Research of magnetism using the magnetic light scattering from spin multiplets

2013 Fiscal Year Final Research Report

• Project/Area Number: 22540350
• Research Category: Grant-in-Aid for Scientific Research (C)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Condensed matter physics II
• Research Institution: Sophia University
• Principal Investigator: KUROE Haruhiko 上智大学, 理工学部, 准教授 (40296885)
• Co-Investigator(Renkei-kenkyūsha): SEKINE Tomoyuki 上智大学, 理工学部, 名誉教授 (60110722) ; TANAKA Hidekazu 東京工業大学, 理学部, 教授 (80188325) ; MATSUMOTO Masashige 静岡大学, 理学部, 准教授 (20281058) ; MASUDA Takatsugu 東京大学, 物性研究所, 准教授 (90313014) ; TAKEMURA Kenichi 物質材料研究機構, ナノ物質ラボ, 主席研究員 (20171671) ; HASE Masashi 物質材料研究機構, 量子ビームセンター, 主席研究員
• Project Period (FY): 2010-04-01 – 2013-03-31
• Keywords: 磁気Raman 散乱 / 磁気励起 / Anderson-Higgs モード / Nambu-Goldstone モード / スピン・ギャップ / 多重極限環境 / マルチフェロイック物質

Research Abstract

We studied the magnetism on the spin-dimer system and the distorted-tetrahedral spin system by using the magnetic Raman scattering. For the spin-dimer system, from the points of view of theory and experiment, we clarified the first-order Anderson-Higgs mode in the antiferromagnetic phase induced by magnetic fields and high pressures. We have not observed the magnetic Raman scattering in a single crystal with the distorted tetrahedral spin chain.

