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2005 Fiscal Year Annual Research Report

電子機能物質における自己組織化の解明と応用

Research Project

Project/Area Number 16GS0219
Research InstitutionThe Institute of Physical and Chemical Research

Principal Investigator

加藤 礼三  独立行政法人理化学研究所, 加藤分子物性研究室, 主任研究員 (80169531)

Co-Investigator(Kenkyū-buntansha) 古崎 昭  独立行政法人理化学研究所, 古崎物性理論研究室, 主任研究員 (10238678)
塚越 一仁  独立行政法人理化学研究所, 河野低温物理研究室, 先任研究員 (50322665)
辛 埴  国立大学法人東京大学, 物性研究所, 教授 (00162785)
高木 英典  国立大学法人東京大学, 新領域創成科学研究科, 教授 (40187935)
桃井 勉  独立行政法人理化学研究所, 古崎物性理論研究室, 先任研究員 (80292499)
Keywords電子機能物質 / 自己組織化 / 分子性導体 / 遷移金属酸化物 / 強相関電子系 / 光電子分光 / 電荷密度波 / フラストレーション
Research Abstract

光学伝導度測定から、分子性導体中の絡み合う電子のコヒーレンス(準粒子状態形成)の発達過程のエネルギー階層を明らかにした。同様の測定から幾何学的フラストレーションが強く支配する無機酸化物LiV_2O_4の重い電子状態形成が同じ物理で理解できることを示し、コヒーレンスの物理の普遍性を確立した。また、層状Ru酸化物の表面において系の臨界性を反映した、電子の自己組織化を発見した。
電荷密度波を生じる有機および無機物質について、超高分解能光電子分光を行い、電荷密度波についての知見を得た。TTF-TCNQ、K_<0.3>MoO_3では2次元的なフェルミ面が低温で1次元的になること、ZrTe_3においては1次元的なフェルミ面と3次元的なフェルミ面との共存を明らかにした。
有機エレクトロニクスの伝導特性の基礎となる界面効果の評価と特性制御を行った。有機トランジスタにおいて電極と有機薄界面や基板表面と有機薄膜界面の状態によって電界効果移動度が大きく依存することを見出し、ナノスケールの分子薄膜を導入することによって制御への可能性を見出した。一方、シリコン基板上で化学反応や電気分解を直接行い、電極と基板に密着した微小サイズの分子性導体単結晶を作製する手法を開発した。
カーボンナノチューブ等で実現する一次元電子系の電気伝導に対する磁場効果を、電子間斥力による繰り込みを考慮して理論解析した。また、フラストレーションをもつ強相関電子系における電荷・スピン・軌道・格子の自由度の競合と協調の効果を理論的に調べた。特に、強磁性揺らぎの強い系において、強磁性がフラストレーションにより壊された時に実現する量子スピン液体状態が、スピンのネマティック状態であることを明らかにした。さらに、フラストレーションの強い模型である2次元チェッカーボード格子上の反強磁性体について、その基底状態相図を決定した。

  • Research Products

    (51 results)

All 2006 2005 Other

All Journal Article (48 results) Patent(Industrial Property Rights) (3 results)

  • [Journal Article] Nematic order in square lattice frustrated ferromagnets2006

    • Author(s)
      N.Shannon, T.Momoi, P.Sindzingre
    • Journal Title

      Phys. Rev.Lett. 96・2

      Pages: 027213(4)

  • [Journal Article] Phase-change magnetic memory effect in cation-deficient iron sulfide Fe_<1-x>S2006

    • Author(s)
      K.Takenaka, H.Takagi
    • Journal Title

      Applied Physics Letters 88/1

      Pages: 012512(3)

  • [Journal Article] Shubnikov-de Haas Effect and Angular-dependent Magnetoresistance in New Layered Organic Conductors ET_3Cl(DFBIB) and ET_3Br(pBIB)2005

    • Author(s)
      S.Yasuzuka, S.Uji, H.M.Yamamoto, J-I.Yamaura, C.Terakura, T.Terashima, T.Yakabe, Y.Terai, R.Maeda, R.Kato
    • Journal Title

      J.Phys.Soc.Jpn 74

      Pages: 679-685

  • [Journal Article] Effect of Hydrostatic Pressure on Molecular Conductors, Pd(dmit)_2 Salts2005

    • Author(s)
      Y.Ishii, M.Tamura, R.Kato, M.Hedo, Y.Uwatoko, N.Mori
    • Journal Title

