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2011 Fiscal Year Final Research Report

The invention of the new layered superconductor by intercalation and the ion exchange.

Research Project

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Project/Area Number 21560006
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied materials science/Crystal engineering
Research InstitutionTohoku University

Principal Investigator

NOJI Takashi  東北大学, 大学院・工学研究科, 助教 (50180740)

Co-Investigator(Kenkyū-buntansha) KOIKE Yoji  東北大学, 大学院・工学研究科, 教授 (70134038)
Project Period (FY) 2009 – 2011
Keywords超伝導 / 鉄系超伝導体 / 単結晶 / 比熱
Research Abstract

We have investigated the electronic specific heat of FeSe1-xTex (0. 6≦x≦1)single crystals as-grown and annealed at 400℃ for 100-200 h in vacuum. The appearance of bulk superconductivity with a clear specific-heat jump at the superconducting (SC)transition temperature, Tc has been confirmed in annealed single-crystals of x=0. 6-0. 9. For annealed single-crystals of x=0. 6-0. 9, values of the SC condensation energy at 0 K, U0, the thermodynamic critical field, Hc(0), the SC gap at 0 K, Δ0 and ΔC/(γn-γ0)Tc [ΔC : the specific-heat jump at Tc, γn : the electronic specific-heat coefficient in the normal state, γ0 : the residual electronic specific-heat coefficient at 0 K in the SC state] have been estimated. It has been found the superconductivity is strongest in the 200h-annealed single-crystal of x=0. 7, where 2Δ0/kBTc estimated using the single-band BCS s-wave model and ΔC/(γn-γ0)Tc are 4. 29 and 2. 76, respectively, indicating that the superconductivity is strong-coupling.

  • Research Products

    (42 results)

All 2012 2011 2010 2009 Other

All Journal Article (10 results) (of which Peer Reviewed: 10 results) Presentation (31 results) Remarks (1 results)

  • [Journal Article] Strong-Coupling Superconductivity2012

    • Author(s)
      Takashi Noji, Masato Imaizumi, Takumi Suzuki, Tadashi Adachi, Masatsune Kato, and Yoji Koike
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 81 Pages: 054708-1-7

    • Peer Reviewed
  • [Journal Article] earch for New Superconductors by Soft-Chemical Techniques2012

    • Author(s)
      asatsune Kato, Tomohisa Takamatsu, Hotaka Yagyu, Takashi Noji and Yoji Koike
    • Journal Title

      Key Engineering Materials

      Volume: 508 Pages: 203-206

    • Peer Reviewed
  • [Journal Article] Synthesis and Specific Heat of CaPdH3-δ with the Perovskite Structure2012

    • Author(s)
      Shin-ya Ayukawa, Kazutaka Ikeda, Masatsune Kato, Takashi Noji, Shin-ichi Orimo, and Yoji Koike
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 81 Pages: 034704-1-5

    • Peer Reviewed
  • [Journal Article] ow-temperature synthesis of T'-La2CuO4 using CaH2 as reductant2011

    • Author(s)
      T. Takamatsu, M. Kato, T. Noji, Y. Koike.
    • Journal Title

      Physica C

      Volume: 471 Pages: 679-681

    • Peer Reviewed
  • [Journal Article] Annealing effects on the crystal structure and physical properties of FeSe1-xTex(0.6≦x≦1)single crystals2011

    • Author(s)
      M. Imaizumi, T. Noji, T. Adachi, Y. Koike.
    • Journal Title

      Physica C

      Volume: 471 Pages: 614-617

    • Peer Reviewed
  • [Journal Article] Growth, Annealing Effects on Superconducting and Magnetic Properties, and Anisotropy of FeSe1-xTex (0.5≦x≦1)Single Crystals2010

    • Author(s)
      Takashi Noji, Takumi Suzuki, Haruki Abe, Tadashi Adachi, Masatsune Kato, Yoji Koike
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 79 Pages: 084711-1-5

