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2012 Fiscal Year Final Research Report

Design of soluble semiconductors and study on their device functionality

Research Project

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Project/Area Number 22350055
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Functional materials chemistry
Research InstitutionHokkaido University

Principal Investigator

INABE Tamotsu  北海道大学, 大学院・理学研究院, 教授 (20168412)

Co-Investigator(Renkei-kenkyūsha) TAKAHASHI Yukihiro  北海道大学, 大学院・理学研究院, 助教 (40443197)
HARADA Jun  北海道大学, 大学院・理学研究院, 准教授 (00313172)
Project Period (FY) 2010 – 2012
Keywords可溶性半導体 / ドーピング / ヨウ化スズ / 有機無機複合ペロブスカイト / 半導体 素子
Research Abstract

Systematic investigation of the electronic structure, doping level, transport properties of the solution processable organic-inorganic hybrid perovskites was performed. Design of the novel doping method and device construction including organic semiconductors was also examined. As for the tin-iodide system, the origin of the high conductivity was clarified by this study. As for the organic semiconductors, novel concept of doping at the contact interface was proposed, and the electronic state at the interface was studied.

  • Research Products

    (26 results)

All 2013 2012 2011 2010

All Journal Article (8 results) (of which Peer Reviewed: 8 results) Presentation (18 results)

  • [Journal Article] Electrochemical Crystallization of Organic Molecular Conductors:Electrode Surface Conditions for Crystal Growth2013

    • Author(s)
      T. Miyahira, H. Hasegawa, Y. Takahashi, T. Inabe
    • Journal Title

      Cryst. Growth Des

      Volume: (in press)

    • DOI

      DOI:10.1021/cg301852k

    • Peer Reviewed
  • [Journal Article] The bis(ethylenedithio)tetrathia- fulvalene based ionic charge-transfer complex with 2,3-dichloro-5,6-dicyano-p-benzo-quinone2013

    • Author(s)
      Y. Nakagawa, Y. Takahashi, J. Harada, T.Inabe
    • Journal Title

      Acta Crystallogr. Sect. C

      Volume: 69 Pages: 400-402

    • DOI

      DOI:10.1107/S0108270113003685

    • Peer Reviewed
  • [Journal Article] Molecular Photo-conductor with Simultaneously Photo-controllable Localized Spins2012

    • Author(s)
      T. Naito, T. Karasudani, S. Mori, K. Ohara, K.Konishi, T. Takano, Y. Takahashi, T. Inabe, S. Nishihara, K. Inoue
    • Journal Title

      J. Am. Chem. Soc

      Volume: 134 Pages: 18656-18666

    • DOI

      DOI:10.1021/ja306260b

    • Peer Reviewed
  • [Journal Article] Simultaneous Control of Carriers and Localized Spins with Light in Organic Materials2012

    • Author(s)
      T. Naito, T. Karasudani, K. Ohara,T. Takano, Y. Takahashi, T. Inabe, K. Furukawa, T. Nakamura
    • Journal Title

      Adv. Mater

      Volume: 24 Pages: 6153-6157

    • DOI

      DOI:10.1002/adma.201203153

    • Peer Reviewed
  • [Journal Article] Carrier doping to the organic Mott insulator by conjugating with tetrathiafulvalene2012

    • Author(s)
      Y. Takahashi, Y. Nakagawa, K. Hayakawa, T.Inabe, T. Naito
    • Journal Title

      Appl. Phys. Lett

      Volume: 101 Pages: 103303(1-4)

    • DOI

      DOI:10.1063/1.4750066

    • Peer Reviewed
  • [Journal Article] What Happens at the Interface between TTF and TCNQ Crystals (TTF=Tetrathiafulvalene and TCNQ =7,7,8,8-Tetracyanoquinodimethane)?2012

    • Author(s)
      Y. Takahashi, K. Hayakawa, T. Naito, T.Inabe
    • Journal Title