      Synth.Met. 152

      Pages: 389-392

  • [Journal Article] Novel phase transition in Et_2Me_2Pb〔Pd(dmit)_2〕_2 at 70 K : A possible mechanism based on strong dimerization of two-level molecules2005

    • Author(s)
      Masafumi Tamura, Akiko Tajima, Reizo Kato
    • Journal Title

      Synth.Met. 152

      Pages: 397-400

  • [Journal Article] Pressure Effect on Fermi Surface in β"-(ET)(TCNQ)"2005

    • Author(s)
      S.Yasuzuka, S.Uji, K.Enomoto, T.Konoike, M.Nishimura, T.Terashima, D.Graf, E.S.Choi, J.S.Brooks, H.M.Yamamoto, R.Kato
    • Journal Title

      Synth.Met. 152

      Pages: 437-440

  • [Journal Article] Fermi Surface Study of β"-(BEDT-TTF)(TCNQ) by Magnetooptical Measurements2005

    • Author(s)
      M.Kimata, Y.Oshima, K.Koyama, H.Ohta, M.Motokawa, H.M.Yamamoto, R.Kato
    • Journal Title

      Synth.Met. 153

      Pages: 369-372

  • [Journal Article] Control of the electronic state in a series of Pd(dmit)_2 salts, a strongly correlated electron system with a quasi-triangular lattice structure2005

    • Author(s)
      R.Kato, A.Tajima, A.Nakao, N.Tajima, N.Tamura, J.Yamaura
    • Journal Title

      Synth.Met. 153

      Pages: 397-400

  • [Journal Article] Electronic Properties of a New Layered Organic Conductor, (BEDT-TTF)_3Br(pBIB)2005

    • Author(s)
      T.Takahashi, S.Suzuki, K.Hiraki, H.M.Yamamoto, R.Kato
    • Journal Title

      Synth.Met. 153

      Pages: 401-404

  • [Journal Article] Structures and electrical conductivities of cation radical salts based on unsymmetrical 〔Au(III)(C-N) (S-S)〕 type dithiolate complexes2005

    • Author(s)
      Kazuya Kubo, Akiko Nakao, Yasuyuki Ishii, Reizo Kato, Gen-etsu Matsubayashi
    • Journal Title

      Synth.Met. 153

      Pages: 425-428

  • [Journal Article] Alignment-Free Top-Contact Formation for Organic Thin Film2005

    • Author(s)
      I..Yagi, K.Shigeto, K.Tsukagoshi, Y.Aoyagi
    • Journal Title

      Japanese Journal of Applied Physics (Express Letter) 44

      Pages: L479-L481

  • [Journal Article] Pentacene transistor encapsulated by poly-para-xylylene behaving as gate dielectric insulator and passivation film2005

    • Author(s)
      K.Tsukahoshi, I.Yagi, K.Shigeto, K.Yamagisawa, J.Tanabe, Y.Aoyagi
    • Journal Title

      Applied Physics Letters 87

      Pages: 183502

  • [Journal Article] Hall effect of quasi-hole gas in organic single-crystal transistors2005

    • Author(s)
      J.Takeya, K.Tsukagoshi, Y.Aoyagi, T.Takenobu, Y.Iwasa
    • Journal Title

      Japanese Journal of Applied Physics (Express Letter) 44

      Pages: L1393-L1396

  • [Journal Article] Control of Carrier Density by a Solution Method in Carbon-Nanotube Devices2005

    • Author(s)
      T.Takenobu, T.Kanbara, N.Akima, T.Takahashi, M.Shiraishi, K.Tsukagoshi, H.Kataura, Y.Aoyagi, Y.Iwasa
    • Journal Title

      Advanced Materials 17

      Pages: 2430-2434

  • [Journal Article] ナノカーボン材料伝導研究のための架橋型ナノ電極作製と応用2005

    • Author(s)
      塚越一仁, 重藤訓志, A.Kasumov, 川村稔, 青柳克信, 小林知洋, 仙波健吾, 兒玉健, 西川浩之, 池本勲, 菊地耕一他
    • Journal Title

      日本顕微鏡学会誌「顕微鏡」 40

      Pages: 96-99

  • [Journal Article] Photoemission Spectroscopic Evidence of Gap Anisotropy in an f-Electron2005

    • Author(s)
      T.Kiss, F.Kanetaka, T.Yokoya, T.Shimojima, K.Kanai, S.Shin, Y.Onuki, T.Tohashi, C.Zhang, C.T.Chen, S.Watanabe
    • Journal Title

