• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to project page

2008 Fiscal Year Final Research Report

Functional Control of the Supra-Molecular Arrays of Artificial Photosynthetic Pigment-Protein Complexes

Research Project

  • PDF
Project/Area Number 17204026
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics I
Research InstitutionOsaka City University

Principal Investigator

HASHIMOTO Hideki  Osaka City University, 大学院・理学研究科, 教授 (50222211)

Co-Investigator(Kenkyū-buntansha) SUGISAKI Mitsuru  大阪市立大学, 大学院・理学研究科, 准教授 (20360042)
FUJII Ritsuko  大阪市立大学, 大学院・理学研究科, 博士研究員 (80351740)
Co-Investigator(Renkei-kenkyūsha) NANGO Mamoru  名古屋工業大学, 大学院・工学研究科, 教授 (90109893)
SUZUKI Masato  大阪市立大学, 大学院・理学研究科, 講師 (70254381)
Project Period (FY) 2005 – 2008
Keywords光合成 / 色素蛋白複合体 / 超高速レーザー分光 / 顕微分光 / 超分子配列 / 人工光合成膜 / 人工光合成 / 光機能統御
Research Abstract

紅色光合成細菌のアンテナ色素蛋白複合体の再構成技術を確立し, 色素構造を改変した人工の光合成色素蛋白複合体の創成に成功した。異種の光合成細菌から調製したアンテナ系色素蛋白複合体を脂質2分子膜に再構築した人工光合成膜試料の作成に成功し, 色素蛋白複合体の配列様式の決定と光機能の評価を達成した。光合成色素および色素蛋白複合体の超高速コヒーレント分光計測を達成し, 光励起後の超高速緩和過程およびエネルギー伝達過程に関する新知見を得た。

  • Research Products

    (32 results)

All 2009 2008 2007 2006 2005 Other

All Journal Article (20 results) (of which Peer Reviewed: 20 results) Presentation (6 results) Book (5 results) Remarks (1 results)

  • [Journal Article] Spectrally-resolved transient grating signals from β-carotene in benzene solution2009

    • Author(s)
      M.Sugisaki, M.Fujiwara, S.V.Nair, H.E.Ruda, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      Phys. Stat. Solidi (c) (in press)

    • Peer Reviewed
  • [Journal Article] Transient grating spectroscopy in photosynthetic purple bacteria Rhodobacter sphaeroides 2.4.12009

    • Author(s)
      M.Sugisaki, M.Fujiwara, R.Fujii, K.Nakagawa, M.Nango, R.J.Cogdelland, and H.Hashimoto
    • Journal Title

      J. Lumin. (in press)

    • Peer Reviewed
  • [Journal Article] Ultrafast optical responses of β-carotene and lycopene probed by sub-20 fs time-resolved coherent spectroscopy2009

    • Author(s)
      M.Fujiwara, M.Sugisaki, A.Gall, B.Robert, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      J. Lumin (in press)

    • Peer Reviewed
  • [Journal Article] Effect of structural modifications on the spectroscopic properties and dynamics of the excited states of peridinin2009

    • Author(s)
      N.Chartterjee, D.M.Niedzwiedzki, K.Aoki, T.Kajikawa. S.Katsumura, H.Hashimoto and H.A.Frank
    • Journal Title

      Arch. Biochem. Biophys 483

      Pages: 146-155

    • Peer Reviewed
  • [Journal Article] Large Third-Order Optical Nonlinearity Realized in Symmetric Nonpolar Carotenoids2008

    • Author(s)
      M.Fujiwara, K.Yamauchi, M.Sugisaki, K.Yanagi, A.Gall, B.Robert, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      Phys. Rev. B78(161101(R))

    • Peer Reviewed
  • [Journal Article] Energy dissipation in the ground-state vibrational manifolds of β-carotene homologues : A sub-20-fs time-resolved transient grating spectroscopic study2008

    • Author(s)
      M.Fujiwara, K.Yamauchi, M.Sugisaki, A.Gall, B.Robert, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      Phys. Rev. B77(205118)

    • Peer Reviewed
  • [Journal Article] Probing the Effect of the Binding Site on the Electrostatic Behavior of a Series of Carotenoids Reconstituted into the Light-Harvesting 1 Complex from Purple Photosynthetic Bacterium Rhodospirillum rubrum Detected by Stark Spectroscopy2008

    • Author(s)
      K.Nakagawa, S.Suzuki, R.Fujii, A.T.Gardiner, R.J.Cogdell, M.Nango, H.Hashimoto
    • Journal Title

      J. Phys. Chem. B112

      Pages: 9467-9475

    • Peer Reviewed
  • [Journal Article] Construction of hybrid photosynthetic units using peripheral and core antennae from two different species of photosynthetic bacteria : Detection of the energy transfer from bacteriochlorophyll a in LH2 to bacteriochlorophyll b in LH12008

