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2018 Fiscal Year Research-status Report

Fine Structure of Bimetallic Solid Solution Nanoparticles Dispersed in Liquid by Double-Head Matrix Sputtering

Research Project

Project/Area Number 17K14072
Research InstitutionHokkaido University

Principal Investigator

グエン タンマイ  北海道大学, 工学研究院, 助教 (00730649)

Project Period (FY) 2017-04-01 – 2020-03-31
Keywordsdouble target head / nanopartiles / alloy / bimetallic / liquid polymer / sputtering onto liquid / plasmonic
Outline of Annual Research Achievements

The growth and oxidation of Cu nanoparticles prepared by sputtering onto liquid polyethylene glycol (PEG, M.W. = 600) have been investigated. Particle growth was observed with an increase in particle size over time. On the other hand, time-dependent oxidation of Cu nanoparticles was monitored and confirmed with fading of the surface plasmon resonance of metallic Cu and changing in color of the nanoparticle dispersions.
Published results of bimetallic alloy nanoparticles in this project were collected and reported in a review for metallic nanoparticles via sputtering onto liquids. The researches in preparation and formation of alloy nanoparticles using two immiscible metals as target for sputtering are in progress for publication.

Current Status of Research Progress
Current Status of Research Progress

2: Research has progressed on the whole more than it was originally planned.

Reason

From the investigation of metals that form intermetallic compounds in the bulk-state, i.e., Cu and Au, and metals form complete solid solution in the bulk state, i.e. Au and Ag, the understanding of experimental set-up and parameters, analysis for resulting bimetal nanoparticles has been obtained. This helps quick access to the further study of on particle formation in immiscible bimetal system.

Strategy for Future Research Activity

Year 2019.
1) Complete the study on particle formation for double-head sputtering of metals that are immiscible in the bulk
2) Study the influence of the liquid composition on particle formation, growth and stability

  • Research Products

    (14 results)

All 2019 2018

All Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (12 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] Monitor the Growth and Oxidation of Cu-nanoparticles in PEG after Sputtering2019

    • Author(s)
      Y.-T. R. Chau, L. Deng, M. T. Nguyen, T. Yonezawa
    • Journal Title

      RSC Adv

      Volume: NA Pages: NA

    • DOI

      10.1557/adv.2019.55 (2019)

    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Sputtering onto a liquid: interesting physical preparation method for multi-metallic nanoparticles2018

    • Author(s)
      M. T. Nguyen, T. Yonezawa
    • Journal Title

      Sci. Technol. Adv. Mater.

      Volume: 19 Pages: 883-889

    • DOI

      DOI: 10.1080/14686996.2018.1542926

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Metal nanoparticles prepared by vacuum sputtering onto liquid: influence of mixing two liquids2019

    • Author(s)
      Mai Thanh Nguyen and Tetsu Yonezawa
    • Organizer
      日本化学会 第99春季年会 2019.3.16~19,甲南大学 岡本キャンパス
  • [Presentation] Study the Growth of Pt/Cu Alloy Nanoparticles Prepared by Sputter Deposition onto a Liquid Polymer2019

    • Author(s)
      L. Deng, M.T. Nguyen, T. Yonezawa
    • Organizer
      日本化学会 第99春季年会 2019.3.16~19,甲南大学 岡本キャンパス
  • [Presentation] Growth and oxidation of Cu-nanoparticles Sputtered in PEG2019

    • Author(s)
      Y. R. Chau, L. Deng, M. T. Nguyen, T. Yonezawa
    • Organizer
      平成30年度 日本鉄鋼協会・日本金属学会両支部合同冬季講演大会 2019.1.10-11,室蘭工業大学(室蘭市))
  • [Presentation] Pt/Cu Alloy Nanoparticles via Sputter Deposition onto Liquid Polymer2019

    • Author(s)
      L. Deng, M. T. Nguyen, T. Yonezawa
    • Organizer
      平成30年度 日本鉄鋼協会・日本金属学会両支部合同冬季講演大会 2019.1.10-11,室蘭工業大学(室蘭市))
  • [Presentation] Sputter Deposition onto Liquid to Prepare Pt and Pt Alloy Nanoparticles2018

    • Author(s)
      L. Deng, M. T. Nguyen, T. Tokunaga, S. Matsumura, T. Yonezawa
    • Organizer
      Material Research Society Fall Meeting, 2018, Boston, MA, USA (2018.11.25-30)
    • Int'l Joint Research
  • [Presentation] Magnetron sputtering onto liquid of Cu2018

    • Author(s)
      M. T. Nguyen, M. Porta, S. Mei, T. Yonezawa
    • Organizer
      第69回コロイドおよび界面化学討論会 (2018.9.18-20, 筑波大学つくばキャンパス)
  • [Presentation] Alloy Nanoparticles vis Sputtering onto Liquid and Their Structure Control2018

    • Author(s)
      M. T. Nguyen, T. Yonezawa
    • Organizer
      第69回コロイドおよび界面化学討論会 (2018.9.18-20, 筑波大学つくばキャンパス)
  • [Presentation] Compositional Dependent AuPt Alloy Nanoparticles via Sputtering onto PEG2018

    • Author(s)
      L. Deng, M. T. Nguyen, T. Tokunaga, S. Matsumura, T. Yonezawa
    • Organizer
      第69回コロイドおよび界面化学討論会 (2018.9.18-20, 筑波大学つくばキャンパス)
  • [Presentation] Sputtering onto PEG for Sub 2nm Single Crystal Pt Nanoparticles2018

    • Author(s)
      L. Deng, M. T. Nguyen, T. Tokunaga, T. Yonezawa
    • Organizer
      第69回コロイドおよび界面化学討論会 (2018.9.18-20, 筑波大学つくばキャンパス)
  • [Presentation] Synthesis of alloy nanoparticles via sputtering onto a liquid polymer2018

    • Author(s)
      M. T. Nguyen, T. Yonezawa, and L. Deng
    • Organizer
      256th ACS National Meeting in Boston, MA, August 19-23, 2018
    • Int'l Joint Research
  • [Presentation] Double-Target Sputtering for Au Containing Alloy Nanoparticles2018

    • Author(s)
      M. T. Nguyen , T. Yonezawa
    • Organizer
      Gold 2018, Sorbonne Universite, Paris, France (2018.7.15-18)
    • Int'l Joint Research
  • [Presentation] Au/Pt alloy nanoparticles prepared by sputtering onto liquid2018

    • Author(s)
      L. Deng, M. T. Nguyen, 徳永智春, 米澤 徹
    • Organizer
      平成30年度日本金属学会・日本鉄鋼協会両北海道支部合同サマーセッション (2018.7.13,札幌市 教育文化会館)

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Published: 2019-12-27  

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