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2011 Fiscal Year Final Research Report

Ultrafast hydrogen migration

Research Project

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Project/Area Number 19002006
Research Category

Grant-in-Aid for Specially Promoted Research

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Chemistry
Research InstitutionThe University of Tokyo

Principal Investigator

YAMANOUCHI Kaoru  東京大学, 大学院・理学系研究科, 教授 (40182597)

Co-Investigator(Renkei-kenkyūsha) KATO Tsuyoshi  東京大学, 大学院・理学系研究科, 准教授 (10321986)
KANYA Reika  東京大学, 大学院・理学系研究科, 助教 (10401168)
OKINO Tomoya  東京大学, 大学院・理学系研究科, 助教 (40431895)
Project Period (FY) 2007 – 2011
Keywords水素移動 / 強光子場 / 超高速化学 / 化学反応動力学
Research Abstract

Dynamics of ultrafast hydrogen migration in intense laser fields was elucidated by a coincidence momentum imaging method with an advanced ultrashort pulsed laser system. A new time-resolved electron diffraction method for tracing ultrafast hydrogen motions was proposed, and electron scattering signals induced by ultrashort pulsed laser fields were observed for the first time, showing the feasibility of the proposed method. Furthermore, quantum dynamics theory for the correlated dynamics of a system consisting of electrons and protons was newly constructed for describing the ultrafast hydrogen migration.

  • Research Products

    (20 results)

All 2012 2011 2010 2009 2008 2007 Other

All Journal Article (9 results) (of which Peer Reviewed: 9 results) Presentation (8 results) Book (1 results) Remarks (2 results)

  • [Journal Article] Hydrogen scrambling in ethane induced by intense laser fields : Statistical analysis of coincidence events2012

    • Author(s)
      R. Kanya, T. Kudou, N. Schirmel, S. Miura, K.-M. Weitzel, K. Hoshina, K. Yamanouchi
    • Journal Title

      J. Chem. Phys.

      Volume: 136 Pages: 204309

    • DOI

      DOI:10.1063/1.4720503

    • Peer Reviewed
  • [Journal Article] Protonic structure of CH_3OH described by electroprotonic wave functions2012

    • Author(s)
      T. Kato, K. Yamanouchi
    • Journal Title

      Phys. Rev. A

      Volume: 85 Pages: 034504

    • DOI

      DOI:10.1103/PhysRevA.85.034504

    • Peer Reviewed
  • [Journal Article] Apparatus for laser-assisted electron scattering in femtosecond intense laser fields2011

    • Author(s)
      R. Kanya, Y. Morimoto, K. Yamanouchi
    • Journal Title

      Rev. Sci. Instrum.

      Volume: 82 Pages: 123105

    • DOI

      DOI:10.1063/1.3665926

    • Peer Reviewed
  • [Journal Article] Ultrafast delocalization of hydrogen atoms in allene in intense laser fields2011

    • Author(s)
      H. Xu, T. Okino, K. Yamanouchi
    • Journal Title

      Appl. Phys. A

      Volume: 104 Pages: 941-945

    • DOI

      DOI:10.1007/s00339-011-6444-7

    • Peer Reviewed
  • [Journal Article] Observation of laser-assisted electron-atom scattering in femtosecond intense laser fields2010

    • Author(s)
      R. Kanya, Y. Morimoto, K. Yamanouchi
    • Journal Title

      Phys. Rev. Lett.

      Volume: 105 Pages: 132202

    • DOI

      DOI:10.1103/PhysRevLett.105.123202

    • Peer Reviewed
  • [Journal Article] Two-proton migration in 1, 3-butadiene in intense laser fields2010

    • Author(s)
      H. Xu, T. Okino, K. Nakai, K. Yamanouchi, S. Roither, X. Xie, D. Kartashov, L. Zhang, A. Baltuska, M. Kitzler
    • Journal Title

      Phys. Chem. Chem. Phys.

