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2021 Fiscal Year Research-status Report

Spin Freezing Crossover and Cooper Pairing Symmetry in the Organic Strange Metal kappa-(ET)4Hg2.89Br8 and kappa-(ET)4Hg2.78Cl8

Research Project

Project/Area Number 21K13885
Research InstitutionShibaura Institute of Technology

Principal Investigator

Dita PuspitaSari  芝浦工業大学, 工学部, 助教 (00821919)

Project Period (FY) 2021-04-01 – 2025-03-31
KeywordsCooper pair / Strange metal / Spin freezing / SYK model / Hubbard model / Non-Fermi liquid / QCP / AdS/CFT correspondence
Outline of Annual Research Achievements

The 200 mg of superconducting k-[ET]4Hg2.89Br8 [k-HgBr] and Mott-insulating k-[ET]4Hg2.78Cl8 (k-HgCl) crystals are synthesized and aligned for the zero (ZF), transverse (TF), and longitudinal-field (LF) muSR experiments. In the k-HgBr, ZF-muSR down to 0.3 K suggest no time-reversal symmetry breaking in the superconducting state while LF and TF muSR for determining the Cooper pairing symmetry, have not been performed.
In the k-HgCl, the muon Knight shift measurement by the high-TF-muSR has been done for the first time in the world. Susceptibility dependence of the shift showed a non-linearity below 100 K occurring at a higher temperature than that in k-HgBr.
We aim to finalize the series of muSR experiments for both samples by the end of next fiscal year.

Current Status of Research Progress
Current Status of Research Progress

1: Research has progressed more than it was originally planned.

Reason

We earned the high-priority muSR beamtime at TRIUMF Canada from the proposal submission in June 2021 and January 2022.

Strategy for Future Research Activity

2022: We will perform Zero-field and Transverse-field muSR experiment on k-(ET)4Hg2.89Br8 and k-(ET)4Hg2.78Cl8 using dilution refrigerator at TRIUMF Canada.

2023: We will perform Zero-field and Laongitudinal-field muSR experiment on k-(ET)4Hg2.89Br8 and k-(ET)4Hg2.78Cl8 at ISIS and JPARC, and finalize the analysis process.

2024: Writing up the papers.

Causes of Carryover

none

  • Research Products

    (3 results)

All 2022 2021

All Presentation (3 results) (of which Int'l Joint Research: 3 results)

  • [Presentation] μ+SR Study of κ-(ET)4Hg3-δBr8 (δ=0.11) and κ-(ET)4Hg3-δCl8 (δ=0.22)2022

    • Author(s)
      Dita P. Sari, Y. Cai, M-V. deToro Sanchez, K. M. Kojima, I. Watanabe, A. Koda, Y. Ishii, H. Taniguchi
    • Organizer
      The 2022Annual 77th Japanese Physical Society Meeting
    • Int'l Joint Research
  • [Presentation] Distorted Superconducting Nodal Line on Single Fermi Surface in Anisotropic Organic Superconductor λ-(BETS)2GaCl42021

    • Author(s)
      D. P. Sari, R. Asih, K. Hiraki, T. Nakano, Y. Nozue, A. D. Hillier, Y. Ishii, I. Watanabe
    • Organizer
      International Conference on Strongly Correlated Electron Systems 2020
    • Int'l Joint Research
  • [Presentation] μ+SR Study of an Organic Doped Spin-Liquid Candidate κ-(ET)4Hg3-δBr8 (δ=0.11)2021

    • Author(s)
      Dita P. Sari, Y. Cai, M-V. deToro Sanchez, K. M. Kojima, I. Watanabe, Y. Ishii, H. Taniguchi
    • Organizer
      Materials Research Meeting 2021
    • Int'l Joint Research

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Published: 2022-12-28  

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