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2021 Fiscal Year Annual Research Report

Application of biochar supported Ni/Fe nanocomposites on feedstock recycling of waste plastics

Research Project

Project/Area Number 20F20089
Research InstitutionTohoku University

Principal Investigator

熊谷 将吾  東北大学, 環境科学研究科, 助教 (40757598)

Co-Investigator(Kenkyū-buntansha) MA CHUAN  東北大学, 環境科学研究科, 外国人特別研究員
Project Period (FY) 2020-09-25 – 2023-03-31
KeywordsPlastic / Waste tire / Pyrolysis / Catalyst / Debromination
Outline of Annual Research Achievements

We have prepared the different catalysts for catalytic pyrolysis of plastics. The experiments have been done by the tandem micro-reactor GC/MS. The co-pyrolysis of PCB and waste tire was conducted. We find that the co-pyrolysis of PCB and waste tire can be beneficial for the production of phenol and largely reduce the content of brominated compounds. The related work has been published in the journal of Green Chemistry and Journal of Hazardous Materials.
We attended the International Symposium on Feedstock Recycling of Polymeric Materials, and gave a presentation on the topic of “Co-pyrolysis of the non-metallic fraction of printed circuit boards and waste tire”.

Current Status of Research Progress
Current Status of Research Progress

2: Research has progressed on the whole more than it was originally planned.

Reason

The ZSM-5 and hierarchical ZSM-5 prepared by acid/alkali treatment and Fe loading biochar was prepared. The catalytic co-pyrolysis of PCB and waste tire has is being conducted.

Strategy for Future Research Activity

We are conducting the fast pyrolysis and the catalytic pyrolysis of PCB and waste tire. The main goals on the product quality and yield, and the migration behaviors of contaminants will be evaluated. The catalytic mechanisms on the degradation of plastics and the removal of contaminant will be comprehensively studied.
The regeneration and activation of catalysts will be conducted under different conditions. Different regeneration methods will be performed to optimize the regeneration conditions.
Attend the 23rd edition of the International Conference on Analytical and Applied Pyrolysis, 15-20 May, 2022.

  • Research Products

    (3 results)

All 2022 2021

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (1 results) (of which Int'l Joint Research: 1 results)

  • [Journal Article] Synergistic effects during co-pyrolysis of milled wood lignin and polyolefins at the gas phase and liquid/solid phase contacting modes2022

    • Author(s)
      Ma Chuan、Xie Shengyu、Kumagai Shogo、Takahashi Yusuke、Saito Yuko、Kameda Tomohito、Yoshioka Toshiaki
    • Journal Title

      Chemical Engineering Journal

      Volume: 431 Pages: 134030~134030

    • DOI

      10.1016/j.cej.2021.134030

    • Peer Reviewed
  • [Journal Article] Enhanced production of phenol and debromination by co-pyrolysis of the non-metallic fraction of printed circuit boards and waste tires2021

    • Author(s)
      Ma Chuan、Kumagai Shogo、Saito Yuko、Kameda Tomohito、Yoshioka Toshiaki
    • Journal Title

      Green Chemistry

      Volume: 23 Pages: 6392~6404

    • DOI

      10.1039/D1GC01176F

    • Peer Reviewed
  • [Presentation] Co-pyrolysis of the non-metallic fraction of printed circuit boards and waste tire2021

    • Author(s)
      Chuan Ma, Shogo Kumagai, Yuko Saito, Tomohito Kameda, Toshiaki Yoshioka
    • Organizer
      International Symposium on Feedstock Recycling of Polymeric Materials
    • Int'l Joint Research

URL: 

Published: 2022-12-28  

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