      Physical Review Letters 94

      Pages: 57001-57004

  • [Journal Article] Determination of Electron Escape Depth in Ultrathin Silicon Oxide2005

    • Author(s)
      H.Nohira, H.Okamoto, K.Azuma, Y.Nakata, E.Ikenaga, Y.Takata, S.Shin, T.Hattori
    • Journal Title

      Applied Physics Letters 86

      Pages: 81911-81913

  • [Journal Article] Iron Nanoparticles in Amorphous SiO_2 : X-ray Emission and Absorption Spectra2005

    • Author(s)
      E.Z.Kurmaev, D.A.Zatsepin, S.O.Cholakh, B.Schmidt, Y.Harada, T.Tokushima, H.Osawa, S.Shin, T.Takeuchi
    • Journal Title

      Physics of the Solid State 47

      Pages: 754-757

  • [Journal Article] Spin-1/2 Heisenberg antiferromagnets on anisotropic triangular lattice,〔Pd(dmit)_2〕salts -- How do they release frustration?2005

    • Author(s)
      M.Tamura, R.Kato
    • Journal Title

      Polyhedron 24

      Pages: 2817-2820

  • [Journal Article] Structural Study of Low Temperature Charge-Separated Phases of Pd(dmit)_2-Based Molecular Conductors2005

    • Author(s)
      A.Nakao, R.Kato
    • Journal Title

      J.Phys.Soc.Jpn. 74

      Pages: 2754-2763

  • [Journal Article] Direct Formation of Micro-/Nanocrystalline 2,5-Dimethyl-N, N'-dicyanoquinonediimine Complexes of SiO_2/Si Substrates and Multiprobe Measurement of Conduction Properties2005

    • Author(s)
      H.M.Yamamoto, H.Ito, K.Shigeto, K.Tsukagoshi, R.Kato
    • Journal Title

      J.Am.Chem.Soc. 128

      Pages: 700-701

  • [Journal Article] Renormalization of impurity scattering in one-dimensional interacting electron systems in magnetic field2005

    • Author(s)
      T.Hikihara, A.Furusaki, K.A.Matveev
    • Journal Title

      Phys.Rev.B 72・3

      Pages: 035301(10)

  • [Journal Article] Anisotropic pyrochlores and the global phase diagram of the checkerboard antiferromagnet2005

    • Author(s)
      O.A.Starykh, A.Furusaki, L.Balents
    • Journal Title

      Phys.Rev.B 72・9

      Pages: 094416(17)

  • [Journal Article] Theory of successive transitions in vanadium spinels and order of orbitals and spins2005

    • Author(s)
      Y.Motome, H.Tsunetsugu
    • Journal Title

      Prog.Theor.Phys.Suppl. 160

      Pages: 203-232

  • [Journal Article] Modification of the electric conduction at the pentacne/SiO_2 interface by surface termination of SiO_22005

    • Author(s)
      I.Yagi, K.Tsukagoshi, Y.Aoyagi
    • Journal Title

      Applied Physics Letters 86

      Pages: 103501

  • [Journal Article] Hard-X-ray Photoelectron Spectroscopy of Na_xCoO_2・yH_2O2005

    • Author(s)
      A.Chainani, T.Yokoya, Y.Takata, K.Tamasaku, M.Taguchi, T.Shimojima, N.Kanakura, K.Horiba, S.Tsuda, S.Shin
    • Journal Title

      Nuclear Instruments and Methods in Physics Research A 547

      Pages: 163-168

  • [Journal Article] Carbon-substitution Dependent Multiple Superconducting Gap of MgB2 : A Sub-meV Resolution Photoemission Study2005

    • Author(s)
      S.Tsuda, T.Yokoya, T.Kiss, T.Shimojima, S.Shin, T.Togashi, S.Watanabe, C.Zhang, C.T.Chen, S.Lee
    • Journal Title

      Physical Review B 72

      Pages: 064527-064531

  • [Journal Article] Temperature-dependent Eu 3d-4f X-ray Absorption and Resonant Photoemission Study of the Valence Transition in EuNi_2(Si_<0.2>Ge_<0.8>)_22005

    • Author(s)
      K.Yamamoto, K.Horiba, M.Taguchi, M.Matsunami, N.Kamakura, A.Chainani, Y.Takata, K.Miura, M.Shiga, H.Wada
    • Journal Title

      Physical Review B 72

      Pages: 161101(R)-161104(R)

  • [Journal Article] Ion Irradiation Induced Reduction of Fe~<3+> to Fe~<2+> and Fe~0 in Triethoxysilane Films2005

