and numerical methods, we have investigated the ground states with zero or finite magnetic fields for various one-dimensional and quasi-one-dimensional spin systems. Especially, we have focused on the spin-gap states in zero or finite magnetic fields.
1. We have proposed several mechanisms for the magnetic-filed-induced spin gap at 1/4 of the saturation magnetization of a ladder type organic spin system BIP-TENO. We have succeeded to explain the behavior of the observed magnetization curve.
2. We have studied the distorted diamond type spin chain, by use of analytical and numerical methods, especially focusing on the ground states in zero and finite magnetic field. In this system, there appears various phases depending upon the quantum parameters. In particular, it was found the change in the mechanism for the magnetization plateau at 1/3 of the saturation magnetization. The magnetic properties of azurite are well described by this model.
3. We have obtained the definitive conclusion on the phase diagram of the spin ladder with the bond alternation.
4. We have found the inversion phenomenon between the anisotropies of the Hamiltonian and the wave function for the spin systems with three keywords : trimer nature, frustration and the XXZ anisotropy of the spin-spin interactions. Namely, in some regions of the quantum parameters, the Neel ground state is realized in spite of the fact that the interactions is XY-like. And also, the spin-fluid ground state is realized when the interaction is Ising-like.
5. We have clarified the condition for the appearance of the spin orderng which is incommensurate to the lattice for the material F5PNN.

  • Research Products

    (61 results)

All 2006 2005 2004 2003 2002 Other

All Journal Article (61 results)

  • [Journal Article] Possibility of field-induced incommensurate order in quasi-one-dimensional frustrated spin system2006

    • Author(s)
      N.Maeshima, K.Okunishi, K.Okamoto, 他
    • Journal Title

      J.Phys. : Condensed Matter 18・20

      Pages: 4819-4826

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Possibility of field-induced incommensurate order in quasi-one-dimensional frustrated spin system2006

    • Author(s)
      N.Maeshima et al.
    • Journal Title

      J.Phys. : Condensed Matter 18

      Pages: 4819-4826

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Half plateau phase diagram in generalized zig-zag spin ladder2005

    • Author(s)
      A.Tokuno, K.Okamoto, T.Tonegawa
    • Journal Title

      Prog. Theor. Phys. Suppl. 159

      Pages: 265-270

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization Plateau of $S=1$ Spin Ladder BIP-TENO2005

    • Author(s)
      M.Kikuchi, K.Okamoto, K.Okunishi, T.Sakai
    • Journal Title

      Prog. Theor. Phys. Suppl. 159

      Pages: 251-255

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Ground-State Phase Diagram of the S=1/2 Distorted Diamond Type Spin Chain with Ferromagnetic Interactions2005

    • Author(s)
      K.Okamoto, T.Tonegawa, T.Yamada, 他
    • Journal Title

      Prog. Theor. Phys. Suppl. 159

      Pages: 17-21

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetic Properties of the Diamond Chain Compound Cu_3(CO_3)_2(OH)_22005

    • Author(s)
      H.Kikuchi他
    • Journal Title

      Prog. Theor. Phys. Suppl. 159

      Pages: 1-10

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Energy Gap of Spin Nanotube2005

    • Author(s)
      T.Sakai, M.Matsumoto, K.Okunishi, K.Okamoto, 他
    • Journal Title

      Physica E 23・3-4

      Pages: 633-636

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Field-Induced Incommensurate Order in Spin Ladder with Ring Exchange2005

    • Author(s)
      T.Sakai, K.Okamoto
    • Journal Title

      J. Phys. Chem. Solids 66・8-9

      Pages: 1442-1445

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Bond-Alternating S = 1 Spin Ladder in Magnetic Field2005

    • Author(s)
      M.Kikuchi, K.Okamoto, K.Okunishi, T.Sakai
    • Journal Title

      J. Phys. Chem. Solids 74・Supp1

      Pages: 169-172

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization Plateaux of an S=1 Frustrated Spin Ladder2005

    • Author(s)
      K.Okamoto, K.Okunishi, T.Sakai
    • Journal Title

      J. Phys. Soc. Jpn. 74・Supp1

      Pages: 165-168

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Finite-Field Ground State of the S=1 Antiferromagnetic-Ferromagnetic Bond-Altermating Chain2005

