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2012 Fiscal Year Final Research Report

Interfacial Engineering of Semiconductor Nanocrystals and their Carrier Dynamics by Microspectroscopy

Research Project

  • PDF
Project/Area Number 22350012
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionKwansei Gakuin University

Principal Investigator

TAMAI Naoto  関西学院大学, 理工学部, 教授 (60163664)

Co-Investigator(Kenkyū-buntansha) OGASAWARA Kazuyoshi  関西学院大学, 理工学部, 教授 (10283631)
Project Period (FY) 2010 – 2012
Keywords電子状態
Research Abstract

II-VI semiconductor nanocrystals (CdS,CdSe,CdTe,PbS) were prepared by colloidal synthetic methods and their interfacial properties were controlled by interfacial engineering using various capping reagents, shells, and metal nanoparticles. Carrier dynamics of these nanocrystals were examined by femtosecond transient absorption, time-resolved emission, and single particle spectroscopy. Effects of interfacial structures and phonons on single exciton dynamics and Auger recombination due to the interaction of multiple excitons were analyzed together with the temperature dependence on carrier dynamics.

  • Research Products

    (42 results)

All 2013 2012 2011 2010 Other

All Journal Article (22 results) (of which Peer Reviewed: 18 results) Presentation (19 results) Remarks (1 results)

  • [Journal Article] Ultrafast Dynamics and Single Particle Spectroscopy of Au-CdSe Nanorods2013

    • Author(s)
      G. Sagarzazu, K. Inoue, M. Saruyama, M.Sakamoto, T. Teranishi, S. Masuo and N.Tamai
    • Journal Title

      Phys.Chem. Chem. Phys.

      Volume: 15 Pages: 2141-2152

    • Peer Reviewed
  • [Journal Article] Natural Photosynthetic Carotenoids for Solution-Processed Organic Bulk- Hetero- junction Solar Cells2013

    • Author(s)
      X-F. Wang, L. Wang, Z.Wang, Y. Wang, N.Tamai, Z. Hong, and J. Kido
    • Journal Title

      J. Phys. Chem. C

      Volume: 117 Pages: 804-811

    • Peer Reviewed
  • [Journal Article] 半導体量子ドットにおけるオージェ再結合の界面効果と温度効果2012

    • Author(s)
      小林洋一,玉井尚登
    • Journal Title

      表面

      Volume: 49 Pages: 397-406

  • [Journal Article] Effect of Dipole Coupling on Near-IR LSPR and Coherent Phonon Vibration of Periodic Gold Pair Nanocuboids2012

    • Author(s)
      L. Wang, Y. Nishijima, K. Ueno, H. Misawa, and N. Tamai
    • Journal Title

      J. Phys. Chem. C

      Volume: 116 Pages: 17838-17846

    • Peer Reviewed
  • [Journal Article] Dual Transient Bleaching of Au/PbS Hybrid Core/Shell Nanoparticles2012

    • Author(s)
      Y. Kobayashi, Y. Nonoguchi, L. Wang, T.Kawai, and N. Tamai
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 3 Pages: 1111-1116

    • Peer Reviewed
  • [Journal Article] Photofabrication of Fullerene-Shelled Quantum Dots Supra- molecular Nanoparticles for Solar Energy Harvesting2012

    • Author(s)
      E. S. Shibu, A. Sonoda, Z. Tao, Q. Feng, A.Furube, S. Masuo, L. Wang, N. Tamai, M. Ishikawa, and V. Biju
    • Journal Title

      ACS Nano

      Volume: 6 Pages: 1601-1608

    • Peer Reviewed
  • [Journal Article] First-principles calculation of ZnS nanocluster and bulk2012

    • Author(s)
      T. Gunshi, S. Watanabe, and K. Ogasawara
    • Journal Title

      Bull. of the Society for Descrete Variational Xα

      Volume: 25 Pages: 124-127

  • [Journal Article] Suppressed Blinking Behavior of Thioglycolic Acid Capped CdTe Quantum Dot by Amine Functionalization2011

    • Author(s)
      A. Mandal and N. Tamai
    • Journal Title

      Appl. Phys. Lett.

