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2011 Fiscal Year Final Research Report

Laboratory study of aging of secondary organic aerosol formed from the photooxidation of aromatic hydrocarbons

Research Project

  • PDF
Project/Area Number 21510023
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionNational Institute for Environmental Studies

Principal Investigator

SATO Kei  独立行政法人国立環境研究所, 地域環境研究センター, 主任研究員 (10282815)

Project Period (FY) 2009 – 2011
Keywords芳香族炭化水素 / 二次有機エアロゾル / 光化学スモッグチャンバー / エアロゾル質量分析計 / 液体クロマトグラフ質量分析計
Research Abstract

Oxygenated organic aerosol(OOA) observed in remote areas is believed to comprise aged secondary organic aerosol(SOA); however, the reaction processes relevant to SOA chemical aging have hitherto been unclear. We analyzed SOA particles formed from the photooxidation of aromatic hydrocarbons using an Aerosol mass spectrometry, liquid chromatography/mass spectrometry, and iodometric spectrophotometry. These results indicate that SOA aging proceeds mainly by formation of carboxylic acids, and that the rate of SOA aging in laboratory chambers is limited by the oxidation of ketone groups.

  • Research Products

    (11 results)

All 2012 2011 2010 2009

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (8 results)

  • [Journal Article] AMS and LC/MS analyses of SOA from the photooxidation of benzene and 1, 3, 5-trimethylbenzene in the presence of NOx : Effects of chemical structure on SOA aging2012

    • Author(s)
      Sato, K., Takami, A., Kato, Y., Seta, T., Fujitani, Y., Hikida, T., Shimono, A., and Imamura, T.
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 12(in press)

    • Peer Reviewed
  • [Journal Article] AMS and LC/MS analyses of SOA from the photooxidation of benzene and 1, 3, 5-trimethylbenzene in the presence of NOx : Effects of chemical structure on SOA aging2012

    • Author(s)
      Sato, K., Takami, A., Kato, Y., Seta, T., Fujitani, Y., Hikida, T., Shimono, A., and Imamura, T.
    • Journal Title

      Atmospheric Chemistry and Physics Discussions

      Volume: 12 Pages: 283-318

    • DOI

      DOI:10.5194/acpd-12-283-2012

    • Peer Reviewed
  • [Journal Article] Mass spectrometric study of secondary organic aerosol formed from the photo-oxidation of aromatic hydrocarbons2009

    • Author(s)
      Sato, K., Takami, A., Isozaki, T., Hikida, T., Shimono, A., Imamura, T.
    • Journal Title

      Atmospheric Environment

      Volume: 44(8) Pages: 1080-1087

    • DOI

      DOI:10.1016/j.atmosenv.2009.12.013

    • Peer Reviewed
  • [Presentation] 芳香族炭化水素の光酸化からの二次有機エアロゾル中に存在する含窒素有機化合物2012

    • Author(s)
      佐藤圭,高見昭憲,加藤吉康,瀬田孝将,疋田利秀,下野彰夫,今村隆史
    • Organizer
      第92日本化学会春季年会
    • Place of Presentation
      慶應義塾大学日吉キャンパス(神奈川県)
    • Year and Date
      2012-03-25
  • [Presentation] 芳香族炭化水素の光酸化からの二次有機エアロゾル生成とそのエイジング2011

    • Author(s)
      佐藤圭,高見昭憲,磯崎輔,加藤吉康,瀬田孝将,下野彰夫,疋田利秀,今村隆史
    • Organizer
      第17回大気化学討論会
    • Place of Presentation
      京都大学宇治キャンパス(京都府)
    • Year and Date
      2011-10-19
  • [Presentation] AMS and LC-MS analyses of secondary organic aerosol formed from the benzene and 1, 3, 5-trimethylbenzene photooxidation in presence of NOx2011

    • Author(s)
      Sato, K., Takami, A., Imamura, T.
    • Organizer
      American Association for Aerosol Research 30^<th> Annual Conference
    • Place of Presentation
      Rosen Shingle Creek Resort & Golf Club(Orlando, USA)
    • Year and Date
      2011-10-05
  • [Presentation] ヨウ素滴定法による二次有機エアロゾル中のオキシダントの測定(II)2011

    • Author(s)
      佐藤圭,藤谷雄二,瀬田孝将,今村隆史,高見昭憲
    • Organizer
      第28回エアロゾル科学・技術研究討論会
    • Place of Presentation
      大阪府立大学中百舌鳥キャンパス(大阪府)
    • Year and Date
      2011-08-29
  • [Presentation] ヨウ素滴定法による二次有機エアロゾル中のオキシダントの測定2011

    • Author(s)
      佐藤圭,藤谷雄二,瀬田孝将,今村隆史,高見昭憲
    • Organizer
      日本地球惑星科学連合2011年大会
    • Place of Presentation
      幕張メッセ国際会議場(千葉県)
    • Year and Date
      2011-05-23
  • [Presentation] 芳香族炭化水素の光酸化で生成する二次有機エアロゾルの質量スペクトル2010

    • Author(s)
      佐藤圭,高見昭憲,磯崎輔,今村隆史
    • Organizer
      2010年光化学討論会
    • Place of Presentation
      千葉大学西千葉キャンパス(千葉県)
    • Year and Date
      2010-09-08
  • [Presentation] Mass spectroscopic study of secondary organic aerosol from the photooxidation of aromatic hydrocarbons2009

    • Author(s)
      Sato, K., Takami, A., Isozaki, T., Hikida, T., Shimono, A., Imamura, T.
    • Organizer
      American Association for Aerosol Research 28^<th> Annual Conference
    • Place of Presentation
      Hyatt Regency Minneapolis(Minneapolis, USA)
    • Year and Date
      2009-10-28
  • [Presentation] エアロゾル質量分析計による芳香族炭化水素からの二次粒子測定2009

    • Author(s)
      佐藤圭,高見昭憲,磯崎輔,疋田利秀,下野彰夫,今村隆史
    • Organizer
      日本地球惑星科学連合2009年大会
    • Place of Presentation
      幕張メッセ国際会議場(千葉県)
    • Year and Date
      2009-05-20

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Published: 2013-07-31  

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