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2007 Fiscal Year Final Research Report Summary

Research on technology for integrating silicon nanocrystals into photonic crystals and its application to optical devices

Research Project

Project/Area Number 17360153
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Electron device/Electronic equipment
Research InstitutionGunma University

Principal Investigator

HANAIZUMI Osamu  Gunma University, Graduate School of Engineering, Professor (80183911)

Co-Investigator(Kenkyū-buntansha) MOTOJIMA Kuniyuki  Gunma University, Graduate School of Engineering, Associate Professor (30272256)
MIURA Kenta  Gunma University, Graduate School of Engineering, Assistant Professor (40396651)
Project Period (FY) 2005 – 2007
Keywordssilicon nanocrystal / photonic crystal / light emission / sputtering / ion implantation / annealing / optical device
Research Abstract

We deposited Si/SiO_2 multilayers having nanometer-order-thick Si and SiO_2 layers using radio-frequency sputtering and obtained ultraviolet (UV) -light emission from the samples after high-temperature annealing. In particular, we found a sharp UV peak around a wavelength of 370 nm after annealing at 1200 ℃. The UV-light emission seems to originate from Si layers, which may be transformed into Si nanocrystals (Si-nc's), and interface layers between Si-nc's and SiO_2 layers. Fused-silica substrates that emit blue light were also fabricated by using Si-ion implantation and high-temperature annealing. Their blue-photoluminescence peaks were located at around a wavelength of 400 nm. We found that the peak intensity can be over four times greater than that of the longer wavelength peak after annealing at 1200 ℃. The blue-light emission seems to originate from both Si-nc's and interface layers between Si-nc's and SiO_2 media produced in fused-silica substrates. We are trying to optimize the … More conditions of Si-ion implantation and annealing to improve the emission intensity and evaluate optical gains of the samples. UV- or blue-light emitting materials can be useful for light sources of higher-density optical-disk systems. If we realize this kind of light source utilizing Si-based materials, we will obtain many benefits, such as matching for LSI's, lower cost, and suitability for environment application.
We fabricated an Si: SiO_2 two-dimensional photonic crystal that emits light at wavelengths from red to infrared by using radio-frequency sputtering, double-interference exposure, and plasma etching. An enhanced photoluminescence spectrum was observed from the sample. We found that the photoluminescence peaks were located at around a wavelength of 800 nm and that the peak intensity can be increased 1.5 times by introducing a periodic structure. Such Si: SiO_2 films with periodic structures can also be useful as substrates of autocloned photonic crystals. We will be able to realize Si-based light-emitting devices utilizing our technologies. Less

  • Research Products

    (46 results)

All 2008 2007 2006 2005 Other

All Journal Article (14 results) (of which Peer Reviewed: 7 results) Presentation (31 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] 高周波スパッタリングによる紫外発光Si/SiO_2多層膜の作製2008

    • Author(s)
      三浦健太, 加藤裕司, 星野ひとみ, 花泉修
    • Journal Title

      照明学会誌 92巻

      Pages: 105-108

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] Fabrication of ultraviolet-light emitting Si/SiO_2 multilayered films using radio-frequency magnetron sputtering and high-temperature annealing2008

    • Author(s)
      K. Miura, Y. Kato, H. Hoshino, and O. Hanaizumi
    • Journal Title

      Thin Solid Films(掲載決定) (未定)

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] Fabrication of ultraviolet-light emission Si/SiO_2 multilayered films by using rf sputtering (in Japanese)2008

    • Author(s)
      K. Miura, Y. Kato, H. Hoshino, and O. Hanaizumi
    • Journal Title

      J. Illum. Engng. Inst. Jpn vol. 92, no. 2

      Pages: 105-108

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] シリコンイオンを注入した石英板からの青色発光帯の観測2007

    • Author(s)
      三浦健太 他
    • Journal Title

      電子情報通信学会論文誌C vol.J90-C

      Pages: 618-620

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] Fabrication of blue-light emission fused-silica substrates by using Si ion implantation and high-temperature annealing2007

    • Author(s)
      K. Miura, et. al.
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B vol.263

      Pages: 532-534

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] フォトニック結晶構造の導入によるSi:SiO_2スパッタ膜の発光効率向上2007

    • Author(s)
      三浦健太, 早川崇志, 花泉修
    • Journal Title

      照明学会誌 91巻

      Pages: 711-714

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] Observation of blue-light emission from nanocrystalline silicon fabricated by ion implantation (in Japanese)2007