      Volume: 99 Pages: 263111-1-263111-4

    • Peer Reviewed
  • [Journal Article] External Electric Field Effects on State Energy and Photoexcitation Dynamics of Water-Soluble CdTe Nanoparticles2011

    • Author(s)
      R. Ohshima, T. Nakabayashi, Y. Kobayashi, N. Tamai, and N. Ohta
    • Journal Title

      J. Phys. Chem. C

      Volume: 115 Pages: 15274-15281

    • Peer Reviewed
  • [Journal Article] Development of Solar Cells Based on Synthetic Near-Infrared Absorbing Purpurins: Observation of Multiple Electron Injection Pathways at Cyclic Tetrapyrrole - Semiconductor Interface2011

    • Author(s)
      X.-F. Wang, L. Wang, N. Tamai, O. Kitao, H. Tamiaki, and S. Sasaki
    • Journal Title

      J. Phys. Chem. C

      Volume: 115 Pages: 24394-24402

    • Peer Reviewed
  • [Journal Article] Hyperbranched CdTe Nanostructures via a Self-Assembly Route: Optical Properties2011

    • Author(s)
      L. Pan, G. Pan, X. Che, L. Wang, N. Tamai, and Z. Dai
    • Journal Title

      Appl. Opt.

      Volume: 50 Pages: G31-G36

    • Peer Reviewed
  • [Journal Article] Plasmon Coupling and Coherent Acoustic Phonon Dynamics of Periodic Gold Pair Nanocuboids by Near-IR Transient Absorption Spectroscopy2011

    • Author(s)
      L. Wang, Y. Nishijima, K. Ueno, H. Misawa, and N. Tamai
    • Journal Title

      J. Photochem. Photobiol. A: Chem.

      Volume: 221 Pages: 164-168

    • Peer Reviewed
  • [Journal Article] 半導体量子ドットのオージェ再結合ダイナミクス2011

    • Author(s)
      小林洋一,玉井尚登
    • Journal Title

      光化学

      Volume: 42 Pages: 20-23

  • [Journal Article] Effect of Surface Defects on Auger Recombination in Colloidal CdS Quantum Dots2011

    • Author(s)
      Y. Kobayashi, T. Nishimura, H. Yamaguchi, and N. Tamai
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 2 Pages: 1051-1055

    • Peer Reviewed
  • [Journal Article] Luminescence Enhancement of Water Soluble CdTe Quantum Dots by Proper Surface Modification with Ethylene Diamine2011

    • Author(s)
      A. Mandal and N. Tamai
    • Journal Title

      Chem.Phys. Lett.

      Volume: 507 Pages: 248-252

    • Peer Reviewed
  • [Journal Article] Ultrafast Spectroscopy and Coherent Acoustic Phonon of Au-Ag Core-Shell Nanorods2011

    • Author(s)
      L. Wang, A. Kiya, Y. Okuno, Y. Niidome, and N. Tamai
    • Journal Title

      J. Chem. Phys.

      Volume: 134 Pages: 054501-1-054501-6

    • Peer Reviewed
  • [Journal Article] Auger Recombination Dynamics in Hybrid Silica-Coated CdTe Nanocrystals2011

    • Author(s)
      G. Sagarzazu, Y. Kobayashi, N. Murase Y.Ping and N. Tamai
    • Journal Title

      Phys. Chem. Chem. Phys.

      Volume: 13 Pages: 3227-3230

    • Peer Reviewed
  • [Journal Article] Electronic structure analysis of CdS surface by first-principles calculations2011

    • Author(s)
      S. Yamaji, K. Yokono, K. Higashiura, and K.Ogasawara
    • Journal Title

      Bull. of the Society for Descrete Variational Xα

      Volume: 24 Pages: 209-213

    • Peer Reviewed
  • [Journal Article] The analysis of the energy levels of CdTe bulk and surface by first-principles calculations2011

    • Author(s)
      K. Yokono, S. Yamaji, K. Higashiura, and K.Ogasawara
    • Journal Title

      Bull. of the Society for Descrete Variational Xα

      Volume: 24 Pages: 124-127

  • [Journal Article] Size-Dependent Multiexciton Spectroscopy and Moderate Temperature Dependence of Biexciton Auger Recombination in Colloidal CdTe Quantum Dots2010

    • Author(s)
      Y. Kobayashi and N. Tamai
    • Journal Title

      J. Phys. Chem. C

      Volume: 114 Pages: 17550-17556

    • Peer Reviewed
  • [Journal Article] Chlorophyll-a Derivatives with Various Hydrocarbon Ester Groups for Efficient Dye-Sensitized Solar Cells: Static and Ultrafast Evaluations on Electron Injection and Charge Collection Processes2010