    • Author(s)
      T.Tonegawa, K.Okamoto, M.Kaburagi
    • Journal Title

      J. Phys. Soc. Jpn. 74・Supp1

      Pages: 161-164

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Inversion phenomena and phase diagram of the S =1/2 distorted diamond chain with the XXZ interaction anisotropy2005

    • Author(s)
      A.Tokuno, K.Okamoto
    • Journal Title

      J. Phys. Soc. Jpn. 74・Suppl

      Pages: 157-160

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Field-induced phase transitions and long-range orders in the S=1/2 spin bond-alternating chain with frustrating interaction2005

    • Author(s)
      N.Maeshima他
    • Journal Title

      J. Phys. Soc. Jpn. 74・Suppl

      Pages: 63-66

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Experimental Observation of the 1/3 Magnetization Plateau in a Diamond Chain Compound Cu_3(CO_3)_2(OH)_22005

    • Author(s)
      H.Kikuchi他
    • Journal Title

      Phys. Rev. Lett. 94

      Pages: 227201-1-4

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Half plateau phase diagram in generalized zig-zap spin ladder2005

    • Author(s)
      A.Tokuno, K.Okamoto, T.Tonegawa
    • Journal Title

      Prog.Theor.Phys.Suppl. 159

      Pages: 265-270

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization Plateau of $S=1$ Spin Ladder BIP-TENO2005

    • Author(s)
      M.Kikuchi, K.Okamoto, K.Okunishi, T.Sakai
    • Journal Title

      Prog.Theor.Phys.Suppl. 159

      Pages: 251-255

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Ground-State Phase Diagram of the S=1/2 Distorted Diamond Type Spin Chain with Ferromagnetic Interactions2005

    • Author(s)
      K.Okamoto et al.
    • Journal Title

      Prog.Theor.Phys.Suppl. 159

      Pages: 17-21

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetic Properties of the Diamond Chain Compound Cu_3(CO_3)2(OH)22005

    • Author(s)
      H.Kikuchi et al.
    • Journal Title

      Prog.Theor.Phys.Suppl. 159

      Pages: 1-10

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Energy Gap of Spin Nanotube2005

    • Author(s)
      T.Sakai et al.
    • Journal Title

      Physica E 23

      Pages: 633-636

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Field-Induced Incommensurate Order in Spin Ladder with Ring Exchange2005

    • Author(s)
      T.Sakai, K.Okamoto
    • Journal Title

      J.Phys.Chem.Solids 66

      Pages: 1442-1445

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Bond-Alternating S=1 Spin Ladder in Magnetic Field2005

    • Author(s)
      M.Kikuchi et al.
    • Journal Title

      J.Phys.Soc.Jpn. 74 Suppl.

      Pages: 169-172

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization Plateaux of an S=1 Frustrated Spin Ladder2005

    • Author(s)
      K.Okamoto, K.Okunishi, T.Sakai
    • Journal Title

      J.Phys.Soc.Jpn. 74 Suppl.

      Pages: 165-168

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Finite-Field Ground State of the S=1 Antiferromagnetic-Ferromagnetic Bond-Alternating Chain2005

    • Author(s)
      T.Tonegawa, K.Okamoto, M.Kaburagi
    • Journal Title

      J.Phys.Soc.Jpn. 74 Suppl.

      Pages: 161-164

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Inversion phenomena and phase diagram of the S=1/2 distorted diamond chain with the XXZ interaction anisotropy2005

    • Author(s)
      A.Tokuno, K.Okamoto
    • Journal Title

      J.Phys.Soc.Jpn. 74 Suppl.

      Pages: 157-160

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Field-induced phase transitions and long-range order in the S=1/2 spin bond-alternating chain with frustrating interaction2005

    • Author(s)
      N.Maeshima et al.
    • Journal Title

      J.Phys.Soc.Jpn. 74 Suppl.

