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2023 Fiscal Year Final Research Report

Attosecond Science in the sub-keV region

Research Project

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Project/Area Number 19H05628
Research Category

Grant-in-Aid for Scientific Research (S)

Allocation TypeSingle-year Grants
Review Section Broad Section D
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

Midorikawa Katsumi  国立研究開発法人理化学研究所, 光量子工学研究センター, センター長 (40166070)

Project Period (FY) 2019-06-26 – 2024-03-31
Keywords量子エレクトロニクス / アト秒科学 / 超高速光科学 / レーザー工学 / 非線形光学
Outline of Final Research Achievements

By compressing the high-energy mid-infrared pulse to two cycles using our uniquely developed DC-OPA and combining this with the loose focusing method, we generate high-energy attosecond high-order harmonics in the water window region. Furthermore, an optical synthesizer consisting of multi-cycle three-wavelength laser pulses realizes an almost single-cycle harmonic driving field and generates a GW class isolated attosecond pulse with high efficiency. We also succeeded in measuring the waveform by using an attosecond streaking method. In addition, we developed a new method for generating circularly polarized light pulses and an attosecond transient absorption simulator for application to the investigation of attosecond electron dynamics in atoms and molecules.

Free Research Field

量子エレクトロニクス

Academic Significance and Societal Importance of the Research Achievements

物質中の電子の動きを捉えることができるアト秒パルスレーザーは、物理学、化学、生物・医科学等の基礎科学分野のみならず、超高速電子デバイス等ならびに高性能触媒や人工光合成等の化学・材料等の産業分野においても必須のツールとなるとものと期待されている。本課題の成果は、このアト秒パルスの利用波長域を水の窓領域までに拡張し生命科学や材料・物性科学の進展に大きく貢献するものである。また、その強度を100倍以上に増強しアト秒領域の非線形光学という新領域への道筋を示した。

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Published: 2025-01-30  

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