    • Author(s)
      R.Fujii, S.Shimonaka, N.Uchida, A.T.Gardiner, R.J.Cogdell, M.Sugisaki, and H.Hashimoto
    • Journal Title

      Photosynth. Res. 95

      Pages: 327-337

    • Peer Reviewed
  • [Journal Article] Linear and nonlinear optical responses in bacteriochlorophyll α2008

    • Author(s)
      M.Sugisaki, R.Fujii, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      Photosynth. Res. 95

      Pages: 309-316

    • Peer Reviewed
  • [Journal Article] Unified explanation for linear and nonlinear optical responses in β-carotene : A sub-20 fs degenerate four-wave mixing spectroscopic study2007

    • Author(s)
      M.Sugisaki, K.Yanagi, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      Phys. Rev. B75

      Pages: 155110/1-11

    • Peer Reviewed
  • [Journal Article] Symmetry Control of Radiative Decay in Linear Polyenes : Low Barriers for Isomerization in the S_1 State of Hexadecaheptaene2007

    • Author(s)
      R.L.Christensen, M.G.I.Galinato, E.F.Chu, R.Fujii, H.Hashimoto, and H.A.Frank
    • Journal Title

      J. Am. Chem. Soc. 129

      Pages: 1769-1775

    • Peer Reviewed
  • [Journal Article] Pump-probe and pump-deplete-probe spectroscopy on carotenoids with N=9-15 conjugated bonds2006

    • Author(s)
      T.Buckup, J.Savolainen, W.Wohlleben, J.L.Herek, H.Hashimoto, R.R.B.Correia, and M.Motzkus
    • Journal Title

      J. Chem. Phys 125

      Pages: 194505/1-194505/7

    • Peer Reviewed
  • [Journal Article] Conjugation length dependence of relaxation kinetics in β-carotene homologs probed by femtosecond Kerr-gate fluorescence spectroscopy2006

    • Author(s)
      D.Kosumi, K.Yanagi, R.Fujii, H.Hashimoto, and M.Yoshizawa
    • Journal Title

      Chem. Phys. Lett. 425

      Pages: 66-70

    • Peer Reviewed
  • [Journal Article] Structures and functions of carotenoids bound to reaction centres from purple photosynthetic bacteria2006

    • Author(s)
      H.Hashimoto, R.Fujii, K.Yanagi, T.Kusumoto, A.T.Gardiner, A.W.Roszal, N.W.Issacs, Z.Pendon, D.Niedzwiedski, H.A.Frank, and R.J.Cogdell
    • Journal Title

      Pure Appl. Chem 78

      Pages: 1505-1518

    • Peer Reviewed
  • [Journal Article] Carotenoid-Bacteriochlorophyll Energy Transfer in LH2 Complexes Studied with 10-fs Time Resolution2006

    • Author(s)
      D.Polli, G.Cerullo, G.Lanzani, S.DeSilvestri, H.Hashimoto, and R.J.Cogdell
    • Journal Title

      Biophys. J. 90

      Pages: 2486-2497

    • Peer Reviewed
  • [Journal Article] Ultrafast Dynamics of All-trans-β-Carotene Explored by Resonant and Nonresonant Photoexcitations2005

    • Author(s)
      D.Kozumi, M.Komukai, H.Hashimoto, and M.Yoshizawa
    • Journal Title

      Phys. Rev. Lett. 95

      Pages: 213601

    • Peer Reviewed
  • [Journal Article] Sub-μ-second time-resolved absorption spectroscopy of a polar carotenoid analogue, 2-(all-trans-retinylidene)-indan-1,3-dione ; formation of the dication by direct triplet-excited sensitization2005

    • Author(s)
      R.Fujii, T.Kusumoto, T.Sashima, R.J.Cogdell, A.T.Gardiner and H.Hashimoto
    • Journal Title

      J. Phys. Chem. A109

      Pages: 11117-11122

    • Peer Reviewed
  • [Journal Article] Excitation energy dependence of excited states dynamics in all-trans-carotenes determined by femtosecond absorption and fluorescence spectroscopy2005

    • Author(s)
      D.Kosumi, K.Yanagi, T.Nishio, H.Hashimoto, and M.Yoshizawa
    • Journal Title

      Chem. Phys. Lett. 408

      Pages: 89-95

    • Peer Reviewed
  • [Journal Article] Local Electrostatic Field Induced by the Carotenoid Bound to the Reaction Center of the Purple Photosynthetic Bacterium Rhodobacter sphaeroides2005

    • Author(s)
      K.Yanagi, M.Shimizu, H.Hashimoto, A.T.Gardiner, A.W.Roszak, and R.J.Cogdell
    • Journal Title

      J. Phys. Chem. B109

      Pages: 992-998

    • Peer Reviewed
  • [Journal Article] Electroabsorption spectroscopy of β-carotene homologs : anomalous enhancement of Δμ2005

