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2018 Fiscal Year Annual Research Report

Fabrication if high performance perovskite solar cell with SWCNT

Research Project

Project/Area Number 17F17364
Research InstitutionThe University of Tokyo

Principal Investigator

丸山 茂夫  東京大学, 大学院工学系研究科(工学部), 教授 (90209700)

Co-Investigator(Kenkyū-buntansha) GHAREEB AHMED  東京大学, 工学(系)研究科(研究院), 外国人特別研究員
Project Period (FY) 2017-11-10 – 2020-03-31
KeywordsCarbon nanotubes / Doping / Hole transport / Electrode / Perovskite Photovoltaics / Antioxidation
Outline of Annual Research Achievements

This research is focuses on development of perovskite solar cells employing SWCNT electrodes having the ability to outperform the metal electrode. The lifetime of the device also can be longer in terms of thermal and chemical stability by adding antioxidant doping. This will solve the current problems of perovskite solar cell technology. In addition, we are negotiating the use of new heterostructures of SWCNT-graphene and MoS2@SWCNT for the next stretchable and tandem solar cell devices, respectively. The achievements include;
-Co-authored publication of review article entitled ‘Single‐Walled Carbon Nanotubes in Emerging Solar Cells: Synthesis and Electrode Applications’in Adv. Energy Mater. (IF: 21.875).
-Fabrication of high-performance perovskite solar cell using doped-SWCNT achieved with ~18.7% of power conversion efficiency.
-Fabrication of highly stable perovskite solar cells employed Li@C60 as antioxidant on laminated SWCNT electrode achieved with ~17.5% of power conversion efficiency.

Current Status of Research Progress
Current Status of Research Progress

1: Research has progressed more than it was originally planned.

Reason

-Finalizing the experiments for the stability test of the high performance SWCNT-based perovskite solar cells.
-Understanding the antioxidation and doping effect of Li@C60 on SWCNT electrode for stable solar cell devices.
-Preparing two manuscripts for submission in high-impact journals.
Obstacles: We are recently trying to certify the photoconversion efficiency of our produced solar cells. The are a lot of restrictions according to measurement’s standards. Therefore, we negotiate the collaboration with different teams in Japan for this issue.

Strategy for Future Research Activity

-Robust doping of CNT films with strong Lewis acids.
-Preparation of hybrid Graphene-CNT electrodes with improved properties for stretchable devices.
-Fabrication of perovskite solar cells with doped SWCNT and SWCNT-Graphene hybrid films seeking a stable photoconversion efficiency of in the ambient conditions.
-Presenting new results in international conferences and publish 2-3 research papers.
-Negotiating research on fabrication of stretchable and tandem devices using SWCNT heterostructures.

  • Research Products

    (7 results)

All 2019 2018

All Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results) Presentation (5 results) (of which Int'l Joint Research: 2 results)

  • [Journal Article] Single‐Walled Carbon Nanotubes in Emerging Solar Cells: Synthesis and Electrode Applications2019

    • Author(s)
      I. Jeon, R. Xiang, A. Shawky, Y. Matsuo and S.Maruyama
    • Journal Title

      Adv. Energy Mater.

      Volume: - Pages: -

    • DOI

      10.1002/aenm.201801312.

    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Non-doped and unsorted single-walled carbon nanotubes as carrier-selective, transparent, and conductive electrode for perovskite solar cells2018

    • Author(s)
      Sakaguchi Takahiro、Jeon Il、Chiba Takaaki、Shawky Ahmed、Xiang Rong、Chiashi Shohei、Kauppinen Esko I.、Park Nam-Gyu、Matsuo Yutaka、Maruyama Shigeo
    • Journal Title

      MRS Communications

      Volume: 8 Pages: 1058~1063

    • DOI

      10.1557/mrc.2018.142

    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Enhancing the Stability of Perovskite Solar Cells via Lithium-ion Endohedral Fullerenes on Top of Laminated Carbon Nanotube Electrodes2019

    • Author(s)
      Ahmed Shawky
    • Organizer
      The 56th Fullerenes-Nanotubes-Graphene General Symposium
  • [Presentation] Enhancing the Stability of Perovskite Solar Cells via Lithium-ion Endohedral Fullerenes on Top of Laminated Carbon Nanotube Electrodes2019

    • Author(s)
      Ahmed Shawky
    • Organizer
      CIAiS International Symposium 2019
    • Int'l Joint Research
  • [Presentation] Cultivating SWCNTs by Robust Doping and Coaxial Wrapping: Toward Applicable Devices2018

    • Author(s)
      Ahmed Shawky
    • Organizer
      The 9th A3 Symposium on Emerging Materials: Nanomaterials for Energy and Electronics
    • Int'l Joint Research
  • [Presentation] SWNT films doped with Trifluoromethanesulfonic acid as durable electrode in perovskite solar cells2018

    • Author(s)
      Ahmed Shawky
    • Organizer
      The 55th Fullerenes-Nanotubes-Graphene General Symposium
  • [Presentation] Improving Single walled Carbon Nanotubes via Coaxial Wrapping and Durable Doping: Toward Applicable Devices2018

    • Author(s)
      Ahmed Shawky
    • Organizer
      ATI Nanocarbon Zao meeting

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Published: 2019-12-27  

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