2009 Fiscal Year Final Research Report
Surface-Mediated Catalyst Design for Selective Oxidation Catalysis
Project/Area Number |
18065003
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Research Category |
Grant-in-Aid for Scientific Research on Priority Areas
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Allocation Type | Single-year Grants |
Review Section |
Science and Engineering
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Research Institution | Institute for Molecular Science (2008-2009) The University of Tokyo (2006-2007) |
Principal Investigator |
TADA Mizuki Institute for Molecular Science, 物質分子科学研究領域, 准教授 (70396810)
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Co-Investigator(Kenkyū-buntansha) |
SASAKI Takehiko 東京大学, 大学院・新領域創成科学研究科, 准教授 (90242099)
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Project Period (FY) |
2006 – 2009
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Keywords | 固定化金属錯体 / 固体触媒 / 触媒構造解析 / 選択酸化 / 触媒反応機構 |
Research Abstract |
Novel unique metal catalysts were designed and prepared on oxide surfaces by metal-complex attaching and selective structural transformation at the surfaces and we have found concerto catalysis for selective oxidation on these surface-mediated metal-complex catalysts. Dynamic structural changes of catalytically active species in the concerto catalysis were investigated by in-situ time-resolved XAFS technique and the reaction mechanism and structural kinetics of the concerto catalysis were demonstrated.
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[Journal Article] In-situ Time-Resolved Dynamic Surface Events on the Pt/C Cathode in a Fuel Cell under Operando Conditions2007
Author(s)
M. Tada, S. Murata, T. Asaoka, K. Hiroshima, K. Okumura, H. Tanida, T. Uruga, H. Nakanishi, S. Matsumoto, Y. Inada, M. Nomura, Y. Iwasawa
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Journal Title
Angew. Chem. Int. Ed 46
Pages: 4310-4315
Peer Reviewed
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