    • Author(s)
      K. Miura, T. Tanemura, O. Hanaizumi, S. Yamamoto, K. Takano, M. Sugimoto, and M. Yoshikawa
    • Journal Title

      The IEICE Transactions on Electronics (Japanese Edition) vol. J90-C, no. 8

      Pages: 618-620

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Fabrication of blue-light emission fused-silica substrates by using Si ion implantation and high-temperature annealing2007

    • Author(s)
      K. Miura, T. Tanemura, O. Hanaizumi, S. Yamamoto, K. Takano, M. Sugimoto, and M. Yoshikawa
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B vol. 263, no. 2

      Pages: 532-534

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Improvement of emission efficiency of Si: SiO_2 sputtered films by introducing 2-D photonic crystals (in Japanese)2007

    • Author(s)
      K. Miura, T. Hayakawa, and O. Hanaizumi
    • Journal Title

      J. Illum. Engng. Inst. Jpn vol. 91, no. 11

      Pages: 711-714

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Rugate filters fabricated by a radio frequency magnetron sputtering system by use of an optical in-situ monitoring technique2006

    • Author(s)
      H. Yoda, D. Tanaka, O. Hanaizumi, Y. Kogami, and K. Shiraishi
    • Journal Title

      Applied Optics vol.45

      Pages: 184-190

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] Rugate filters fabricated by a radio frequency magnetron sputtering system by use of an optical in-situ monitoring technique2006

    • Author(s)
      H. Yoda, D. Tanaka, O. Hanaizumi, Y. Kogami, and K. Shiraishi
    • Journal Title

      Applied Optics vol. 45, no. 1

      Pages: 184-190

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Optical gain in as-grown sputtered SiO_2 film contained Si-Ge nanocrystals2005

    • Author(s)
      C. Chaudhari, O. Takei, and O. Hanaizumi
    • Journal Title

      J. Light & Visual Environment vol.29

      Pages: 51-54

    • Description
      「研究成果報告書概要(和文)」より
    • Peer Reviewed
  • [Journal Article] Optical gain in as-grown sputtered SiO_2 film contained Si-Ge nanocrystals2005

    • Author(s)
      C. Chaudhari, O. Takei, and O. Hanaizumi
    • Journal Title

      J. Light & Visual Environment vol. 29, no. 2

      Pages: 51-54

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Fabrication of ultraviolet-light emitting Si/SiO_2 multilayered films using radio-frequency magnetron sputtering and high-temperature annealing

    • Author(s)
      K. Miura, Y. Kato, H. Hoshino, and O. Hanaizumi
    • Journal Title

      Thin Solid Films (in press)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Improvement of emission efficiency of Si:SiO_2 sputtered films by introducing two-dimensional periodic structures2008

    • Author(s)
      K. Miura, T. Hayakawa, and O. Hanaizumi
    • Organizer
      The 6th International Conference on Optics-photonics Design and Fabrication (ODF'08)
    • Place of Presentation
      Taipei, Taiwan
    • Year and Date
      2008-06-10
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Improvement of emission efficiency of Si: SiO_2 sputtered films by introducing two-dimensional periodic structures2008

    • Author(s)
      K. Miura, T. Hayakawa, and O. Hanaizumi
    • Organizer
      The 6th International Conference on Optics-photonics Design and Fabrication (ODF'08)
    • Place of Presentation
      Taipei, Taiwan (to be presented)
    • Year and Date
      2008-06-10
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] タンタル酸化物スパッタ薄膜からの青色発光の観測2008

    • Author(s)
      三浦健太, 宮崎弘規, 伏木厳穣, 花泉修
    • Organizer
      第55回応用物理学関係連合講演会
    • Place of Presentation
      船橋
    • Year and Date
      2008-03-28
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Observation of blue-light emission from tantalum oxide sputtered films2008

    • Author(s)
      K. Miura, H. Miyazaki, G. Fusegi, and O. Hanaizumi
    • Organizer
      The 55rd Spring Meeting of the Japan Society of Applied Physics and Related Societies
    • Place of Presentation
      Funabashi
    • Year and Date
      2008-03-28
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] スパッタリング法により作製したタンタル酸化物薄膜からの青色発光の観測2007

    • Author(s)
      三浦健太, 宮崎弘規, 花泉修
    • Organizer
      電子情報通信学会光エレクトロニクス研究会
    • Place of Presentation
      東京
    • Year and Date
      2007-12-14
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Observation of blue-light emission from tantalum oxide films fabricated by using rf sputtering2007