    • Author(s)
      X.-F. Wang, H. Tamiaki, L. Wang, N. Tamai, O. Kitao, H. Zhou and S. Sasaki
    • Journal Title

      Langmuir

      Volume: 26 Pages: 6320-6327

    • Peer Reviewed
  • [Journal Article] Ultrafast Carrier Dynamics of Titanic Acid Nanotubes Investigated by Transient Absorption Spectroscopy2010

    • Author(s)
      L. Wang, H. Zhao, L. Pan, Y.-X. Weng, Y.Nakato, and N. Tamai
    • Journal Title

      J. Nanosci. Nanotech.

      Volume: 10 Pages: 8349-8355

    • Peer Reviewed
  • [Presentation] HotElectron Transfer in Au-CdSe Nanorods2012

    • Author(s)
      G. Sagarzazu, K. Inoue, M. Saruyama, M.Sakamoto, T. Teranishi, N. Tamai
    • Organizer
      7th Asian Photochemistry Conference 2012 (Icho Kaikan
    • Place of Presentation
      Osaka University
    • Year and Date
      20121112-15
  • [Presentation] Energy Transfer Dynamics of CdTe Quantum Dots on Epitaxial Graphene prepared by Si sublimation of 4H-SiC(0001)2012

    • Author(s)
      T. Hirose, H. Shigemasa, Y. Kutsuma, T.Kaneko and N. Tamai
    • Organizer
      7th Asian Photochemistry Conference 2012 (Icho Kaikan
    • Place of Presentation
      Osaka, University
    • Year and Date
      20121112-15
  • [Presentation] Hot Carrier and Coherent Phonon Dynamics of CdTe/Au Hybrid Nanostructures2012

    • Author(s)
      T. Okuhata, Y. Kobayashi, Y. Nonoguchi, T.Kawai, and N. Tamai
    • Organizer
      7th Asian Photochemistry Conference 2012 (Icho Kaikan
    • Place of Presentation
      Osaka University
    • Year and Date
      20121112-15
  • [Presentation] Luminescence Properties and Auger Recombination of Cu-doped CdSe Nanocrystals2012

    • Author(s)
      M. Ozaki, M. Tsuboi, and N. Tamai
    • Organizer
      7th Asian Photochemistry Conference 2012
    • Place of Presentation
      Icho Kaikan, Osaka University
    • Year and Date
      20121112-15
  • [Presentation] Carrier Relaxation and Luminescence Properties of Semiconductor Nanoparticles and Their Applications2012

    • Author(s)
      N. Tamai
    • Organizer
      FluoroFest Workshop
    • Place of Presentation
      Kyoto, Japan
    • Year and Date
      20121108-09
  • [Presentation] Elementary Processes of Photoexcited Semiconductor Nanoparticles2012

    • Author(s)
      L. Wang, S. Gabriel, T. Okuhata, Y.Kobayashi, and N. Tamai
    • Organizer
      Japan-India Bilateral Symposium on Supramolecular Nanomaterials for Energy Innovation
    • Place of Presentation
      Alpha Anabuki Hall, Takamatsu, Japan
    • Year and Date
      20121015-16
  • [Presentation] Preparation and Evaluation of CdSe Quantum Dots Direct-coated with TiO2 for Energy Conversion2012

    • Author(s)
      T. Hirai, C. L. Li, M. Ando, N. Murase, and N.Ta mai
    • Organizer
      Japan-India Bilateral Symposium on Supramolecular Nanomaterials for Energy Innovation
    • Place of Presentation
      Alpha Anabuki Hall, Takamatsu, Japan
    • Year and Date
      20121015-16
  • [Presentation] Elementary Processes of Photoexcited Nanoparticles: Plasmonic Systems and Semiconductor Quantum Dots2012

    • Author(s)
      N. Tamai
    • Organizer
      The International Workshop on Single Molecule/Nanoparticle Spectroscopy
    • Place of Presentation
      National Chiao Tung Univ., Taiwan
    • Year and Date
      20120627-28
  • [Presentation] Synthesis and Carrier Dynamics of CdTe/Au Hybrid Nanostructures2012