    • Peer Reviewed
  • [Journal Article] A new family of superconducting intercalation compound of MgxMNCl (M=Zr, Hf)2010

    • Author(s)
      Hotaka Yagyu, Masatsune Kato, Hiroto Tezuka, Takashi Noji, Shoji Yamanaka, Yoji Koike
    • Journal Title

      Physica C

      Volume: 470 Pages: S760-S61

    • Peer Reviewed
  • [Journal Article] Superconductivity and electrochemistry of the spinel Li1+ xTi2O42010

    • Author(s)
      Shota Hamada, Masatsune Kato, Takashi Noji, Yoji Koike
    • Journal Title

      Physica C

      Volume: 470 Pages: S766-S767

    • Peer Reviewed
  • [Journal Article] A New Intercalation Superconductor Mgx(PC)yZrNCl2010

    • Author(s)
      H. Tezuka, M. Kato, T. Noji, S. Yamanaka, and Y. Koike
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 49 Pages: 020210-1-2

    • Peer Reviewed
  • [Journal Article] Rapid low-temperature synthesis of superconducting (Ba, Ru)BiO3 usingmolten RbOH2009

    • Author(s)
      M. Kato, S. Shitara, T. Minakawa, T. Noji, and Y. Koike
    • Journal Title

      Journal of Physics

      Volume: 150 Pages: 052100-1-4

    • Peer Reviewed
  • [Presentation] FeSe1-xTex (0. 6≦x≦1)単結晶の磁場中比熱2012

    • Author(s)
      今泉真人、足立匡、野地尚、川股隆行、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      西宮市
    • Year and Date
      2012-03-26
  • [Presentation] μSRからみたFeSe1-xTex (0. 6≦x≦1)単結晶におけるab面内磁場侵入長2012

    • Author(s)
      足立匡、今泉真人、鈴木謙介、野地尚、大石一城、渡邊功雄、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      西宮市
    • Year and Date
      2012-03-25
  • [Presentation] 還元剤CaH2を用いたホールドープ型T'-La2-xCaxCuO4のバルク試料の合成」2012

    • Author(s)
      高松智寿、加藤雅恒、野地尚、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      西宮市
    • Year and Date
      2012-03-25
  • [Presentation] ペロブスカイト型水素化物APdH3-δ(A=Ca, Sr)における超伝導発現の可能性」2012

    • Author(s)
      鮎川晋也、池田一貴、加藤雅恒、野地尚、折茂慎一、小池洋二
    • Organizer
      応用物理学会
    • Place of Presentation
      東京都
    • Year and Date
      2012-03-15
  • [Presentation] Search for New Superconductors by Soft-Chemical Techniques2011

    • Author(s)
      Masatsune Kato, Tomohisa Takamatsu, Takashi Noji and Yoji Koike
    • Organizer
      The 2nd International Symposium on Advanced Synthesis and Processing Technology for Matertials
    • Place of Presentation
      仙台市
    • Year and Date
      2011-12-01
  • [Presentation] 新規ビスマス層状物質Bi4O4Cl2Seの発見と超伝導化を目指したLiインターカレーションによるキャリアドープ」2011

    • Author(s)
      若吉一輝、加藤雅恒、野地尚、小池洋二
    • Organizer
      応用物理学会東北支部学術講演会
    • Place of Presentation
      盛岡市
    • Year and Date
      2011-12-01
  • [Presentation] アニール処理した11相鉄系超伝導体FeSe1-xTex (0. 6≦x≦1)単結晶の比熱2011

    • Author(s)
      野地尚、今泉真人、足立匡、小池洋二
    • Organizer
      第5回物性科学領域横断研究会
    • Place of Presentation
      仙台市
    • Year and Date
      2011-11-20
  • [Presentation] FeSe1-xTex (0. 6≦x≦1)単結晶の超伝導と磁気相関のx依存性2011

    • Author(s)
      今泉真人、野地尚、足立匡、大石一城、渡邊功雄、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      富山市
    • Year and Date
      2011-09-22
  • [Presentation] 比熱とμSRから見たFeSe1-xTex (0. 6≦x≦1)単結晶の超伝導と電子状態2011