Research Products

• [Journal Article] Thermal, Dielctric, and Magnetic Properties in Multiferroic Cu_<2.85>Zn_<0.15>Mo_2O_9 (2014)
  • Author(s): H. Kuroe, K. Aoki, R. Itoh, T. Hosaka, T. Hasegawa, S. Hachiuma, M. Akaki, H. Kuwahara, T. Sekine, M. Hase, K. Oka, T. Ito, and H. Eisaki
  • Journal Title: J. Kor. Phys. Soc. Volume: 63 Pages: 542-545
  • Peer Reviewed
• [Journal Article] Muon Spin Spectroscopy in Multiferroic (Cu,Zn)_3Mo_2O_9 (2014)
  • Author(s): H. Kuroe, K. Aoki, T. Sato, R. Kino, H. Kuwahara, T. Sekine, M. Hase, I. Kawasaki, T. Kawamata, T. Suzuki, I. Watanabe, K. Oka, T. Ito, and H. Eisaki
  • Journal Title: J. Conf Proc. Volume: 2, 010206 Pages: 8
  • Peer Reviewed
• [Journal Article] Longitudinal magnetic excitation in KCuCl_3 studied by Raman scattering under hydrostatic pressures (2012)
  • Author(s): H. Kuroe, N. Takami, N. Niwa, T. Sekine, M. Matsumoto, F. Yamada, H. Tanaka and K. Takemura
  • Journal Title: J. Phys. Conf. Ser. Volume: 400 Pages: 032042
  • Peer Reviewed
• [Journal Article] NMR study on field-induced charge anomaly in Cu_3Mo_2O_9 (2012)
  • Author(s): K Misoka, H Kuroe, K Doi, T Hamasaki, T Sekine, T Goto, M Hase, K Oka, T Ito, H Eisaki and T Sasaki
  • Journal Title: J. Phys.: Conf. Ser. Volume: 400 Pages: 032056
  • Peer Reviewed
• [Journal Article] Magnetic Excitation and Electric Polarization in Strongly Coupled Spin Monomer and Dimer System Cu_3Mo_2O_9 (2012)
  • Author(s): M. Matsumoto, H. Kuroe, T. Sekine, and M. Hase
  • Journal Title: J. Phys. Soc. Jpn. Volume: 81 Pages: 024711
  • Peer Reviewed
• [Journal Article] Hybridization of magnetic excitations between quasi-one-dimensional spin chains and spin dimers in Cu_3Mo_2O_9 observed using inelastic neutron scattering (2011)
  • Author(s): H. Kuroe, T. Hamasaki, T. Sekine, M. Hase, K. Oka, T. Ito, H. Eisaki, K. Kaneko, N. Metoki, M. Matsuda, and K. Kakurai
  • Journal Title: Phys. Rev. B Volume: 83 Pages: 184423
  • Peer Reviewed
• [Journal Article] Electric Polarization Induced by Néel Order without Magnetic Superlattice : Experimental Study of Cu_3Mo_2O_9 and Numerical Study of a Small Spin Cluster (2011)
  • Author(s): H. Kuroe, T. Hosaka, S, Hachiuma, T. Sekine, M. Hase, K. Oka, T. Ito, H. Eisaki, M. Fujisawa, S. Okubo, and H. Ohta,"" 80 (2011) 083705. (査読あり)
  • Journal Title: J. Phys. Soc. Jpn. Volume: 80 Pages: 083705
  • Peer Reviewed
• [Journal Article] Crystal growth of Cu_<3−>xZn_xMo_2O_9 by continuous solid-state crystallization method (2011)
  • Author(s): K. Oka, T. Ito, H. Eisaki, M. Hase, T. Hamasaki, H. Kuroe and T. Sekine
  • Journal Title: J. Cryst. Growth Volume: 334[1] Pages: 108-112
  • Peer Reviewed
• [Journal Article] Transverse and Longitudinal Excitation Modes in Interacting Multispin Systems (2010)
  • Author(s): M. Matsumoto, H. Kuroe, T. Sekine, and T. Masuda
  • Journal Title: J. Phys. Soc. Jpn. Volume: 79 Pages: 084703
  • Peer Reviewed
• [Journal Article] Theory of magnetic excitation for coupled spin dimer and spin chain system Cu_2Fe_2Ge_4O_<13> (2010)
  • Author(s): M. Matsumoto, H. Kuroe, T. Sekine, and T. Masuda
  • Journal Title: J. Phys.: Conf. Ser. Volume: 200 Pages: 022034
  • Peer Reviewed
• [Journal Article] Triplon-spinon hybridization in Cu_3Mo_2O_9 observed using inelastic neutron scattering (2010)
  • Author(s): H. Kuroe, T. Hamasaki, T. Sekine, M. Hase, K. Oka, T. Ito, H. Eisaki and M. Matsuda
  • Journal Title: J. Phys.: Conf. Ser. Volume: 200 Pages: 022028
  • Peer Reviewed
• [Journal Article] Effects of magnetic field and pressure on the antiferromagnetic and weak-ferromagnetic orders in tetrahedral spin chain system Cu_3Mo_2O_9 (2010)
  • Author(s): T. Hamasaki, H. Kuroe, T. Sekine, M. Akaki, H. Kuwahara and M. Hase
  • Journal Title: J. Phys.: Conf. Ser. Volume: 200 Pages: 022013
  • Peer Reviewed
• [Journal Article] Cu-NMR study of the quasi-one-dimensional magnet Cu_3Mo_2O_9 (2010)
  • Author(s): K. Doi, T. Hamasaki, H. Kuroe, T. Sekine and T. Goto
  • Journal Title: J. Phys. Conf. Ser. Volume: 200 Pages: 022006
  • Peer Reviewed
• [Journal Article] Raman Scattering in (Cu,Zn)_3(Mo,W)_2O_9
  • Author(s): T. Sato, K. Aoki, R. Kino, H. Kuroe T. Sekine, M. Hase, K. Oka, T. Ito, and H. Eisaki
  • Journal Title: JPS Conf. Proc. as a part of Proceedings of SCES2013 Volume: (in press)
  • Peer Reviewed
• [Journal Article] Magnetic and Dielectric Properties in Multiferroic Cu_3Mo_2O_9 under High Magnetic Fields
  • Author(s): H. Kuroe, K. Aoki, R. Kino, T. Sato, H. Kuwahara, T. Sekine, T. Kihara, M. Akaki, Y. Kohama, M. Tokunaga, A. Matsuo, K. Kindo, M. Hase, K. Takehana, H. Kitazawa, K. Oka, T. Ito, and H. Eisaki
  • Journal Title: JPS Conf. Proc. as a part of Proceedings of SCES2013 Volume: (in press)