      J. Phys. Chem. C

      Volume: 116 Pages: 700-703

    • DOI

      DOI:10.1021/jp2074368

    • Peer Reviewed
  • [Journal Article] Charge-Transport in Tin-Iodide Perovskite CH3NH3SnI3: Origin of High Conductivity2011

    • Author(s)
      Y. Takahashi, R. Obara, Z. Lin, Y. Takahashi, T. Naito, T. Inabe, S. Ishibashi, K. Terakura
    • Journal Title

      Dalton Trans

      Volume: 40 Pages: 5563-5568

    • DOI

      DOI:10.1039/c0dt01601b

    • Peer Reviewed
  • [Journal Article] Growth of Nanocrystals in a Single Crystal of Different Materials: A Way of Giving Function to Molecular Crystals2011

    • Author(s)
      T. Naito, A. Kakizaki, T. Inabe, R. Sakai, E.Nishibori, H. Sawa
    • Journal Title

      Cryst. Growth Des

      Volume: 11 Pages: 501-506

    • DOI

      DOI:10.1021/cg101295p

    • Peer Reviewed
  • [Presentation] 有機・無機ハイブリッド半導体の物性とデバイス化2013

    • Author(s)
      長谷川裕之,大崎剛,工藤勇,ロレーナジーヤンカルロ,高橋幸裕,原田潤,稲辺保
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      立命館大学びわこ・くさつキャンパス(草津市)
    • Year and Date
      20130322-0325
  • [Presentation] 有機・無機ハイブリッド層状ペロブスカイト化合物A_2MX_4(M=Pb,CuandX=Cl,Br,I)の構造と物性2013

    • Author(s)
      ロレーナジーヤンカルロ,高橋幸裕,長谷川裕之,原田潤,稲辺保
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      立命館大学びわこ・くさつキャンパス(草津市)
    • Year and Date
      20130322-0325
  • [Presentation] Crystal Structure and Properties of Organic-Inorganic Hybrid Perovskites based on A_2MX_4 (where A=Organicammonium, M=Pb, CuandX=Cl, Br, I)2012

    • Author(s)
      G. S. Lorena、T. Osaki、Y. Kudo, H.Hasegawa、Y. Takahashi、J. Harada、T. Inabe
    • Organizer
      ElecMol'12
    • Place of Presentation
      MINATEC HOUSE in Grenoble (France)
    • Year and Date
      20121203-1207
  • [Presentation] The metallic transport properties at contact the interface of donor and acceptor molecular crystals2012

    • Author(s)
      Y. Takahashi、Y. Nakagawa、K. Takayama、 J. Harada、T. Inabe
    • Organizer
      ElecMol'12
    • Place of Presentation
      MINATEC HOUSE inGrenoble (France)
    • Year and Date
      20121203-1207
  • [Presentation] Charge Transport at theCrystal-to-Crystal Interface2012

    • Author(s)
      T. Inabe、Y. Takahashi、H. Hasegawa、J.Harada
    • Organizer
      MDF2012
    • Place of Presentation
      宮崎国際会議場(宮崎市)
    • Year and Date
      20121201-1204
  • [Presentation] (Pb,Sn)-I系層状ペロブスカイト型化合物の構造と電子機能2012

    • Author(s)
      工藤勇、大崎剛、ロレーナジーヤンカルロ、長谷川裕之、高橋幸裕、原田潤、稲辺保
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京大学本郷キャンパス(東京都)
    • Year and Date
      20120918-0921
  • [Presentation] ハロゲン化スズペロブスカイト化合物の電子物性2012

    • Author(s)
      長谷川裕之、大崎剛、工藤勇、ロレーナジーヤンカルロ、高橋幸裕、原田潤、稲辺保
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京大学本郷キャンパス(東京都)
    • Year and Date
      20120918-0921
  • [Presentation] 分子結晶接触界面へのキャリヤ注入2012