    • Author(s)
      今泉真人、野地尚、足立匡、川股隆行、大石一城、渡邊功雄、小池洋二
    • Organizer
      応用物理学会
    • Place of Presentation
      山形市
    • Year and Date
      2011-09-01
  • [Presentation] Cl部分欠損によるMOCl(M=Y, La)への電子キャリアドープ」2011

    • Author(s)
      柳生穂高、加藤雅恒、野地尚、小池洋二
    • Organizer
      応用物理学会
    • Place of Presentation
      山形市
    • Year and Date
      2011-09-01
  • [Presentation] Superconductivity and electronic state of annealed single-crystals of FeSe1-xTex (0. 6≦x≦1)studied by specific heat2011

    • Author(s)
      M. Imaizumi, T. Noji, T. Adachi, K. Ohishi, I. Watanabe, and Y. Koike
    • Organizer
      International Conference of Low Temperature Physics (LT26)
    • Place of Presentation
      北京「中国」
    • Year and Date
      2011-08-10
  • [Presentation] Specific-heat of the superconductivity and electronic state in FeSe1-xTex single crystals2011

    • Author(s)
      Y. Koike, M. Imaizumi and T. Noji
    • Organizer
      The International Conference on Novel Superconductivity (ICNSCT2011)
    • Place of Presentation
      台南「台湾」
    • Year and Date
      2011-08-05
  • [Presentation] Search for new superconductors in layered oxychlorides MOCl (M : Y, La)by soft-chemical techniques2011

    • Author(s)
      H. Yagyu, M. Kato, T. Noji and Y. Koike
    • Organizer
      The International Conference on Novel Superconductivity (ICNSCT2011)
    • Place of Presentation
      台南「台湾」
    • Year and Date
      2011-08-04
  • [Presentation] 比熱とμSRから見たアニール処理したFeSe1-xTex (0. 5≦x ≦1)単結晶の超伝導特性と磁性2011

    • Author(s)
      今泉真人、野地尚、足立匡、小池洋二、大石一城、渡邊功雄
    • Organizer
      日本物理学会
    • Place of Presentation
      新潟市
    • Year and Date
      2011-03-27
  • [Presentation] Electronic Specific-Heat of Annealed Single-Crystals of FeSe1-xTex (0. 6≦x≦1)2011

    • Author(s)
      Takashi Noji, Masao Imaizumi, Tadashi Adachi, Yoji Koike
    • Organizer
      International Workshop on Superconductors and Super Materials 2011
    • Place of Presentation
      東京
    • Year and Date
      2011-03-07
  • [Presentation] ソフト化学法を用いたMOCl(M=Y, La, Yb)における新超伝導物質探索2010

    • Author(s)
      柳生穂高、加藤雅恒、野地尚、小池洋二
    • Organizer
      応用物理学会東北支部学術講演会
    • Place of Presentation
      仙台市
    • Year and Date
      2010-11-25
  • [Presentation] Low-temperature synthesis of T'-La2CuO4 using CaH2 as reductant2010

    • Author(s)
      T. Takamatsu, M. Kato, T. Noji, Y. Koike
    • Organizer
      23th International Symposium on Superconductivity (ISS)
    • Place of Presentation
      つくば市
    • Year and Date
      2010-11-01
  • [Presentation] Annealing effects on crystal structure and physical properties of FeSe1-xTex (0. 5≦x≦1)single crystals2010

    • Author(s)
      M. Imaizumi, T. Noji, T. Suzuki, T. Adachi, M. Kato, Y. Koike
    • Organizer
      23th International Symposium on Superconductivity(ISS)
    • Place of Presentation
      つくば市
    • Year and Date
      2010-11-01
  • [Presentation] 層状塩化酸化物MOCl(M=Y, La)における新超伝導物質探索2010