    • Author(s)
      R.G.Wilks, E.Z.Kurmaev, J.C.Pivin, A.Hunt, M.V.Yablonskikh, D.A.Zatsepin, A.Moewes, S.Shin, P.Palade, G.Principi
    • Journal Title

      Journal of Physics : Condensed Matter 17

      Pages: 7023-7028

  • [Journal Article] Evidence for Suppressed Screening on the Surface of High Temperature La_<2-x> Sr_xCuO_4 and Nd_<2-x>Ce_xCuo_4 Superconductors2005

    • Author(s)
      M.Taguchi, A.Chainani, K.Horiba, Y.Takata, M.Yabashi, K.Tamasaku, Y.Nishino, D.Miwa, T.Ishikawa
    • Journal Title

      Physical Review Letters 95

      Pages: 177002-177005

  • [Journal Article] Electronic Structure of Protonic Conductor SrZr_<0.90>M_<0.10>O_3(M=Y~<3+>,SC~<3+>) Probed by Soft-X-ray Spectroscopy2005

    • Author(s)
      T.Higuchi T.Tsukamoto, H.Matsumoto, T.Shimura, K.Yashiro, T.Kawada, J.Mizusaki, S.Shin, T.Hattori
    • Journal Title

      Solid State Ionics 176

      Pages: 2435-2438

  • [Journal Article] Temperature-Dependent Luttinger Surfaces2005

    • Author(s)
      T.Ito, A.Chainani, T.Haruna, K.Kanai, T.Yokoya, S.Shin, R.Kato
    • Journal Title

      Physical Review Letters 95

      Pages: 246402-246405

  • [Journal Article] Electronic Structure in Valence Band of Nd-Substituted Bi_4Ti_3O_<12> Single Crystal Probed by Soft-X-Ray Emission Spectroscopy2005

    • Author(s)
      T.Higuchi, Y.Noguchi, T.Goto, M.Miyayama, S.Shin, K.Kaneda, T.Hattori, T.Tsukamoto
    • Journal Title

      Japanese Journal of Applied Physics 44

      Pages: L1491-L1493

  • [Journal Article] Role of Charge-density-wave Fluctuations on the Spectral Function in a Metallic Charge-density-wave System2005

    • Author(s)
      T.Yokoya, T.Kiss, A.Chainani, S.shin, K.Yamaya
    • Journal Title

      Physical Review B 71

      Pages: 140504-140507

  • [Journal Article] Direct Observation of a Neutral Mn Acceptor in Ga_<1-x>Mn_xAs by Resonant x-ray Emission Spectroscopy2005

    • Author(s)
      Y.Ishiwata, T.Takeuchi, R.Eguchi, M.Watanabe, Y.Harada, K.Kanai, A.Chinani, M.Taguchi, S.Shin
    • Journal Title

      Physical Review B 71

      Pages: 121202(R)-121205(R)

  • [Journal Article] Bulk Screening in Core-level Photoemission from Mott-Hubbard and Charge-transfer Systems2005

    • Author(s)
      M.Taguchi, A.Chainani, N.Kamakura, K.Horiba, Y.Takata, M.Yabashi, K.Tamasaku, Y.Nishino, D.Miwa
    • Journal Title

      Physical Review B 71

      Pages: 155102-155106

  • [Journal Article] Contribution of Electronic Structure to Thermoelectric Power in (Bi,PB)_2(Sr,La)_2CuO_<6+δ>2005

    • Author(s)
      T.Kondo, T.Takeuchi, U.Mizutani, T.YOkoya, S.Tsuda, S.Shin
    • Journal Title

      Physical Review B 72

      Pages: 024533-024541

  • [Journal Article] Role of Ag Doping in Ba_8Si_<46> Compounds2005

    • Author(s)
      N.Kamakura, T.Nakano, Y.Ikemoto, N.Usuda, H.Fukuoka, S.Yamanaka, S.Shin, K.Kobaysahi
    • Journal Title

      Physical Review B 72

      Pages: 014511-014516

  • [Journal Article] Laser-excited Ultrahigh-resolution Photoemission Spectroscopy of Na_xCoO_2/yH_2O : Evidence for Pseudogap Formation2005

    • Author(s)
      T.Shimojima, T.YOkoya, T.Kiss, A.Chainani, S.Shin, T.Togashi, S.Watanabe, C.Zhang, C.T.Chen
    • Journal Title