    • Author(s)
      高橋幸裕、横倉聖也、中川裕貴、三笠仁裕、長谷川裕之、原田潤、稲辺保
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京大学本郷キャンパス(東京都)
    • Year and Date
      20120918-0921
  • [Presentation] Sn-I系ペロブスカイト型化合物へのドーピングによる導電性制御の試み2012

    • Author(s)
      高橋由香利,長谷川裕之,高橋幸裕,稲辺保
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      慶応義塾大学日吉キャンパス(横浜市)
    • Year and Date
      20120325-0328
  • [Presentation] 臭化スズ系有機・無機ハイブリッド半導体へのドーピング効果2012

    • Author(s)
      長谷川裕之,大崎剛,工藤勇,高橋由香利,高橋幸裕,稲辺保
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      慶応義塾大学吉キャンパス(横浜市)
    • Year and Date
      20120325-0328
  • [Presentation] (Pb,Sn)-I系層状ペロブスカイト型化合物の電子機能開拓2012

    • Author(s)
      工藤勇,高橋由香利,高橋幸裕,長谷川裕之,稲辺保
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      慶応義塾大学日吉キャンパス(横浜市)
    • Year and Date
      20120325-0328
  • [Presentation] 有機ジカチオンを用いた有機・無機複合Sn-I系層状ペロブスカイト型化合物へのカチオン欠損による導電性制御の試み2011

    • Author(s)
      高橋由香利,長谷川裕之,高橋幸裕,稲辺保
    • Organizer
      第5回分子科学討論会
    • Place of Presentation
      札幌コンベンションセンター(札幌市)
    • Year and Date
      20110920-0923
  • [Presentation] 臭化スズ系有機・無機ハイブリッド半導体の構造と物性2011

    • Author(s)
      長谷川裕之,工藤勇,高橋由香利,高橋幸裕,稲辺保
    • Organizer
      第5回分子科学討論会
    • Place of Presentation
      札幌コンベンションセンター(札幌市)
    • Year and Date
      20110920-0923
  • [Presentation] Physical and FET Properties of Alloyed Organic-Inorganic Hybrids2011

    • Author(s)
      Y. Kudo, Y. Takahashi, Y. Takahashi, T. Inabe, T. Naito
    • Organizer
      ECME2011
    • Place of Presentation
      Auditorio Axa in Barcelona (Spain)
    • Year and Date
      20110707-0710
  • [Presentation] Hole Doping in Soluble Organic-Inorganic Hybrid Perovskites using organic dications2011

    • Author(s)
      Y. Tkahashi, Y. Tkahashi, T. Inabe, T. Naito
    • Organizer
      ECME2011
    • Place of Presentation
      Auditorio Axa in Barcelona (Spain)
    • Year and Date
      20110707-0710
  • [Presentation] Inabe, Hole doping in soluble organic-inorganic hybrid perovskites2010

    • Author(s)
      Y. Takahashi, Z-Z Lin, Y. Takahashi, T. Naito, T
    • Organizer
      PACIFICHEM2010
    • Place of Presentation
      HAWAII CONVENTION CENTER (U.S.A.)
    • Year and Date
      20101215-1220
  • [Presentation] Sn-I系ペロブスカイト型化合物へのドーピングの試み2010

    • Author(s)
      高橋由香利,Lin Zheng-Zhong,高橋幸裕,内藤俊雄,稲辺保
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪大学豊中キャンパス(大阪市)
    • Year and Date
      20100914-0917
  • [Presentation] Hole Doping in Soluble Organic-Inorganic Hybrid Semiconductors Using Organic Dications2010

    • Author(s)
      Y. Takahashi, Y. Takahashi, T. Inabe
    • Organizer
      ICSM 2010
    • Place of Presentation
      Kyoto International Conference Center (Kyoto)
    • Year and Date
      20100704-0709

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Published: 2014-08-29  

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