Towards the three dimensional structural analysis of liquid by using x-ray free electron laser

2011 Fiscal Year Final Research Report

• Project/Area Number: 21654050
• Research Category: Grant-in-Aid for Challenging Exploratory Research
• Allocation Type: Single-year Grants
• Research Field: Condensed matter physics II
• Research Institution: Kyoto University
• Principal Investigator: YAO Makoto 京都大学, 大学院・理学研究科, 教授 (70182293)
• Co-Investigator(Kenkyū-buntansha): NAGAYA Kiyonobu 京都大学, 大学院・理学研究科, 助教 (30273436) ; KAWAKITA Yukinobu 日本原子力研究開発機構, J-PARCセンター (50264015)
• Project Period (FY): 2009 – 2011
• Keywords: X線自由電子レーザー / ナノ液滴 / 室温イオン液体 / 液体構造解析 / 逆モンテカルロ法

Research Abstract

We have developed an experimental apparatus and an analysis method aiming at realization of the three-dimensional structural analysis of the liquid using X-ray free electron laser. We developed an electro-spray ionization apparatus for producing liquid droplet sample for XFEL experiments. We also estimated the sample damage caused by FEL using SCSS test accelerator. A structure analysis method in the real space based on the reverse Monte Carlo method was developed.

Research Products

• [Journal Article] Doubly resonant three-photon double ionization of Ar atoms induced by an EUV free-electron laser (2011)
  • Author(s): E. V. Gryzlova, Ri Ma, H. Fukuzawa, K. Motomura, A. Yamada, K. Ueda, A. N. Grum-Grzhimailo, N. M. Kabachnik, S. I. Strakhova, A. Rouz´ee, A. Hundermark, M. J. J. Vrakking, P. Johnsson, K. Nagaya, S. Yase, Y. Mizoguchi, M. Yao, M. Nagasono, K. Tono, T. Togashi, Y. Senba, H. Ohashi, M. Yabashi, and T. Ishikawa
  • Journal Title: Phys Rev Volume: A84 Pages: 063405
  • Peer Reviewed
• [Journal Article] Second-order autocorrelation of XUV FEL pulses via time resolved two-photon single ionization of He (2011)
  • Author(s): R. Moshammer, Th. Pfeifer, A. Rudenko, Y. H. Jiang, L. Foucar, M. Kurka, K. U. Kuhnel, C. D. Schroter, J. Ullrich, O. Herrwerth, M. F. Kling, X.-J. Liu, K. Motomura, H. Fukuzawa, A. Yamada, K. Ueda, K. L. Ishikawa, K. Nagaya, H. Iwayama, A. Sugishima, Y. Mizoguchi, S. Yase, M. Yao, N. Saito, A. Belkacem, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura, and T. Togash
  • Journal Title: OPTICS EXPRESS Volume: Vol.19, Issue 22 Pages: 21698-21706
  • Peer Reviewed
• [Journal Article] Coulomb explosion imaging of bromo-benzene and bromophenol molecules following Br K-shell ionization (2010)
  • Author(s): H Iwayama, K Nagaya, H Murakami, Y Ohmasa, M Yao
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 43 Pages: 185207
  • Peer Reviewed
• [Journal Article] Photoelectron spectroscopy of sequential three-photon double ionization of Ar irradiated by EUV free-electron laser pulses (2010)
  • Author(s): H Fukuzawa, E V Gryzlova, K Motomura, A Yamada, K Ueda, A N Grum-Grzhimailo, S I Strakhova, K Nagaya, A Sugishima, Y Mizoguchi, H Iwayama, M Yao, N Saito, P Piseri, T Mazza, M Devetta, M Coreno, M Nagasono, K Tono, M Yabashi, T Ishikawa, H Ohashi, H Kimura, T Togashi and Y Senba
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 43 Pages: 111001
  • Peer Reviewed
• [Journal Article] Ion-ion coincidence studies on multiple ionizations of N2 and O2 molecules irradiated by EUV free-electron laser pulses (2010)
  • Author(s): A. Yamada, H. Fukuzawa, K. Motomura, X.-J. Liu, L. Foucar, M. Kurka, M. Okunishi, K. Ueda, N. Saito, H. Iwayama, K. Nagaya, A. Sugishima, H. Murakami, M. Yao, A. Rudenko, K. U. Kuhnel, J. Ullrich, R. Feifel, A. Czasch, R. Dorner, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura, and T. Togashi
  • Journal Title: J. Chem. Phys. Volume: 132 Pages: 204305
  • Peer Reviewed
• [Journal Article] Contact less measurements of charge migration within single molecules (2010)
  • Author(s): K. Nagaya, H. Iwayama, A. Sugishima, Y. Ohmasa, M. Yao
  • Journal Title: App. Phys. Lett. Volume: 96 Pages: 233101
  • Peer Reviewed
• [Journal Article] Inhomogeneous charge redistribution in Xe clusters exposed to intense extreme ultraviolet free electron laser (2010)
  • Author(s): H. Iwayama, A. Sugishima, K. Nagaya, M. Yao, , H. Fukuzawa, K. Motomura, X.-J. Liu, A. Yamada, C. Wang, K. Ueda, N. Saito, M. Nagasono, K. Tono, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura, and T. Togashi