    • Author(s)
      柳生穂高、加藤雅恒、野地尚、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府
    • Year and Date
      2010-09-25
  • [Presentation] FeSe1-xTex(0. 5≦x≦1)単結晶のアニール処理による結晶構造と物性の変化2010

    • Author(s)
      今泉真人、野地尚、鈴木匠、足立匡、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府
    • Year and Date
      2010-09-25
  • [Presentation] Bi2Se3へのインターカレーションによる新超伝導物質の探索2010

    • Author(s)
      若吉一輝、加藤雅恒、野地尚、小池洋二
    • Organizer
      応用物理学会
    • Place of Presentation
      大阪府
    • Year and Date
      2010-09-25
  • [Presentation] BiOX(X=CL, I)へのLiインターカレーションによる新超伝導物質の探索2010

    • Author(s)
      濱田翔太、加藤雅恒、野地尚、小池洋二
    • Organizer
      応用物理学会
    • Place of Presentation
      長崎市
    • Year and Date
      2010-09-14
  • [Presentation] ソフト化学法を用いたα. MOCl(M=Y, La)における新超伝導物質探索2010

    • Author(s)
      加藤雅恒、柳生穂高、高松智寿、野地尚、小池洋二
    • Organizer
      日本セラミックス協会
    • Place of Presentation
      小金井市
    • Year and Date
      2010-03-23
  • [Presentation] FeSe1-xTex(0. 5≦x≦1)単結晶のアニール効果とHc2の異方性2010

    • Author(s)
      鈴木匠、野地尚、阿部晴幾、足立匡、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      岡山市
    • Year and Date
      2010-03-21
  • [Presentation] FeSe1-xTex単結晶育成と上部臨界磁場の異方性2010

    • Author(s)
      野地尚、鈴木匠、阿部晴幾、足立匡、小池洋二
    • Organizer
      応用物理学会
    • Place of Presentation
      平塚市
    • Year and Date
      2010-03-18
  • [Presentation] FeSe系超伝導体へのLiインターカレーション効果2009

    • Author(s)
      鈴木匠、野地尚、阿部晴幾、足立匡、小池洋二
    • Organizer
      応用物理学会東北支部学術講演会
    • Place of Presentation
      郡山市
    • Year and Date
      2009-12-03
  • [Presentation] FeTe1-xMx(M=Se, S)へのLiインターカレーション効果2009

    • Author(s)
      阿部晴幾、野地尚、加藤雅恒、鈴木匠、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      熊本市
    • Year and Date
      2009-09-26
  • [Presentation] Liインターカレーション・デインタカレーションによるLi1+ xTi2O4の超伝導2009

    • Author(s)
      濱田翔太、加藤雅恒、野地尚、小池洋二
    • Organizer
      日本物理学会
    • Place of Presentation
      熊本市
    • Year and Date
      2009-09-26
  • [Presentation] Superconductivity and Electrochemistry of Spinel Li1+ xTi2O42009

    • Author(s)
      S. Hamada, M. Kato, T. Noji, and Y. Koike
    • Organizer
      9th International Conference on Materials and Mechanisms of Superconductivity
    • Place of Presentation
      東京都
    • Year and Date
      2009-09-09
  • [Presentation] A New Family of Superconducting Intercalation Compound Of MgxZrNCl2009

    • Author(s)
      M. Kato, H. Tezuka, T. Noji, S. Yamanaka, and Y. Koike
    • Organizer
      9th International Conference on Materials and Mechanisms of Superconductivity
    • Place of Presentation
      東京都
    • Year and Date
      2009-09-09
  • [Presentation] Electrochemical Li-Intercalation into the Fe-Based Superconductor FeSe1-xTex2009

    • Author(s)
      H. Abe, T. Noji, M. Kato, and Y. Koike
    • Organizer
      9th International Conference on Materials and Mechanisms of Superconductivity
    • Place of Presentation
      東京都
    • Year and Date
      2009-09-09
  • [Remarks]

    • URL

      http://www.apph.tohoku.ac.jp/low-temp-lab/

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Published: 2013-07-31  

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