      Pages: 63-66

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Experimental Observation of the 1/3 Magnetization Plateau in a Diamond Chain Compound Cu_3(CO_3)2(OH)_22005

    • Author(s)
      H.Kikuchi et al.
    • Journal Title

      Phys.Rev.Lett. 94

      Pages: 227201-1-227201-4

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Frustration-Induced η in the S=1/2 Bond-Alternating Spin Chain2004

    • Author(s)
      N.Maeshima, K.Okunishi, K.Okamoto, T.Sakai
    • Journal Title

      Phys. Rev. Lett. 93・12

      Pages: 127203-1-4

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization Plateau and Cusp in S=1 Spin Ladder2004

    • Author(s)
      T.Sakai他
    • Journal Title

      Physica B 346-347

      Pages: 34-37

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization plateau in an anisotropic S=1/2 antiferromagnetic chain with frustration and bond-alternation2004

    • Author(s)
      T.Tonegawa他
    • Journal Title

      Physica B 346-347

      Pages: 50-54

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Anomalous magnetization process in frustrated spin ladders2004

    • Author(s)
      T.Sakai, K.Okamoto, K.Okunishi, M.Sato
    • Journal Title

      J. Phys. : Cond. Matter 16・11

      Pages: S785-S789

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Frustration-Induced eta Inversion in the S=1/ Bond-Alternating Spin Chain2004

    • Author(s)
      N.Maeshima, K.Okunishi, K.Okamoto, T.Sakai
    • Journal Title

      Phys.Rev.Lett. 93

      Pages: 127203-1-127203-4

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization Plateau and Cusp in S=1 Spin Ladder2004

    • Author(s)
      T.Sakai et al.
    • Journal Title

      Physica B 364-347

      Pages: 34-37

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization plateau in an anisotropic S=1/2 antiferromagnetic chain with frustration and bond-alternation2004

    • Author(s)
      T.Tonegawa et al.
    • Journal Title

      Physica B 346-347

      Pages: 50-54

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Anomalous magnetization process in frustrated spin ladders2004

    • Author(s)
      T.Sakai, K.Okamoto, K.Okunishi, M.Sato
    • Journal Title

      J.Phys. : Cond.Matter 16

      Pages: S785-S789

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetic Properties of S=1/2 Distorted Diamond Chain2003

    • Author(s)
      K.Okamoto, T.Tonegawa, M.Maburagi
    • Journal Title

      J. Phys. : Condesed Matter 15・35

      Pages: 5979-5995

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Spin-Peierls Mechanism for the Non-Trivial Magnetization Plateaux in Two-Leg Spin Ladders2003

    • Author(s)
      K.Okamoto, T.Sakai
    • Journal Title

      Physica B 329-333・2

      Pages: 1207-1208

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization Plateaux in S=1 Organic Spin Ladder BIP-TENO2003

    • Author(s)
      T.Sakai, 他
    • Journal Title

      Physica B 329-333・2

      Pages: 1203-1204

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Phase diagram of the S=1/2 two-leg spin ladder with staggered bond alternation2003

    • Author(s)
      K.Okamoto
    • Journal Title

      Phys. Rev. B 67・21

      Pages: 212408-1-3

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization Plateaux in S=1 Spin Ladder2003

    • Author(s)
      T.Sakai, 他
    • Journal Title

      Phys. Status Sol. (b) 236・2

      Pages: 429-432

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetic Properties of S=1/2 Distorted Diamond Chain2003

    • Author(s)
      K.Okamoto, T.Tonegawa, M.Kaburagi
    • Journal Title

      J.phys. : Cond.Matter 15

      Pages: 5979-5995

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Spin-Peierls Mechanism for the Non-Trivial Magnetization Plateaux in Two-Leg Spin Ladders2003

    • Author(s)
      K.Okamoto, T.Sakai
    • Journal Title

      Physica B 329-333

      Pages: 1207-1208

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization Platezux in S=1 Organic Spin Ladder BIP-TENO2003

    • Author(s)
      T.Sakai et al.
    • Journal Title

      Physica B 329-333

      Pages: 1203-1204

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Phase diagram of the S=1/2 two-leg spin ladder with staggered bond alternation2003

    • Author(s)
      K.Okamoto
    • Journal Title

      Phys.Rev.B 67

      Pages: 212408-1-212408-3

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization Plateaux in S=1 Spin Ladder2003

    • Author(s)
      T.Sakai et al.
    • Journal Title

      Phys.Status Sol.(b) 236

      Pages: 429-432

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Field-Induced Transitions and Spin Gaps in Low-Dimensional Quantum Antiferromagnets2002

    • Author(s)
      T.Sakai, K.Okamoto, N.Okazaki
    • Journal Title

      Proceedings of French-Japanese Symposium on Quantum Properties of Low-Dimensional Antiferromagnets

      Pages: 62-69

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Anisotropies of the Hamiltonian and the Wave Function --- Inversion Phenonema in Quantum Spin Chains2002

    • Author(s)
      K.Okamoto
    • Journal Title

      Prog. Theor. Phys. Suppl. 145

      Pages: 208-211

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Level Spectroscopy : Physical Meaning and Application to Magnetization Plateaux2002

    • Author(s)
      K.Okamoto
    • Journal Title

      Prog. Theor. Phys. Suppl. 145

      Pages: 113-118

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Inversion Phenomena of the Anisotropies of the Hamiltonian and the Wave-Function in the Distorted Diamond Type Spin Chain2002

    • Author(s)
      K.Okamoto, Y.Ichikawa
    • Journal Title

      J. Phys. Chem. Solids 63・6-8

      Pages: 1575-1578

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Magnetization Plateau in the S=1 Spin Ladder with Competing Interactions2002

    • Author(s)
      N.Okazaki, K.Okamoto, T.Sakai
    • Journal Title

      J. Phys. Chem. Solids 63・6-8

      Pages: 1455-1458

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Mechanisms for Non-Trivial Magnetization Plateaux of an S=1 Frustrated Spin Ladder2002

    • Author(s)
      K.Okamoto, N.Okazaki, T.Sakai
    • Journal Title

      J. Phys. Soc. Jpn. Suupl. 71

      Pages: 196-198

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Quantum Magnetization plateaux of an anisotropic ferrimagnetic spin chain2002

    • Author(s)
      T.Sakai, K.Okamoto
    • Journal Title

      Physs. Rev. B 65・21

      Pages: 214403-214408

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Anisotropies of the Hamiltonian and the Wave Function --- Inversion Phenonema in Quantum Spin Chains2002

    • Author(s)
      K.Okamoto
    • Journal Title

      Prog.Theor.Phys.Suppl. 145

      Pages: 208-211

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Level Spectroscopy : Physical Meaning and Application to Magnetization Plateaux2002

    • Author(s)
      K.Okamoto
    • Journal Title

      Prog.Theor.Phys.Suppl. 145

      Pages: 113-118

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Inversion Phenomena of the Anisotropies of the Hamiltonian and the Wave-Function in the Distorted Diamond Type Spin Chain2002

    • Author(s)
      K.Okamoto, Y.Ichikawa
    • Journal Title

      J.Phys.Chem.Solids 63

      Pages: 1575-1578

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Magnetization Plateau in the S=1 Spin Ladder with Competing Interactions2002

    • Author(s)
      N.Okazaki, K.Okamoto, T.Sakai
    • Journal Title

      J.Phys.Chem.Solids 63

      Pages: 1455-1458

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Mechanisms for Non-Trivial Magnetization Plateaux of an S=1 Frustrated Spin Ladder2002

    • Author(s)
      K.Okamoto, N.Okazaki, T.Sakai
    • Journal Title

      J.Phys.Soc.Jpn.Suupl. 71

      Pages: 196-98

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Quantum Magnetization Plateaux of an anisotropic ferrimagnetic spin chain2002

    • Author(s)
      T.Sakai, K.Okamoto
    • Journal Title

      Physs.Rev.B 65

      Pages: 214403-214408

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Theory of Excitation Modes in Diamond Chain Compound Cu_3(CO_3)_2(OH)_2

    • Author(s)
      M.Matsumoto, T.Yamada, K.Koga, K.Okamoto, T.Sakai
    • Journal Title

      Physica B (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Field-Induced Incommensurate Order in Quai-1D S=1 Antiferromagnet

    • Author(s)
      T.Sakai, K.Okamoto, K.Okunishi, T.Tonegawa
    • Journal Title

      LT24 proceedings (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Theory of Excitation Modes in diamond Chain compound Cu_3(CO_3)_2(OH)_2

    • Author(s)
      M.Matsumoto, T.Yamada, K.Koga, K.Okamoto, T.Sakai
    • Journal Title

      Physica B (in press)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Field-Induced Incommensurate Order in Quai-1D S=1 Antiferromagnet

    • Author(s)
      T.Sakai, K.Okamoto, K.Okunishi, T.Tonegawa
    • Journal Title

      LT24 proceedings (in press)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2007-12-13  

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