      Volume: 12 Pages: 12939

    • DOI

      DOI:10.1039/C0CP00628A

    • Peer Reviewed
  • [Journal Article] Two stages of ultrafast hydrogen migration in methanol driven by intense laser fields2010

    • Author(s)
      H. Xu, C. Marceau, K. Nakai, T. Okino, S. L. Chin, K. Yamanouchi
    • Journal Title

      J. Chem. Phys.

      Volume: 133 Pages: 071103

    • DOI

      DOI:10.1063/1.3473931

    • Peer Reviewed
  • [Journal Article] Time-dependent multiconfiguration theory for describing molecular dynamics in diatomic-like molecules2009

    • Author(s)
      T. Kato, K. Yamanouchi
    • Journal Title

      J. Chem. Phys.

      Volume: 131 Pages: 164118

    • DOI

      DOI:10.1063/1.3249967

    • Peer Reviewed
  • [Journal Article] Ultrafast hydrogen scrambling in methylacetylene and methyl-d3-acetylene ions induced by intense laser fields

    • Author(s)
      T. Okino, A. Watanabe, H. Xu, K. Yamanouchi
    • Journal Title

      Phys. Chem. Chem. Phys

      Volume: (in press)

    • Peer Reviewed
  • [Presentation] Ultrafast probing of molecules in intense laser fields by coincidence momentum imaging and gas electron diffraction2011

    • Author(s)
      K. Yamanouchi
    • Organizer
      XXVII International Conference on Photonic, Electronic and Atomic Collisions, Queen's University Belfast
    • Place of Presentation
      Northern Ireland, UK
    • Year and Date
      2011-07-27
  • [Presentation] Ultrafast hydrogen migration in intense laser fields studied by coincidence momentum imaging and gas electron diffraction2011

    • Author(s)
      K. Yamanouchi
    • Organizer
      The Madrid Conference on Femtochemistry(FEMTO10)
    • Place of Presentation
      Madrid, Spain
    • Year and Date
      2011-07-14
  • [Presentation] New approaches to investigating ultrafast hydrogen migration in hydrocarbon molecules in intense laser fields : Momentum imaging and gas electron diffraction2010

    • Author(s)
      K. Yamanouchi
    • Organizer
      International Symposium on Ultrafast Intense Laser Science 9(ISUILS9)
    • Place of Presentation
      Maui, Hawaii, U. S. A.
    • Year and Date
      20101209-13
  • [Presentation] Ultrafast Delocalization of Hydrogen Atoms in Hydrocarbon Molecules in Intense Laser Fields2010

    • Author(s)
      K. Yamanouchi
    • Organizer
      The 7th International Conference on Photo-Excited Processes and Applications(ICPEPA-7)
    • Place of Presentation
      Lundbeck Auditorium, Biocenter, Copenhagen, Denmark
    • Year and Date
      2010-08-17
  • [Presentation] Application of attosecond pulses and high-order harmonics to physics and chemistry2009

    • Author(s)
      K. Yamanouchi
    • Organizer
      The 2nd International Conference on Ultra-Intense Laser Interaction Science
    • Place of Presentation
      Frascati, Italy
    • Year and Date
      2009-05-28
  • [Presentation] Ultrafast HydrogenMigration in Molecules in Intense Laser Fields : New Frontiers in Attosecond Chemistry2008

    • Author(s)
      K. Yamanouchi
    • Organizer
      17th International Laser Physics Workshop(LPHYS' 08)
    • Place of Presentation
      Trondheim, Norway
    • Year and Date
      2008-07-04
  • [Presentation] Ultrafast Hydrogen Migration in Hydrocarbon Molecules in Intense Laser Fields2007

    • Author(s)
      K. Yamanouchi
    • Organizer
      The 7th Pacific Rim Conference on Lasers and Electro-Optics(CLEO-PR 2007)
    • Place of Presentation
      Seoul, Korea
    • Year and Date
      20070826-31
  • [Presentation] Ultrafast Hydrogen Migration in Hydrocarbon Molecules in Intense Laser Fields2007

    • Author(s)
      K. Yamanouchi
    • Organizer
      International Conference on Photochemistry 2007
    • Place of Presentation
      Cologne, Germany
    • Year and Date
      20070729-0803
  • [Book] 強光子場科学の新展開、『強光子場科学の最前線2』2009

    • Author(s)
      山内薫
    • Total Pages
      1-10
    • Publisher
      強光子場科学研究懇談会
  • [Remarks] 電子の散乱状況フェムト秒の観測成功-東大連続写真撮影向け技術-(日刊工業新聞2010年9月17日付22面)

  • [Remarks]

    • URL

      http://www.yamanouchi-lab.org/index.html

URL: 

Published: 2013-07-31  

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