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2018 Fiscal Year Annual Research Report

太陽光を利用した水中細菌の新規光触媒処理システムの開発

Research Project

Project/Area Number 18J20620
Research InstitutionUniversity of Tsukuba

Principal Investigator

LIU NA  筑波大学, 生命環境科学研究科, 特別研究員(DC1)

Project Period (FY) 2018-04-25 – 2021-03-31
KeywordsPhotocatalyst / Solar-light-driven / Water disinfection / Gram-positive / Gram-negative
Outline of Annual Research Achievements

During the first fiscal year of my research, the photocatalytic inactivation ability of a novel solar-light-driven P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst on two different types of microorganisms was systematically studied both in single and mixed bacteria system. According to previous studies, the novel solar-light-driven P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst, firstly synthesized by our lab, has shown remarkable disinfection ability on Gram-negative E. coli. Considering in real water environment, Gram-negative and Gram-positive bacteria are usually coexistent, as such, it is of practical significance to investigate the photocatalytic inactivation efficiency on Gram-negative and Gram-positive bacteria, respectively, in single and mixed bacteria system.
In order to clarify the novel photocatalyst disinfection ability on different types of microorganisms, the study was carried out through the following three key points. (1) Comparison of the photocatalytic inactivation between different types microorganisms: Gram-positive and Gram-negative. (2) Evaluation of the photocatalytic disinfection performance both in single and mixed bacteria system.(3) Investigation of the bacteria damage process during the photocatalytic disinfection process.
The results showed the novel P/Ag/Ag2O/Ag3PO4/TiO2 composite could effectively inactivate both Gram-negative and Gram-positive bacterium either in single or mixed bacteria system.The present study results will help optimize engineering parameters in future application of this novel photocatalyst in large-scale wastewater disinfection system.

Current Status of Research Progress
Current Status of Research Progress

2: Research has progressed on the whole more than it was originally planned.

Reason

In FY 2018, with the aim of "clarifying the photocatalytic inactivation ability of the novel solar-light-driven P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst on two different types of microorganisms",the research was conducted from three categories:(1) Comparison of the photocatalytic inactivation between different types microorganisms: Gram-positive and Gram-negative. (2) Evaluation of the photocatalytic disinfection performance both in single and mixed bacteria system. (3) Investigation of the bacteria damage process during the photocatalytic disinfection process.The present study results will help optimize engineering parameters in future application of this novel photocatalyst in large-scale wastewater disinfection system.

Strategy for Future Research Activity

Based on the result obtained in the previous fiscal year, the novel P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst with remarkable disinfection ability for both Gram-negative and Gram-positive bacteria, can be very suitable for practical bacterial inactivation. Therefore, in this fiscal year, following the research plan, to further scale up the present reactor system and make full use of the solar light energy, a continuous-cycle photocatalytic disinfection system based on the Inclined Plate Collectors (IPC) photoreactor will be developed. Moreover, the optimum conditions of this solar photocatalytic disinfection system will be established, including reaction volume, flow rate and initial concentration of bacteria by using different types of bacteria. Compared to other photoreactor designs, the significantly simplified design and low material cost of this inclined plate photoreactor makes it particularly suitable for use in economically and logistically challenged areas.
Based on the above experiments, the results will be summarized and presented on conferences. Also, the research paper will be summarized and submitted to the international journal.

  • Research Products

    (13 results)

All 2019 2018

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (11 results) (of which Int'l Joint Research: 4 results)

  • [Journal Article] Superior disinfection effect of Escherichia coli by hydrothermal synthesized TiO2-based composite photocatalyst under LED irradiation: Influence of environmental factors and disinfection mechanism2019

    • Author(s)
      Liu Na、Zhu Qi、Zhang Nan、Zhang Cheng、Kawazoe Naoki、Chen Guoping、Negishi Nobuaki、Yang Yingnan
    • Journal Title

      Environmental Pollution

      Volume: 247 Pages: 847~856

    • DOI

      10.1016/j.envpol.2019.01.082

    • Peer Reviewed
  • [Journal Article] Development of Solar-light-driven Photocatalyst for energy and environmental application2019

    • Author(s)
      Liu, N, Zhu Q., Zhang, N., Wang, J., Yang, Y. N.
    • Journal Title

      Materials Science and Engineering

      Volume: 印刷中 Pages: 印刷中

    • Peer Reviewed
  • [Presentation] Insights into photocatalytic inactivation mechanism of a novel hydrothermal synthesized P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst with superior bactericidal activity2019

    • Author(s)
      Liu, N., Ma, Q., Negishi, N., Yang, Y. N.
    • Organizer
      第7回日本生物工学会東支部コロキウム
  • [Presentation] Continuous Bio-hydrogen Production by Iron-modified Zeolite Addition in Hybrid Fixed-bed Reactor2019

    • Author(s)
      Zhao, C. Y., Zhang, N., Zheng, H. Y., Liu, N., Sharma, A., Yang, Y. N.
    • Organizer
      The 53rd Annual Conference of JSWE
  • [Presentation] Enhanced Photocatalytic Activity of Graphene Oxide Modified Visible-light-driven Photocatalysts for Organic Pollutant Degradation2019

    • Author(s)
      Gu, W., Ma, Q. S., Liu, N., Zhang, N., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
  • [Presentation] Development of Linear Fresnel Photoreactor (LFP) for Water Purification Under Solar Light Irradiation2019

    • Author(s)
      Zhang, C., Liu, N., Ma, Q. S., Zhang, N., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
  • [Presentation] Effective Treatment of Seawater Pollutants Under Simulated Solar Light Using Modified-TiO2 Photocatalyst2019

    • Author(s)
      Sharma, A., Liu, N., Zhang, N., Ma, Q. S., Zhao, C. Y., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
  • [Presentation] Fabrication of High Performance and Stability Bi2WO6 Based Photocatalytic Thin Film Doping with Polyethylene Glycol for Wastewater Treatment2019

    • Author(s)
      Ma, Q. S., Liu, N., Sharma, A., Zhang, N., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
  • [Presentation] Photocatalytic Disinfection Performance in Gram-Negative/Gram-Positive Bacteria Mixed System by A Novel TiO2-Based Composite2019

    • Author(s)
      Liu, N., Ma, Q. S., Zhang, C., Sharma, A., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
  • [Presentation] Comparison of The Photocatalytic Inactivation Between Two Model Microorganisms: Gram-Positive Enterococcus Sp. and Gram-Negative E. coli2018

    • Author(s)
      Liu, N., Zhu, Q., Zhang, N., Ma, Q. S., Negishi, N., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Int'l Joint Research
  • [Presentation] Development of Polyethylene Glycol Modified Bi2WO6-based Composite Photocatalytic Thin Film with High Photocatalytic Activity for Wastewater Treatment under Visible Light2018

    • Author(s)
      Ma, Q. S., Liu, N., Zhang, N., Sharma, A., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Int'l Joint Research
  • [Presentation] Effect of Salinity on Degradation of Organic Pollutants in Seawater Using TiO2-Based Composite Photocatalyst2018

    • Author(s)
      Sharma, A., Zheng, H. Y., Liu, N., Zhao, C. Y., Zhang, N., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Int'l Joint Research
  • [Presentation] Investigating the Effects of Bioreactor Design and Continuous Nutrition Release from Bed Material During the Hydrogen Fermentation2018

    • Author(s)
      Zhao, C. Y., Zhang, N., Zheng, H. Y., Liu, N., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Int'l Joint Research

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Published: 2019-12-27  

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