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 43 Pages: 161001
  • Peer Reviewed
• [Journal Article] Multiple ionization of atomic argon irradiated by EUV free-electron laser pulses at 62 nm : evidence of sequential electron strip (2009)
  • Author(s): K. Motomura, H. Fukuzawa, L. Foucar, X.-J. Liu, G. Prumper, K. Ueda, N. Saito, H. Iwayama, K. Nagaya, H. Murakami, M. Yao, A. Belkacem, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi and H. Kimura
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys Volume: 42 Pages: 221003
  • Peer Reviewed
• [Journal Article] Dissociation dynamics of C6H6 and C6H5F molecules following carbon 1s and fluorine 1s photoionization studied by 3D momentum imaging method (2009)
  • Author(s): K. Nagaya, H. Iwayama, M. Yao, J. Adachi, Y. Kimura, M. Yamazaki, A. Yagishita
  • Journal Title: J. Chem. Phys. Volume: 131 Pages: 114309
  • Peer Reviewed
• [Journal Article] Frustration of direct photoionizations of Ar clusters in intense extreme ultraviolet pulses from a free electron laser (2009)
  • Author(s): K. Nagaya, M. Yao, H. Fukuzawa, X.-J. Liu, G. Prumper, M. Okunishi, K. Shimada, K. Ueda, T. Harada, M. Toyoda, M. Yanagihara, M. Yamamoto, K. Motomura, N. Saito, A. Rudenko, J. Ullrich, L. Foucar, A. Czasch, R. Dorner, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, and H. Kimura
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 42 Pages: 134019
  • Peer Reviewed
• [Presentation] Dynamics of multiple photoionization of rare-gas clusters caused by intense EUV-FEL pulses (2011)
  • Author(s): K. Nagaya
  • Organizer: International workshop DyNano 2011 Structure and Dynamics of Nano-objects using short wavelength radiation
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 20111003-07
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 日本物理学会第66回年次大会
  • Place of Presentation: 新潟大学
  • Year and Date: 20110325-28
• [Presentation] 動的光散乱法による複雑液体の表面張力波の研究 (2011)
  • Author(s): 大政義典, 八尾誠
  • Organizer: 文部科学省科学特別研究費補助金特定領域研究報告会特定領域研究ソフトマター物理研究会
  • Place of Presentation: 東京大学
  • Year and Date: 20110100
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 日本物理学会秋季大会
  • Place of Presentation: 富山大学
  • Year and Date: 2011-09-24
• [Presentation] International workshop DyNano2011" Structure and Dynamics of Nano-objects using short wavelength radiation" (2010)
  • Author(s): K. Nagaya, H. Iwayama and M. Yao, Kyoto U.
  • Organizer: Measurements of charge migration within single molecules using deep inner-core excitation combined with molecular imaging method
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 20101003-07
• [Presentation] Studies on Interaction of Clusters with Intense EUV-FEL Pulses at Spring 8 (2010)
  • Author(s): K. Nagaya
  • Organizer: International conference on many particle spectroscopy of atoms, molecules, clusters and surfaces(MPS2010)
  • Place of Presentation: Sendai, Japan
  • Year and Date: 20100904-07
• [Presentation] Metallic-like droplets produced by irradiating rare-gas clusters with free electron laser pulses (2010)
  • Author(s): Makoto Yao
  • Organizer: 14th International Conference on Liquid and Amorphous Metals
  • Place of Presentation: Italy, Roma
  • Year and Date: 20100711-16
• [Presentation] Self-organized charge redistribution in pure and mixed rare-gas clusters (2010)
  • Author(s): Makoto YAO
  • Organizer: International Workshop(DyNano-2010): Structure and Dynamics of Nano-objects using short wavelength radiation
  • Place of Presentation: France, Corsica
  • Year and Date: 20100421-25
• [Presentation] イオン化におけるMore is Different (2010)
  • Author(s): 八尾誠
  • Organizer: Symposium on"Invitation to Integrated Complex System Sciences"
  • Place of Presentation: 京都大学理学研究科セミナーハウス
  • Year and Date: 2010-08-05
• [Presentation] Inhomogeneous chemical reaction fields (2010)
  • Author(s): M. Yao
  • Organizer: Workshop of Room Temperature Ionic Liquids in NDA
  • Place of Presentation: 防衛大学
  • Year and Date: 2010-07-21
• [Presentation] Cluster experiments at SCSS : present status and perspective
  • Author(s): K. Nagaya, Kyoto U.
  • Organizer: JSPS-DFG Bilateral Seminar
  • Place of Presentation: Kyoto, Japan