    • Author(s)
      K.Yanagi, A.T.Gardiner, R.J.Cogdell, and H.Hashimoto
    • Journal Title

      Phys. Rev. B71

      Pages: 195118

    • Peer Reviewed
  • [Presentation] "Sub-20-fs Coherent Spectroscopy of Carotenoids", ESF Workshop "Novel Methods in Exploring Carotenoid Excited State Dynamics"2008

    • Author(s)
      H.Hashimoto, M.Sugisaki, M.Fujiwara, and R.J.Cogdell
    • Organizer
      Nove Hrady, Czech Republic
    • Place of Presentation
      Invited Lecture
    • Year and Date
      20080921-25
  • [Presentation] Current Understanding of the Photophysics of Carotenoids2008

    • Author(s)
      H.Hashimoto and R.J.Cogdell
    • Organizer
      The 15th International Symposium on Carotenoids, Hotel Moon Beach
    • Place of Presentation
      Okinawa, Japan(Plenary Lecture)
    • Year and Date
      20080622-27
  • [Presentation] Solar to Fuels ; Natural Tactics of Solar Energy Conversion by Photosynthesis2008

    • Author(s)
      H. Hashimoto
    • Organizer
      15th International SPACC Symposium, Osaka, Japan
    • Place of Presentation
      (SPACC賞受賞記念基調講演)
    • Year and Date
      2008-11-20
  • [Presentation] Banz Monastery, German "Very early photophysics of carotenoids probed by sub-20 fs degenerated four-wave mixing(DFWM)spectroscopy"2007

    • Author(s)
      H.Hashimoto, M.Sugisaki, and R.J.Cogdell
    • Organizer
      International Conference onLight-Harvesting Processes
    • Place of Presentation
      Banz Monastery, German(Invited Lecture)
    • Year and Date
      20070321-24
  • [Presentation] Very early photophysics of carotenoids probed by sub-20 fs degenerated four-wave mixing (DFWM) spectroscopy2007

    • Author(s)
      H.Hashimoto, M.Sugisaki, A.T.Gardiner, and R.J.Cogdell
    • Organizer
      7^<th> Gordon Research Conference on Carotenoids
    • Place of Presentation
      Ventura, California, USA(Invited Lecture)
    • Year and Date
      20070107-12
  • [Presentation] Structures and Functions of Carotenoids Bound to Reaction Centres from Purple Photosynthetic Bacteria2005

    • Author(s)
      H.Hashimoto, R.Fujii, K.Yanagi, A.T.Gardiner, A.W.Roszak, N.W.Issacs, H.A.Frank and R.J.Cogdell
    • Organizer
      14^<th> International Symposium on Carotenoids
    • Place of Presentation
      Edinburgh, Scotland, UK.(Invited Lecture)
    • Year and Date
      20050717-22
  • [Book] The Structure of Purple Bacterial Antenna Complexes(Wiley-VCH Verlag GmbH & Co. KGaA)2008

    • Author(s)
      R.J.Cogdell, A.T.Gardiner, M.Gabrielsen,J.Southall, A.W.Roszak, N.W.Isaacs, R.Fujii and H.Hashimoto
    • Total Pages
      325-340
    • Publisher
      Petra Fromme (Ed.), Photosynthetic Protein Complexes A Structural Approach, Weinheim
  • [Book] 第3章テラヘルツ光源, 3.1超短パルステラヘルツ光源, 3.1.3非線形光学結晶からのテラヘルツ発生, 3.1.3.2有機非線形結晶, (2)有機非線形結晶BNA2007

    • Author(s)
      高橋宏典, 橋本秀樹
    • Total Pages
      123-125
    • Publisher
      "テラヘルツ技術要覧", テラヘルツテクノロジーフォーラム編(NGT)
  • [Book] 光技術の最先端を探る(光合成をこの手に!)2007

    • Author(s)
      橋本秀樹
    • Total Pages
      79-109
    • Publisher
      (独)科学技術振興機構編, アドスリー, 丸善
  • [Book] 第5章有機・バイオ-光合成アンテナ色素蛋白複合体・カロテノイド・超高速レーザー分光-2006

    • Author(s)
      橋本秀樹, 藤井律子, 杉崎満
    • Total Pages
      239-261
    • Publisher
      オプトロニクス社, "光物性の基礎と応用", 光物性研究会組織委員会編
  • [Book] 第1章光合成の基礎2光合成の初期過程の最新の描像2006

    • Author(s)
      橋本秀樹, 藤井律子
    • Total Pages
      18-37
    • Publisher
      シーエムシー出版, 光合成微生物の機能と応用", 上原赫監修
  • [Remarks]

    • URL

      http://www.sci.osaka-cu.ac.jp/phys/PBM/index-j.html

URL: 

Published: 2010-06-10   Modified: 2015-09-24  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi