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2011 Fiscal Year Final Research Report

Atomic scale observation of grain boundary segregation in nuclear materials by atom probe tomography and study on mechanism of grain boundary degradation

Research Project

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Project/Area Number 21246142
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionTohoku University

Principal Investigator

NAGAI Yasuyoshi  東北大学, 金属材料研究所, 教授 (10302209)

Co-Investigator(Kenkyū-buntansha) TOYAMA Takeshi  東北大学, 金属材料研究所, 助教 (50510129)
HATAKEYAMA Masahiko  東北大学, 金属材料研究所, 助教 (30375109)
MATSUKAWA Yoshitaka  東北大学, 金属材料研究所, 助教 (70566356)
SHIMIZU Yasuo  東北大学, 金属材料研究所, 助教 (40581963)
Co-Investigator(Renkei-kenkyūsha) NISHIYAMA Yutaka  独立行政法人日本原子力研究開発機構, 安全研究センター, 主任研究員 (60414596)
YAMAGUCHI Masatake  独立行政法人日本原子力研究開発機構, システム計算科学センター, 研究副主幹 (50360417)
Project Period (FY) 2009 – 2011
Keywords粒界偏析 / 粒界脆化 / 3次元アトムプローブ / 原子炉高経年化
Research Abstract

It is important to understand the degradation mechanism of the grain boundary in the structural materials of aged nuclear reactors for nuclear safety. We have developed new method to observe grain boundary segregations on inter-granular fractured surfaces using laser-assisted three-dimensional atom probe method. The obtained results, combined with the other methods such as Auger electron spectroscopy and the first principles calculations, showed the relationship between inter-granular fracture and grain boundary segregations.

  • Research Products

    (26 results)

All 2012 2011 2010 2009

All Journal Article (10 results) (of which Peer Reviewed: 10 results) Presentation (16 results)

  • [Journal Article] Post-irradiation annealing behavior of microstructure and hardening of a reactor pressure vessel steel studied by positron annihilation and atom probe tomography2012

    • Author(s)
      A. Kuramoto, T. Toyama, T. Takeuchi, Y. Nagai, M. Hasegawa, T. Yoshiie, Y. Nishiyama
    • Journal Title

      J. Nucl. Mater

      Volume: 425 Pages: 65-70

    • Peer Reviewed
  • [Journal Article] Grain boundary segregation in neutron-irradiated 304 stainless steel studied by atom probe tomography2012

    • Author(s)
      T. Toyama, Y. Nozawa, W. Van Renterghem, Y. Matsukawa, M. Hatakeyama, Y. Nagai, A. Al Mazouzi, S. Van Dyck
    • Journal Title

      J. Nucl. Mater

      Volume: 425 Pages: 71-75

    • Peer Reviewed
  • [Journal Article] Microstructural changes of a thermally aged stainless steel submerged arc weld overlay cladding of nuclear reactor pressure vessels2012

    • Author(s)
      T. Takeuchi, J. Kameda, Y. Nagai, T. Toyama, Y. Matsukawa, Y. Nishiyama, K. Onizawa
    • Journal Title

      J. Nucl. Mater

      Volume: 425 Pages: 54-59

    • Peer Reviewed
  • [Journal Article] Irradiation-induced precipitates in a neutron irradiated 304 stainless steel studied by three-dimensional atom probe2011

    • Author(s)
      T. Toyama, Y. Nozawa, W. Van Renterghem, Y. Matsukawa, M. Hatakeyama, Y. Nagai, A. Al Mazouzi, S. Van Dyck
    • Journal Title

      J. Nucl. Mater

      Volume: 418 Pages: 62-68

    • Peer Reviewed
  • [Journal Article] Study on microstructural changes in thermally-aged stainless steel weld-overlay cladding of nuclear reactor pressure vessels by atom probe tomography2011

    • Author(s)
      T. Takeuchi, J. Kameda, Y. Nagai, T. Toyama, Y. Nishiyama, K. Onizawa
    • Journal Title

      J. Nucl. Mater.

      Volume: 415 Pages: 198-204

    • Peer Reviewed
  • [Journal Article] Effects of chemical composition and dose on microstructure evolution and hardening of neutron irradiated reactor pressure vessel steels2010

    • Author(s)
      T. Takeuchi, A. Kuramoto, J. Kameda, T. Toyama, Y. Nagai, M. Hasegawa, T. Ohkubo, T. Yoshiie, Y. Nishiyama and K. Onizawa
    • Journal Title

      J. Nucl. Mater

      Volume: 402 No.2-3 Pages: 93-101

    • Peer Reviewed
  • [Journal Article] Irradiation-induced changes of the atomic distributions around the interfaces of carbides in a nuclear reactor pressure vessel steel2010

    • Author(s)
      T. Toyama, N. Tsuchiya, Y. Nagai, A. Almazouzi, M. Hatakeyama, M. Hasegawa, T. Ohkubo, E. van Walle, R. Gerard
    • Journal Title

      J. Nucl. Mater

      Volume: 405 Pages: 177-180

    • Peer Reviewed
  • [Journal Article] Hardening and microstructural evolution in A533B steels under neutron irradiation and a direct comparison with electron irradiation2010

    • Author(s)
      K. Fujii, H. Nakata, K. Fukuya, T. Ohkubo, K. Hono, Y. Nagai, M. Hasegawa, T. Yoshiie
    • Journal Title

      J. Nucl. Mater

      Volume: 400 Pages: 46-55

    • Peer Reviewed
  • [Journal Article] Use of the Frank-Bilby equation for calculating misfit dislocation arrays in interfaces2010

    • Author(s)
      J. B. Yang, Y. Nagai, M. Hasegawa
    • Journal Title

      Scripta Mater

      Volume: 62 Pages: 458-461

    • Peer Reviewed
  • [Journal Article] Interactions between Fermi surfaces and Brillouin zone boundaries and phase stability of embedded metallic nanoparticles2009

    • Author(s)
      Y. Nagai, T. Toyama, Z. Tang, K. Inoue, T. Chiba, M. Hasegawa, S. Hirosawa and T. Sato
    • Journal Title

      Phys. Rev

      Volume: B79 Pages: 201405(R)

    • Peer Reviewed
  • [Presentation] 原子炉圧力容器オーバーレイクラッドの熱時効によるナノ組織変化2012

    • Author(s)
      鹿窪勇太、武内伴照、西山裕孝、勝山仁哉、鬼沢邦雄、野沢康子、松川義孝、外山健、永井康介、亀田純
    • Organizer
      日本金属学会2012年春期大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2012-03-29
  • [Presentation] 原子力材料の欠陥分布と機能-3次元APと陽電子消滅-2012

    • Author(s)
      永井康介
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-25
  • [Presentation] A533B鋼粒界破面直下からの3次元アトムプローブ観察2011

    • Author(s)
      外山健、野沢康子、松川義孝、畠山賢彦、永井康介、西山裕孝
    • Organizer
      金研ワークショップ「鉄鋼材料照射影響機構研究の最近の進展~ナノ組織から機械的特性へいかにつなげるか? 」
    • Place of Presentation
      東北大学金属材料研究所
    • Year and Date
      20110929-30
  • [Presentation] Positron annihilation study of neutron-irradiated nuclear reactor pressure vessel steels and their model alloys2011

    • Author(s)
      Y. Nagai, A. Kuramoto, T. Toyama, T. Takeuchi, M. Hasegawa
    • Organizer
      The 10^<th> International Workshop on Positron and Positronium Chemistry
    • Place of Presentation
      Smolenice, Slovakia
    • Year and Date
      20110905-11
  • [Presentation] Microstructural analysis just below intergranular fractured surfaces in RPV steels and their model alloys using atom probe tomography2011

    • Author(s)
      T. Toyama, Y. Nozawa, Y. Matsukawa, M. Hatakeyama, Y. Nishiyama, M. Hasegawa, Y. Nagai
    • Organizer
      IGRDM-16
    • Place of Presentation
      Santa Barbara, USA
    • Year and Date
      2011-12-05
  • [Presentation] The correlation of microstructural evolution and hardening of RPV steels studied by atom probe tomography and Positron annihilation2011