    • Author(s)
      K. Miura, H. Miyazaki, and O. Hanaizumi
    • Organizer
      OPE
    • Place of Presentation
      Tokyo
    • Year and Date
      2007-12-14
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Siイオンを注入した石英基板からの青色発光2007

    • Author(s)
      三浦健太 他
    • Organizer
      第18回日本MRS学術シンポジウム
    • Place of Presentation
      東京
    • Year and Date
      2007-12-09
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Blue-light emission from silica substrates implanted Si ions2007

    • Author(s)
      K. Miura, T. Tanemura, M. Honmi, O. Hanaizumi, S. Yamamoto, K. Takano, M. Sugimoto, and M. Yoshikawa
    • Organizer
      The 18th MRS-J Academic Symposium
    • Place of Presentation
      Tokyo
    • Year and Date
      2007-12-09
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Development of optical-functional elements composed of silicon-based materials2007

    • Author(s)
      K. Miura, H. Miyazaki, T. Hayakawa, and O. Hanaizumi
    • Organizer
      The 3rd International Symposium on Development of Silicon-based Functional Materials
    • Place of Presentation
      Kiryu
    • Year and Date
      2007-11-30
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Observation of ultraviolet-light emission from Si/SiO_2 multilayer films prepared by using rf magnetron sputtering2007

    • Author(s)
      K. Miura, Y. Kato, H. Hoshino, and O. Hanaizumi
    • Organizer
      SSDM 2007
    • Place of Presentation
      Tsukuba
    • Year and Date
      2007-09-20
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Blue-light emission from Si ion implanted fused-silica substrates generated by high temperature annealing2007

    • Author(s)
      K. Miura, et. al.
    • Organizer
      OECC/IOOC 2007
    • Place of Presentation
      Yokohama
    • Year and Date
      2007-07-13
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Observation of blue light emission from Si ion implanted fused-silica substrates2007

    • Author(s)
      K. Miura, et. al.
    • Organizer
      CLEO/Europe-IQEC 2007
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2007-06-20
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Observation of blue light emission from Si ion implanted fused-silica substrates2007

    • Author(s)
      K. Miura, T. Tanemura, O. Hanaizumi, S. Yamamoto, K. Takano, M. Sugimoto, and M. Yoshikawa
    • Organizer
      OLEO/Europe-IQEC 2007
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2007-06-20
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Siイオンを注入した石英板からの青色発光帯の観測と発光強度のアニール温度依存性2007

    • Author(s)
      三浦健太 他
    • Organizer
      第54回応用物理学関係連合講演会
    • Place of Presentation
      相模原
    • Year and Date
      2007-03-28
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Observation of strong blue light emission from Si nanocrystals produced by ion implantation and annealing2007

    • Author(s)
      K. Miura, T. Tanemura, O. Hanaizumi, S. Yamamoto, K. Takano, M. Sugimoto, and M. Yoshikawa
    • Organizer
      The 54rd Spring Meeting of the Japan Society of Applied Physics and Related Societies
    • Place of Presentation
      Sagamihara
    • Year and Date
      2007-03-28
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Effect of annealing temperature on optical amplification in SiO_2 thin films containing silicon nanocrystals2006

    • Author(s)
      C. Chaudhari, O. Valle, K. Miura, and O. Hanaizumi
    • Organizer
      Photonics India 2006
    • Place of Presentation
      Hyderabad, India
    • Year and Date
      2006-12-13
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Si:SiO_2共スパッタ膜の発光起源の一検証とデバイス応用の検討2006

    • Author(s)
      三浦健太, 松本敏明, 武井修, 加藤裕司, 種村豪, 星野ひとみ, 花泉修
    • Organizer
      電子情報通信学会光エレクトロニクス研究会
    • Place of Presentation
      東京
    • Year and Date
      2006-11-15
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] A study on photoluminescence mechanism of Si:SiO_2 sputtered films and its device application2006

    • Author(s)
      K. Miura, T. Matsumoto, O. Takei, Y. Kato, T. Tanemura, H. Hoshino, and O. Hanaizumi
    • Organizer
      OPE
    • Place of Presentation
      Tokyo
    • Year and Date
      2006-11-15
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Fabrication and evaluation of Si:SiO_2 thin films for light emission devices2006

    • Author(s)
      K. Miura and O. Hanaizumi
    • Organizer
      The 2nd International Symposium on Development of Silicon-based Functional Materials
    • Place of Presentation
      Kiryu
    • Year and Date
      2006-11-09
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Fabrication and evaluation of Si: SiO_2 thin films for light emission devices2006

