ハロゲン化鉛ペロブスカイトメソ多孔体の合成

2017 Fiscal Year Annual Research Report

• Project/Area Number: 16F16050
• Research Institution: National Institute for Materials Science
• Principal Investigator: 山内 悠輔 国立研究開発法人物質・材料研究機構, 国際ナノアーキテクトニクス研究拠点, MANA主任研究者 (10455272)
• Co-Investigator(Kenkyū-buntansha): MALGRAS VICTOR 国立研究開発法人物質・材料研究機構, 国際ナノアーキテクトニクス研究拠点, 外国人特別研究員
• Project Period (FY): 2016-04-22 – 2018-03-31
• Keywords: Mesoporous materials

Outline of Annual Research Achievements

Mainly we carried the research on mesoporous template/perovskite composite using thin film technology. More precisely, we synthesized film with hierarchical pore structures (8 and 3 nm diameters), which greatly enhances the precursor solution penetration through the template. The composite has a high concentration of small crystals (3 nm) which dominates the optical properties. Strong quantum confinement is observed as well as increased photoluminescence quantum efficiency. These preliminary results are encouraging for future works related to integration of such composite in light emitting devices.

Research Progress Status

29年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

29年度が最終年度であるため、記入しない。

Research Products

• [Journal Article] Hierarchical porous carbons with layer-by-layer motif architectures from confined soft-template self-assembly in layered materials (2017)
  • Author(s): Wang Jie, Tang Jing, Ding Bing, Malgras Victor, Chang Zhi, Hao Xiaodong, Wang Ya, Dou Hui, Zhang Xiaogang, Yamauchi Yusuke
  • Journal Title: Nature Communications Volume: 8 Pages: 15717～15717
  • DOI: 10.1038/ncomms15717
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Perfectly ordered mesoporous iron-nitrogen doped carbon as highly efficient catalyst for oxygen reduction reaction in both alkaline and acidic electrolytes (2017)
  • Author(s): Tan Haibo, Li Yunqi, Jiang Xiangfen, Tang Jing, Wang Zhongli, Qian Huayu, Mei Peng, Malgras Victor, Bando Yoshio, Yamauchi Yusuke
  • Journal Title: Nano Energy Volume: 36 Pages: 286～294
  • DOI: 10.1016/j.nanoen.2017.04.014
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Hollow carbon nanobubbles: monocrystalline MOF nanobubbles and their pyrolysis (2017)
  • Author(s): Zhang Wei, Jiang Xiangfen, Zhao Yanyi, Carne-Sanchez Arnau, Malgras Victor, Kim Jeonghun, Kim Jung Ho, Wang Shaobin, Liu Jian, Jiang Ji-Sen, Yamauchi Yusuke, Hu Ming
  • Journal Title: Chemical Science Volume: 8 Pages: 3538～3546
  • DOI: 10.1039/C6SC04903F
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Effect of Various Carbonization Temperatures on ZIF-67 Derived Nanoporous Carbons (2017)
  • Author(s): Guo Yanna, Tang Jing, Salunkhe Rahul R., Alothman Zeid Abdullah, Hossain Md. Shahriar A., Malgras Victor, Yamauchi Yusuke
  • Journal Title: Bulletin of the Chemical Society of Japan Volume: 90 Pages: 939～942
  • DOI: 10.1246/bcsj.20170138
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Layer-by-Layer Motif Architectures: Programmed Electrochemical Syntheses of Multilayer Mesoporous Metallic Films with Uniformly Sized Pores (2017)
  • Author(s): Jiang Bo, Li Cuiling, Qian Huayu, Hossain Md. Shahriar A., Malgras Victor, Yamauchi Yusuke
  • Journal Title: Angewandte Chemie International Edition Volume: 56 Pages: 7836～7841
  • DOI: 10.1002/anie.201703609
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Continuous Mesoporous Pd Films by Electrochemical Deposition in Nonionic Micellar Solution (2017)
  • Author(s): Iqbal Muhammad, Li Cuiling, Wood Kathleen, Jiang Bo, Takei Toshiaki, Dag Omer, Baba Daisuke, Nugraha Asep Sugih, Asahi Toru, Whitten Andrew E., Hossain Md. Shahriar A., Malgras Victor, Yamauchi Yusuke
  • Journal Title: Chemistry of Materials Volume: 29 Pages: 6405～6413
  • DOI: 10.1021/acs.chemmater.7b01811
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Hybrid methylammonium lead halide perovskite nanocrystals confined in gyroidal silica templates (2017)
  • Author(s): Malgras Victor, Henzie Joel, Takei Toshiaki, Yamauchi Yusuke
  • Journal Title: Chem Commun Volume: 53 Pages: 2359～2362
  • DOI: 10.1039/C6CC10245J
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Periodically Arranged Arrays of Dendritic Pt Nanospheres Using Cage-Type Mesoporous Silica as a Hard Template (2017)
  • Author(s): Kani Kenya, Malgras Victor, Jiang Bo, Hossain Md. Shahriar A., Alshehri Saad M., Ahamad Tansir, Salunkhe Rahul R., Huang Zhenguo, Yamauchi Yusuke
  • Journal Title: Chemistry - An Asian Journal Volume: 13 Pages: 106～110
  • DOI: 10.1002/asia.201701393
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Understanding chemically processed solar cells based on quantum dots (2017)
  • Author(s): Malgras Victor, Nattestad Andrew, Kim Jung Ho, Dou Shi Xue, Yamauchi Yusuke
  • Journal Title: Science and Technology of Advanced Materials Volume: 18 Pages: 334～350
  • DOI: 10.1080/14686996.2017.1317219
  • Peer Reviewed / Int'l Joint Research
• [Journal Article] Prussian blue derived iron oxide nanoparticles wrapped in graphene oxide sheets for electrochemical supercapacitors (2017)
  • Author(s): Tanaka Shunsuke, Salunkhe Rahul R., Kaneti Yusuf Valentino, Malgras Victor, Alshehri Saad M., Ahamad Tansir, Zakaria Mohamed B., Dou Shi Xue, Yamauchi Yusuke, Hossain Md. Shahriar A.
  • Journal Title: RSC Advances Volume: 7 Pages: 33994～33999
  • DOI: 10.1039/C7RA03179C
  • Peer Reviewed / Int'l Joint Research