    • Author(s)
      A. Kuramoto, T. Takeuchi, T. Toyama, Y. Nagai, M. Hasegawa, T. Yoshiie, Y. Nishiyama
    • Organizer
      IGRDM-16
    • Place of Presentation
      Santa Barbara, USA
    • Year and Date
      2011-12-05
  • [Presentation] 中性子照射した原子炉圧力容器鋼中の溶質クラスターおよびマトリックス欠陥の硬化への寄与2011

    • Author(s)
      蔵本明、外山健、武内伴照、永井康介、長谷川雅幸、義家敏正、西山裕孝
    • Organizer
      日本金属学会2011年秋期大会
    • Place of Presentation
      沖縄コンベンションセンター
    • Year and Date
      2011-11-07
  • [Presentation] 原子炉燃料被覆管材Zr-Nb合金の陽電子消滅法と3次元アトムプローブによる解析2011

    • Author(s)
      松川義孝、斎藤健、外山健、永井康介、金思雄、佐藤裕樹、阿部弘亨、篠原靖周
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学
    • Year and Date
      2011-09-21
  • [Presentation] Effects of Irradiation Dose on Microstructural Evolution and Hardening of High-and Low-Cu Reactor Pressure Vessel Steels2011

    • Author(s)
      A. Kuramoto, T. Takeuchi, T. Toyama, Y. Nagai, M. Hasegawa, T. Yoshiie, Y. Nishiyama
    • Organizer
      TMS 2011
    • Place of Presentation
      San Diego, USA
    • Year and Date
      2011-02-27
  • [Presentation] Atom Probe Technology for Variability Study2011

    • Author(s)
      Y. Nagai
    • Organizer
      International Symposium on Characteristics Variability in Scaled Transistors
    • Place of Presentation
      Institute of Industrial Science, the University of Tokyo
    • Year and Date
      2011-02-10
  • [Presentation] 3次元アトムプローブで調べた中性子照射304ステンレス鋼中のNi-Si析出物の照射後焼鈍回復2010

    • Author(s)
      外山健、野沢康子、松川義孝、畠山賢彦、W. van Renterghem、S. van Dyck、A. Almazouzi
    • Organizer
      日本金属学会2010年秋期大会
    • Place of Presentation
      北海道大学
    • Year and Date
      2010-09-26
  • [Presentation] EBSD・FIB・アトムプローブを用いたΣ3粒界における偏析不純物の定量分析2010

    • Author(s)
      松川義孝、村上有美、永井康介
    • Organizer
      日本金属学会2010年秋期大会
    • Place of Presentation
      北海道大学
    • Year and Date
      2010-09-25
  • [Presentation] 3D Atom Probe Field Ion Microscopy and Positron Annihilation Complementary Use for Materials Research2010

    • Author(s)
      Y. Nagai
    • Organizer
      12^<th> International Workshop on Slow Positron Beam Techniques
    • Place of Presentation
      Magnetic Island, Australia
    • Year and Date
      2010-08-03
  • [Presentation] Evolution of Nano-structures in Pressure Vessel Steels in the Course of Irradiation2010

    • Author(s)
      Y. Nagai, T. Toyama, M. Hasegawa, T. Ohkubo, A. Almazouzi, E. van Walle, R. Gerard
    • Organizer
      5^<th> Forum on New Materials, CIMTEC 2010
    • Place of Presentation
      Montecatini Terme, Italy
    • Year and Date
      2010-06-17
  • [Presentation] ナノ構造変化の解明に基づいた原子炉材料の劣化予測の重要性2010

    • Author(s)
      永井康介
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      岡山大学
    • Year and Date
      2010-03-22
  • [Presentation] Post irradiation annealing of a surveillance test specimen of Dole-4 reactor in Belgium studied by LEAP and positron annihilation2009

    • Author(s)
      T. Toyama, Y. Nagai, N. Tsuchiya, M. Hasegawa, T. Ohkubo, A. Almazouzi, E. van Walle, R. Gerard
    • Organizer
      IGRDM-15
    • Place of Presentation
      Budapest, Hungary
    • Year and Date
      2009-10-12

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Published: 2013-07-31  

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