    • Author(s)
      T. Okuhata, Y. Kobayashi, Y. Nonoguchi, T.Kawai, N. Tamai
    • Organizer
      Yamada Conference LXVI, International Conference on theNanostructure-Enhanced Photo-EnergyConversion
    • Place of Presentation
      Miraikan
    • Year and Date
      20120603-06
  • [Presentation] Auger Recombination and Multiexciton States of II-VI Semiconductor Quantum Dots2012

    • Author(s)
      Y. Kobayashi, Y. Matsumoto, Y. Tian, L.Wang and N. Tamai
    • Organizer
      7th International Conference on Quantum Dots (QD 2012)
    • Place of Presentation
      Santafe Convention Center, Santafe, New Mexico, USA
    • Year and Date
      20120513-18
  • [Presentation] Ultrafast Electron Transfer in Au-CdSe Nanorods2012

    • Author(s)
      G. Sagarzazu, M. Saruyama, K. Inoue, T.Teranishi, S. Masuo and N. Tamai
    • Organizer
      7th International Conference on Quantum Dots (QD 2012)
    • Place of Presentation
      Santafe Convention Center,Santafe, New Mexico, USA
    • Year and Date
      20120513-18
  • [Presentation] Carrier Dynamics of Au-CdSe Colloidal Nanorods2011

    • Author(s)
      G. Sagaruzazu, M. Saruyama, T. Teranishi, and N. Tamai
    • Organizer
      XXV International Conference on Photochemistry
    • Place of Presentation
      Beijing, China
    • Year and Date
      20110807-12
  • [Presentation] Influence of Dipole Coupling on Periodic Gold Pair Nanocuboids by Near-IR Transient Absorption Spectroscopy2011

    • Author(s)
      L. Wang, Y. Nishijima, K. Ueno, H. Misawa, and N. Tamai
    • Organizer
      XXV International Conference on Photochemistry
    • Place of Presentation
      Beijing, China
    • Year and Date
      20110807-12
  • [Presentation] Effect of Surface Defects on Size-dependent Auger Recombination in CdS Quantum Dots2011

    • Author(s)
      Y. Kobayashi, T. Nishimura, H. Yamaguchi, and N. Tamai
    • Organizer
      XXV International Conference on Photochemistry
    • Place of Presentation
      Beijing, China
    • Year and Date
      20110807-12
  • [Presentation] Effect of Plasmon Coupling on Near-IR Vibrational Dynamics of Periodic Gold Nanocuboids2010

    • Author(s)
      L. Wang, Y. Nishijima, K. Ueno, H. Misawa, and N. Tamai
    • Organizer
      Pacifichem 2010
    • Place of Presentation
      Honolulu, Hawaii
    • Year and Date
      20101215-20
  • [Presentation] Multiexciton Spectroscopy and Temperature Dependence of Auger Recombination in CdTe Quantum Dots2010

    • Author(s)
      N. Tamai and Y. Kobayashi (Invited)
    • Organizer
      The 7th Korea-Japan Symposium on Frontier Photoscience 2010
    • Place of Presentation
      Daegu, Korea
    • Year and Date
      20101023-26
  • [Presentation] Coherent Phonon Vibration of Gold Nanostractures and Its Control by Two Excitation Pulses2010

    • Author(s)
      N. Tamai, L. Wang, Y. Nishijima, K. Ueno, H. Misawa, A. Kiya, Y. Okuno, Y. Niidome
    • Organizer
      XXIIIth IUPAC Symposium on Photochemistry
    • Place of Presentation
      Ferrara, Italy
    • Year and Date
      20100711-16
  • [Presentation] Effects of Temperature on Biexciton Auger Recombination of Cadmium Telluride Quantum Dots2010

    • Author(s)
      Y. Kobayashi, N. Tamai
    • Organizer
      XXIIIth IUPAC Symposiumon Photochemistry
    • Place of Presentation
      Ferrara, Italy
    • Year and Date
      20100711-16
  • [Presentation] Single-Particle Spectroscopy and Energy Transfer Dynamics of CdTe Quantum Dots Bound to DNA2010

    • Author(s)
      S. Kudo and N. Tamai
    • Organizer
      XXIIIth IUPAC Symposium on Photochemistry
    • Place of Presentation
      Ferrara, Italy
    • Year and Date
      20100711-16
  • [Remarks]

    • URL

      http://sci-tech.ksc.kwansei.ac.jp/~tamai/Top.htm

URL: 

Published: 2014-08-29  

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