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2022 Fiscal Year Annual Research Report

MOFを出発物質として用いた固体スーパーキャパシタ用新規電極材料の創製

Research Project

Project/Area Number 21F20072
Research InstitutionNational Institute for Materials Science

Principal Investigator

山内 悠輔  国立研究開発法人物質・材料研究機構, 国際ナノアーキテクトニクス研究拠点, MANA主任研究者 (10455272)

Co-Investigator(Kenkyū-buntansha) LIU SHUDE  国立研究開発法人物質・材料研究機構, 国際ナノアーキテクトニクス研究拠点, 外国人特別研究員
Project Period (FY) 2021-09-28 – 2023-03-31
KeywordsPorous materials
Outline of Annual Research Achievements

Our research has focused on developing MOF-derived materials for energy storage and conversion applications with improved electrochemical performance. Through various synthesis methods, including direct carbonization, template-assisted synthesis, and chemical activation, we have prepared MOF-derived carbon-based materials with high specific surface area, pore volume, and conductivity, which are crucial factors for enhancing electrochemical performance in energy storage devices. For example, wevhave used a self-templating method to prepare hollow ordered mesoporous carbon (HOMC) materials with high N-doping, which have demonstrated superior electrochemical performance for supercapacitors. In addition, I have explored the potential of sulfides in energy storage and conversion, constructing a dual-modulated NiCo2O4@NiCo2S4 heterostructure and incorporating sulfur vacancies in CuCo2S4 hollow nanoarchitectures to achieve enhanced electrochemical performance. Furthermore, we have explored interfacial coupled engineering of plasmonic amorphous MoO3-x nanodots/g-C3N4 nanosheets for photocatalytic water splitting and photothermal conversion, developing highly active photocatalysts with excellent electrochemical performance. Overall, our research has demonstrated the great potential of MOF-derived materials, sulfides, and their heterostructures for energy storage and conversion applications, with publications in prestigious journals such as Energy Storage Materials, Carbon Energy, Advanced Energy Materials, and Small.

Research Progress Status

令和4年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

令和4年度が最終年度であるため、記入しない。

  • Research Products

    (4 results)

All 2023 2022

All Journal Article (4 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 4 results)

  • [Journal Article] Unveiling the effect of structural water on Zn-ion storage of polyoxovanadate for high-rate and long-life aqueous zinc ion battery2023

    • Author(s)
      He Huan、Pan Fu-Chun、Liang Xue-Wei、Hu Qiang、Liu Shude、Hu Jisong、Jun Seong Chan、Lin Dunmin、Yamauchi Yusuke、Huo Yu
    • Journal Title

      Chemical Engineering Journal

      Volume: 462 Pages: 142221~142221

    • DOI

      10.1016/j.cej.2023.142221

    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Interfacial coupled engineering of plasmonic amorphous MoO3-x nanodots/g-C3N4 nanosheets for photocatalytic water splitting and photothermal conversion2023

    • Author(s)
      Ren Yumei、Feng Desheng、Yan Zhiming、Sun Zixu、Zhang Zixuan、Xu Dongwei、Qiao Chong、Chen Zhonghui、Jia Yu、Chan Jun Seong、Liu Shude、Yamauchi Yusuke
    • Journal Title

      Chemical Engineering Journal

      Volume: 453 Pages: 139875~139875

    • DOI

      10.1016/j.cej.2022.139875

    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Sodium preintercalation-induced oxygen-deficient hydrated potassium manganese oxide for high-energy flexible Mg-ion supercapacitors2023

    • Author(s)
      Liu Shude、Kang Ling、Zhang Jian、Jun Seong Chan、Yamauchi Yusuke
    • Journal Title

      NPG Asia Materials

      Volume: 15 Pages: 9

    • DOI

      10.1038/s41427-022-00450-z

    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Covalently Interlayer‐Confined Organic-Inorganic Heterostructures for Aqueous Potassium Ion Supercapacitors2022

    • Author(s)
      Chen Jianping、Liu Bin、Cai Hang、Liu Shude、Yamauchi Yusuke、Jun Seong Chan
    • Journal Title

      Small

      Volume: 19 Pages: 2204275~2204275

    • DOI

      10.1002/smll.202204275

    • Peer Reviewed / Int'l Joint Research

URL: 

Published: 2023-12-25  

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