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2010 Fiscal Year Final Research Report

Investigation of the interactions between femto-second pulse laser and ultrapure water

Research Project

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Project/Area Number 20246037
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Fluid engineering
Research InstitutionShizuoka University

Principal Investigator

SAITO Takayuki  Shizuoka University, 創造科学技術大学院, 教授 (10324328)

Co-Investigator(Kenkyū-buntansha) SANADA Toshiyuki  静岡大学, 工学部, 准教授 (50403978)
OKAMOTO Masayoshi  静岡大学, 工学部, 准教授 (90293604)
Co-Investigator(Renkei-kenkyūsha) AOSHIMA Shin-ichiro  浜松ホトニクス株式会社, 浜松ホトニクス中央研究所, 室長 (70393931)
Project Period (FY) 2008 – 2010
Keywordsフェムト秒レーザー / 気泡生成 / 気泡運動 / 相互作用 / 混相流
Research Abstract

Femtosecond-pulse lasers (fs pulses) cause very interesting phenomena due to their extremely high energy density. The effects on substances are not thermal, but multi-photon absorption. When this multi-photon absorption of fs pulses operates on water, extraordinary phenomena different from laser-induced cavitation by a usual laser such as a nano-pulse laser are induced. In the present investigation, fs pulses of 50-150fs in duration, 1kHz in repetition rate and 0.2-1.4μJ in pulse energy were focused at ultrapure water in a glass cell through several types of lens. The fs pulses split from original beams through a beam splitter were used as probe light. The femtosecond-order time-resolved optical measurement was realized by adjusting a light path length of the probe light (fs pulses). By effectively using this measurement technique, we elucidated the changes of refraction index of the water, the bubble nucleation and growth processes at an interval of femtoseconds, and the bubble properties at an interval of milliseconds. Based on these results, we have elucidated a relationship between those and fs-pulse peak intensity. In addition, we investigated the nucleation and growth processes in femtosecond- to picosecond-order. Finally, we have discovered the water molecules excited by the multi-photon absorption were decomposed into H_2 and O_2 molecules. We found out a new method of hydrogen production.
Furthermore, based on the above results, the interactions between a solid transparent material (quartz) and the fs pulses were investigated. An optical fiber was microfabricated by the fs pulses, and a new type optical fiber probe was created. The excellent performances of the probe were demonstrated in micro droplet/bubble measurement (the paper received the Outstanding Paper Award from Institute of Physics, 2010).

  • Research Products

    (12 results)

All 2011 2010 2009 2008 Other

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (5 results) Remarks (1 results)

  • [Journal Article] Deep Ocean CO2 Sequestration via GLAD (Gas-Lift Advanced Dissolution) System2011

    • Author(s)
      T.Saito, T.Kajishima, K.Tsuchiya
    • Journal Title

      Journal of Environment and Engineering Vol.6, No.2

      Pages: 412-415

    • Peer Reviewed
  • [Journal Article] Dynamical Mass Transfer Process of a CO2 Bubble Measured by using LIF/HPTS Visualization and Photoelectric Probing2010

    • Author(s)
      K.Hanyu, T.Saito
    • Journal Title

      Canadian Journal of Chemical Engineering Vol.88

      Pages: 551-560

    • Peer Reviewed
  • [Journal Article] Flow structure of steam-water mixed spray2010

    • Author(s)
      T.Sanada, T.Saito, et al.
    • Journal Title

      Nuclear Engineering and Design Vol.240

      Pages: 3974-3983

    • Peer Reviewed
  • [Journal Article] A Study of Surfactant Effects on the Liquid-Phase Motion around a Zigzagging-ascent Bubble Using a Recursive Cross Correlation PIV2010

    • Author(s)
      T.Saito, et al.
    • Journal Title

      Chemical Engineering Journal, Elsevier Vol.158

      Pages: 39-50

    • Peer Reviewed
  • [Journal Article] Quantitative characterizations of long-period fluctuations in a large-diameter bubble column based on point-wise void fraction measurements2010

    • Author(s)
      M.Higuchi, T.Saito
    • Journal Title

      Chemical Engineering Journal, Elsevier Vol.160

      Pages: 284-292

    • Peer Reviewed
  • [Journal Article] Measurement of tiny-droplets using a newly developed optical fiber probe microfabricated by femtosecond pulse laser2009

    • Author(s)
      T.Saito, S.Aoshima, et al.
    • Journal Title

      Measurement Science and Technology, Institute of Physics Vol.20

      Pages: 114002

    • Peer Reviewed
  • [Presentation] Newly developed measurement technique for bubbles by an Optical fiber probe improved by using the Pre-signal method2010

    • Author(s)
      Y.Mizushima, T.Saito
    • Organizer
      APS (American Physical Society) 63rd Annual Meeting
    • Place of Presentation
      Long beach Convention Center, USA.
    • Year and Date
      2010-11-23
  • [Presentation] 混相流計測のための多機能光ファイバープローブ2010

    • Author(s)
      齋藤隆之
    • Organizer
      日本機械学会流体工学部門講演会
    • Place of Presentation
      工学院大学(東京都)(招待講演)
    • Year and Date
      2010-10-30
  • [Presentation] フェムト秒レーザーを用いた気液二相流の時間分解計測2010

    • Author(s)
      齋藤隆之
    • Organizer
      可視化情報シンポジウム(日本可視化情報学会主催)
    • Place of Presentation
      山形大学(山形県)(招待講演)
    • Year and Date
      2010-07-21
  • [Presentation] Nucleation of mysterious bubbles by irradiation of femtosecond pulses2009

    • Author(s)
      T.Saito, S.Aoshima, et al.
    • Organizer
      APS 62nd Annual Meeting
    • Place of Presentation
      Marriott Hotel San Antonio, USA.
    • Year and Date
      2009-11-22
  • [Presentation] A study on the interactions between femtosecond-pulse laser and water from a viewpoint of multiphase flows2008

    • Author(s)
      T.Saito, S.Aoshima
    • Organizer
      APS 61st Annual Meeting
    • Place of Presentation
      Minneapolis Convention Center, USA.
    • Year and Date
      2008-11-23
  • [Remarks] ホームページ

    • URL

      http://flow.eng.shizuoka.ac.jp/

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Published: 2012-01-26   Modified: 2016-04-21  

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