  • Peer Reviewed
• [Presentation] First-Order Magnetic Raman Scattering from Magnetic-Field-Induced Higgs Mode through Second-Order Magnetic Raman Process (2014)
  • Author(s): H. Kuroe and T. Sekine
  • Organizer: Hiigs Modes in Condensed Matter Physics and Quantum Gases
  • Place of Presentation: Kyoto
  • Year and Date: 20140623-25
• [Presentation] Muon spin relaxation/rotation in Cu_3Mo_2O_9 single crystals (2014)
  • Author(s): H. Kuroe, H. Kuwahara, T. Sekine, M. Hase, I. Kawasaki, T. Kawamata, T. Suzuki, I. Watanabe, K. Oka, T. Ito, and H. Eisaki
  • Organizer: μSR2014
  • Place of Presentation: Grendelwald Switzerland(ポスター掲示6/1-6/2014,発表6/5/2014)
  • Year and Date: 20140601-06
• [Presentation] Magnetic Properties in Multiferroic Cu_3Mo_2O_9 Detected by Particle Beams (2013)
  • Author(s): H. Kuroe, K. Aoki, T. Sato, R. Kino, T. Hamasaki, T. Sekine M. Hase, I. Kawasaki, T. Kawamata, T. Suzuki, I. Watanabe, M. Matsuda K. Kakurai, K. Oka, T. Ito, and H. Eisaki
  • Organizer: LPBMS2013
  • Place of Presentation: Tsukuba, Japan (発表日8/29,30/2013ポスター掲示期間8/29.30/2013 )
  • Year and Date: 20130829-31
• [Presentation] Muon spin spectroscopy in multiferroic (Cu,Zn)_3Mo_2O_9 (2013)
  • Author(s): H. Kuroe, K. Aoki, T. Sato, R, Kino, H. Kuwahara, T. Sekine, M. Hase, I. Kawasaki, T. Kawamata, T. Suzuki, I. Watanabe, K. Oka, T. Ito, and H. Eisaki
  • Organizer: USM2013
  • Place of Presentation: Matsue, Japan(発表日8/9-12/2013ポスター掲示期間8/9.11/2013 ) (ポスター賞受賞)
  • Year and Date: 20130809-12
• [Presentation] Effect of Magnetic Field on the Novel Ground State of C_u3Mo_2O_9 (2013)
  • Author(s): Y. Kohama, H. Kuroe, T. Sekine, M. Hase, K. Oka, T. Ito, H. Eisaki, M. Tokunaga, K. Kindo
  • Organizer: SCES2013
  • Place of Presentation: Tokyo, Japan
  • Year and Date: 20130805-09
• [Presentation] Raman Scattering in (Cu,Zn)_3Mo_2O_9 (2013)
  • Author(s): T. Sato, K. Aoki, R. Kino, H. Kuroe, T. Sekine, M. Hase, K. Oka, T. Ito, H. Eisaki
  • Organizer: SCES2013
  • Place of Presentation: Tokyo, Japan
  • Year and Date: 20130805-09
• [Presentation] Magnetic Properties in Multiferroic (Cu,Zn)_3Mo_2O_9 (2013)
  • Author(s): K. Aoki, R. Kino, T. Sato, H. Kuroe, T. Sekine, M. Hase, K. Oka, T. Ito, H. Eisaki
  • Organizer: SCES2013
  • Place of Presentation: Tokyo, Japan
  • Year and Date: 20130805-09
• [Presentation] Magnetic and Dielectric Properties in Multiferroic Cu_3Mo_2O_9 under High Magnetic Field (2013)
  • Author(s): H. Kuroe, K. Aoki, R. Kino, T. Sato, H. Kuwahara, T. Sekine, T. Kihara, M. Akaki, Y .Kohama, M Tokunaga, M. .Hase, K. Takehana, H. Kitazawa, K. Oka, T. Ito, H. Eisaki
  • Organizer: SCES2013
  • Place of Presentation: Tokyo, Japan
  • Year and Date: 20130805-09
• [Presentation] Cross-correlation effects in multiferroic Cu_3Mo_2O_9 (2012)
  • Author(s): R. Itoh, T. Hosaka, T. Hasegawa, H.. Kuroe, T. Sekine, M. Hase, K. Oka, T. Ito and H. Eisaki
  • Organizer: ICM2012
  • Place of Presentation: Busan, Korea
  • Year and Date: 20120708-13
• [Presentation] High field phase diagram in multiferroic Cu_3Mo_2O_9 (2012)
  • Author(s): H. Kuroe, R. Kino, R. Itoh, T. Hosaka, T. Hasegawa, T. Sekine, T. Kihara, M. Tokunaga, M. Hase, K. Takehana, H. Kitazawa, K. Oka, T. Ito and H. Eisaki
  • Organizer: ICM2012
  • Place of Presentation: Busan, Korea
  • Year and Date: 20120708-13
• [Presentation] Zn-substitution effects in multiferroic Cu_3Mo_2O_9 (2012)
  • Author(s): H. Kuroe, K. Aoki, R. Itoh, T. Hosaka, T. Hasegawa, S. Hachiuma, M. Akaki, H. Kuwahara, T. Sekine, M. Hase, K. Oka, T. Ito and H. Eisaki
  • Organizer: ICM2012
  • Place of Presentation: Busan, Korea
  • Year and Date: 20120708-13
• [Presentation] Magnetic and Electric Properties in the Distorted Tetrahedral Spin Chain System Cu_3MoO_9 (2011)
  • Author(s): T. Hosaka, S. Hachiuma, H. Kuroe, T. Sekine, M .Hase, K. Oka, T. Ito, H. Eisaki, M. Fuzisawa, S. Okubo and H. Ohta
  • Organizer: LT26
  • Place of Presentation: Beijing, Chaina
  • Year and Date: 20110810-17
• [Presentation] Longitudinal Magnetic Excitation in KCuCl_3 Studied by Raman Scattering under Hydrostatic Pressures (2011)
  • Author(s): H. Kuroe, N. Takami, M. Niwa, T. Sekine, Matsumoto, F. Yamada, H. Tanaka and K. Takemura
  • Organizer: LT26
  • Place of Presentation: Beijing, Chaina
  • Year and Date: 20110810-17
• [Presentation] Cu-NMR study on dimer-chain complex quantum spin system Cu_3Mo_2O_9 (2011)
  • Author(s): K. Misoka, K. Doi, T. Hamasaki, H. Kuroe, T. Goto, T. Sekine, T. Sasaki, M. Hase, K. Oka, T. Ito, and H. Eisaki
  • Organizer: LT26
  • Place of Presentation: Beijing, Chaina
  • Year and Date: 20110810-17
• [Remarks] 日本語による解説記事
• [Remarks] 黒江晴彦,関根智幸,長谷正司,"マルチフェロイック物質Cu3Mo2O9",固体物理47, 33 (2012).