    • Author(s)
      K. Miura and O. Hanaizumi
    • Organizer
      The 2nd International Symposium on Development of Silicon-based Functional Materials
    • Place of Presentation
      Kiryu
    • Year and Date
      2006-11-09
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] a-Si/SiO_2超格子における紫外域発光の観測2006

    • Author(s)
      加藤裕司, 種村豪, 星野ひとみ, 山外一徳, 三浦健太, 花泉修
    • Organizer
      第53回応用物理学関係連合講演会
    • Place of Presentation
      東京
    • Year and Date
      2006-03-25
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Fabrication of a-Si/SiO_2 superlattices by using rfsputtering and its luminescent properties2006

    • Author(s)
      Y. Kato, T. Tanemura, H. Hoshino, K. Yamahoka, K. Miura, and O. Hanaizumi
    • Organizer
      The 53rd Spring Meeting of the Japan Society of Applied Physics and Related Societies
    • Place of Presentation
      Tokyo
    • Year and Date
      2006-03-25
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] RFスパッタリングによるアモルファスSi/SiO_2超格子構造の作製とその発光特性2006

    • Author(s)
      加藤裕司, 種村豪, 星野ひとみ, 三浦健太, 花泉修
    • Organizer
      電子情報通信学会光エレクトロニクス研究会
    • Place of Presentation
      東京
    • Year and Date
      2006-02-17
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Fabrication of amorphous Si/SiO_2 superlattices by using RF sputtering and their luminescence properties2006

    • Author(s)
      Y. Kato, T. Tanemura, H. Hoshino, K. Miura, and O. Hanaizumi
    • Organizer
      OPE
    • Place of Presentation
      Tokyo
    • Year and Date
      2006-02-17
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Blue-light emission from sputtered Si:SiO_2 films without annealing2005

    • Author(s)
      K. Miura and O. Hanaizumi
    • Organizer
      The first international symposium on development of silicon-based functional materials
    • Place of Presentation
      Kiryu
    • Year and Date
      2005-11-21
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Effect of annealing temperature and time on photoluminescence intensity from SiO_2 thin films containing silicon nanocrystals2005

    • Author(s)
      C. Chaudhari, O. Valle, K. Miura, and O. Hanaizumi
    • Organizer
      The first international symposium on development of silicon-based functional materials
    • Place of Presentation
      Kiryu
    • Year and Date
      2005-11-21
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Blue-light emission from sputtered Si: SiO_2 films without annealing2005

    • Author(s)
      K. Miura and O. Hanaizumi
    • Organizer
      The first international symposium on development of silicon-based functional materials
    • Place of Presentation
      Kiryu
    • Year and Date
      2005-11-21
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] 含ケイ素機能性材料の開拓(3):アニールなしで青色発光するSiナノクリスタル薄膜の作製と評価2005

    • Author(s)
      三浦健太, 花泉修
    • Organizer
      第10回ケイ素化学協会シンポジウム
    • Place of Presentation
      宮島
    • Year and Date
      2005-10-28
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Development of silicon-containing functional materials (3): blue-light emission from nanocrystalline silicon without annealing2005

    • Author(s)
      K. Miura and O. Hanaizumi
    • Organizer
      The 10th Symposium of the Society of Silicon Chemistry
    • Place of Presentation
      Miyajima
    • Year and Date
      2005-10-28
    • Description
      「研究成果報告書概要(欧文)」より
  • [Presentation] Blue-light emission from sputtered Ti:SiO_2 films without annealing2005

    • Author(s)
      O. Hanaizumi, K. Ono, Y. Ogawa, and T. Matsumoto
    • Organizer
      The European Conference on Lasers and Electro-Optics (CLEO/Europe 2005)
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2005-06-17
    • Description
      「研究成果報告書概要(和文)」より
  • [Presentation] Blue-light emission from sputtered Ti: SiO_2 films without annealing2005

    • Author(s)
      O. Hanaizumi, K. Ono, Y. Ogawa, and T. Matsumoto
    • Organizer
      CLEO/Europe 2005
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2005-06-17
    • Description
      「研究成果報告書概要(欧文)」より
  • [Patent(Industrial Property Rights)] 青色発光石英部材の製造方法及び発光素子2007

    • Inventor(s)
      花泉修 他
    • Industrial Property Rights Holder
      群馬大学, 日本原子力研究開発機構
    • Industrial Property Number
      特願2007-80148
    • Filing Date
      2007-03-26
    • Description
      「研究成果報告書概要(和文)」より

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Published: 2010-02-04  

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