      Physical Review B 71

      Pages: 020505R-020508R

  • [Journal Article] Intermolecular Interaction by Apical Oxygen in Titanyl Phthalocyanine2005

    • Author(s)
      Y.Harada, T.Tokushima, Y.Takata, N.Kamakura, T.Takeuchi, K.Kobayashi, Y.Shirota, S.Shin
    • Journal Title

      Japanese Journal of Applied Physics 44

      Pages: L1147-L1149

  • [Journal Article] Angle-resolved Photoemission Study of K_<0.3>MoO_3 : Direct Observation of Temperature-dependent Fermi Surface across the Peierls Transition2005

    • Author(s)
      H.Ando, T.Yokoya, K.Ishizaka, S.Tsuda, T.Kiss, S.Shin, T.Eguchi, M.Hohara, H.Takagi
    • Journal Title

      Journal of Phycsics : Condensed Matter 17

      Pages: 4935-4940

  • [Journal Article] Photocarrier-injected Electronic Structure of VO_2/TiO_2 : Nb2005

    • Author(s)
      R.Eguchi, S.Shin, A.Fukushima, T.Kiss, T.Shimojima, Y.Muraoka, Z.Hiroi
    • Journal Title

      Applied Physics Letters 87

      Pages: 211912-211914

  • [Journal Article] Electronic Structure of Proton Conducting SrCeO_3-SrZrO_3 Thin Films2005

    • Author(s)
      T.Higuchi, T.Tsukamoto, N.Sata, S.Yamaguchi, S.Shin, T.Hattori
    • Journal Title

      Solid State Ionics 176

      Pages: 2963-2966

  • [Journal Article] Electronic structure of proton conducting BaCe_<0.90>Y_<0.10>O_<3-δ>2005

    • Author(s)
      T.Higuchi, T.Tsukamoto, H.Matsumoto, T.Shimura, K.Yashiro, T.Kawada, J.Mizusaki, S.Shin, T.Hattori
    • Journal Title

      Solid State Ionics 176

      Pages: 2967-2970

  • [Journal Article] Spectroscopic evidence for the low-temperature charge-separated state of [Pd(dmit)_2] salts2005

    • Author(s)
      M.Tamura, K.Takenaka, H.Takagi, S.Sugai, A.Tajima, R.Kato
    • Journal Title

      Chemical Physics Letters 411/1-3

      Pages: 133-137

  • [Journal Article] Magnetic-field induced transition to the 1/2 magnetization plateau state in the geometrically frustrated magnet CdCr_2O_42005

    • Author(s)
      H.Ueda, H.Aruga Katori, H.Mitamura, T.Goto, H.Takagi
    • Journal Title

      Physical Review Letters 94/4

      Pages: 047202(4)

  • [Journal Article] Collapse of Coherent Quasiparticle States in θ-(BEDT-TTF)_2I_3 Observed by Optical Spectroscopy2005

    • Author(s)
      K.Takenaka, M.Tamura, N.Tajima, H.Takagi, J.Nohara, S.Sugai
    • Journal Title

      Physical Review Letters 95/22

      Pages: 227801(4)

  • [Journal Article] Giant negative thermal expansion in Ge-doped antiperovskite manganese nitrides2005

    • Author(s)
      K.Takenaka, H.Takagi
    • Journal Title

      Applied Physics Letters 87/26

      Pages: 261902(3)

  • [Patent(Industrial Property Rights)] 薄膜トランジスタおよびその製造方法2005

    • Inventor(s)
      塚越一仁, 菅原孝宜, 重藤訓志, 青柳克信
    • Industrial Property Rights Holder
      独立行政法人理化学研究所
    • Industrial Property Number
      特願2005-248571
    • Filing Date
      2005-08-30
  • [Patent(Industrial Property Rights)] 有機薄膜トランジスタおよび有機薄膜トランジスタにおけるゲート絶縁層の表面改質方法2005

    • Inventor(s)
      重藤訓志, 八木巌, 塚越一仁, 青柳克信
    • Industrial Property Rights Holder
      独立行政法人理化学研究所
    • Industrial Property Number
      特願2005-252256
    • Filing Date
      2005-08-31
  • [Patent(Industrial Property Rights)] 微細パターン形性方法

    • Inventor(s)
      沖仲元毅, 塚越一仁, 青柳克信
    • Industrial Property Rights Holder
      独立行政法人理化学研究所
    • Industrial Property Number
      特願2005-249447
    • Filing Date
      出願:20050830

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Published: 2008-05-08   Modified: 2016-04-21  

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