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2011 Fiscal Year Final Research Report

Observation of phase-transition dynamics of amorphous oxide by Boson peak

Research Project

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Project/Area Number 22760505
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Inorganic materials/Physical properties
Research InstitutionTohoku University

Principal Investigator

TAKAHASHI Yoshihiro  東北大学, 工学研究科, 助教 (50442728)

Project Period (FY) 2010 – 2011
Keywords酸化物ガラス / 非弾性光散乱 / ボソンピーク / ラマン散乱 / 結晶化 / 分光測定
Research Abstract

In amorphous materials, an asymmetrical broad band is observed in a low-frequency region of inelastic light scattering spectra, the so-called"Boson peak". Since the Boson peak reflects the medium-range structure of the amorphous matter, it is expected that the Boson peak provides a significant insight about the glass. crystal transition state. Therefore, in this study, in-situ measurement of Boson peak in oxide glasses was performed during heating/crystallization for the purpose of understanding the structural inhomogeneity in oxide glass and its crystallization dynamics.

  • Research Products

    (19 results)

All 2012 2011 2010 Other

All Journal Article (12 results) (of which Peer Reviewed: 12 results) Presentation (4 results) Book (2 results) Remarks (1 results)

  • [Journal Article] Effect of annealing at maximum nucleation temperature on boson peak in lithium-disilicate glass2012

    • Author(s)
      中村健作, 高橋儀宏, 長田実, 井原梨恵, 藤原巧
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: Vol.120 Pages: 256-258

    • Peer Reviewed
  • [Journal Article] Nanocrystallization and optical property of willemite-type semiconductive Zn_2GeO_4 in glass2012

    • Author(s)
      高橋儀宏, 安藤正尊, 井原梨恵, 藤原巧, 長田実
    • Journal Title

      Functional Materials Letters

      Volume: Vol.5 Pages: 1260008-1-1260008-4

    • DOI

      DOI:10.1142/S1793604712600089

    • Peer Reviewed
  • [Journal Article] Soft-phonon mode observation in Li_2Ge_4O_9 phase above room temperature2012

    • Author(s)
      高橋儀宏, 国友潤, 中村健作, 長田実, 藤原巧
    • Journal Title

      Applied Physics Letters

      Volume: Vol.100 Pages: 091902-1-091902-3

    • DOI

      DOI:10.1063/1.3688603

    • Peer Reviewed
  • [Journal Article] High-energy shift of Boson peak and its broadening in crystallization regime : A qualitative aspect2011

    • Author(s)
      高橋儀宏, 長田実, 井原梨恵, 藤原巧
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: Vol.80 Pages: 095003-1-095003-2

    • DOI

      DOI:10.1143/JPSJ.80.095003

    • Peer Reviewed
  • [Journal Article] Low-frequency inelastic light scattering of zincogerrnanate glass in supercooledliquid regime2011

    • Author(s)
      高橋儀宏, 長田実, 安藤正尊, 井原梨恵, 藤原巧
    • Journal Title

      Journal of Applied Physics

      Volume: Vol.109 Pages: 126105-1-126105-3

    • DOI

      DOI:10.1063/1.3602085

    • Peer Reviewed
  • [Journal Article] In situ observation of supercooled liquid-crystal phase transition in glassy ferroelectric LaBGeO_52011

    • Author(s)
      高橋儀宏, 安岡知道, 長田実, 井原梨恵, 藤原巧
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: Vol.50 Pages: 068002-1-068002-2

    • DOI

      DOI:10.1143/JJAP.50.068002

    • Peer Reviewed
  • [Journal Article] Green-emissive Mn-activated nanocrystallized glass with willemite-type Zn_2GeO_42011

    • Author(s)
      高橋儀宏, 安藤正尊, 井原梨恵, 藤原巧
    • Journal Title

      Optical Materials Express

      Volume: Vol.1 Pages: 372-378

    • DOI

      DOI:10.1364/OME.1.000372

    • Peer Reviewed
  • [Journal Article] Formation of Zn defects in willemite-type Zn_2GeO_4 during supercooled liquid-crystal phase transition2011

    • Author(s)
      高橋儀宏, 安藤正尊, 井原梨恵, 藤原巧
    • Journal Title

      Applied Physics Letters

      Volume: Vol.98 Pages: 221907-1-221907-3

    • DOI

      DOI:10.1063/1.3597300

    • Peer Reviewed
  • [Journal Article] Crystallization of tungstenbronze-type Ba_2NaNb_5O_<15> in high-Nb_2O_5-content glass : An inelastic light scattering study2010

    • Author(s)
      高橋儀宏, 藤江将啓, 長田実, 正井博和, 井原梨恵, 藤原巧
    • Journal Title

      Journal of Applied Physics

      Volume: Vol.108 Pages: 103519-1-103519-5

    • DOI

      DOI:10.1063/1.3512909

    • Peer Reviewed
  • [Journal Article] Formation of spherulite and metastable phase in stoichiometric Ba_2Si_3O_8 glass2010

    • Author(s)
      高橋儀宏, 正井博和, 長田実, 井原梨恵, 藤原巧
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: Vol.118 Pages: 955-958

    • Peer Reviewed
  • [Journal Article] Transmission electron microscopy and in situ Raman studies of glassy sanbornite : An insight into nucleation trend and its relation to structural variation2010

    • Author(s)
      高橋儀宏, 長田実, 正井博和, 藤原巧
    • Journal Title

      Journal of Applied Physics

      Volume: Vol.108 Pages: 063507-1-063507-5

    • DOI

      DOI:10.1063/1.3487473

    • Peer Reviewed
  • [Journal Article] Inelastic light scattering from nanocrystallizing niobiotellurite glass : an insight into the metastable phase and phase-transformation dynamics2010

    • Author(s)
      高橋儀宏, 岩渕直樹, 長田実, 正井博和, 井原梨恵, 藤原巧
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: Vol.118 Pages: 814-818

    • Peer Reviewed
  • [Presentation] 非弾性光散乱による酸化物ガラスの相転移ダイナミクスの解明2012

    • Author(s)
      高橋儀宏
    • Organizer
      日本セラミックス協会2012年年会
    • Place of Presentation
      京都大学吉田キャンパス
    • Year and Date
      2012-03-20
  • [Presentation] ガラス構造制御による希土類フリー発光体の開発~ 光エネルギーを操作する環境調和材料2011

    • Author(s)
      高橋儀宏
    • Organizer
      応用物理学会東北支部第66回学術講演会特別シンポジウム「グリーンテクノロジー時代の幕開け」
    • Place of Presentation
      岩手大学工学部テクノホール
    • Year and Date
      2011-12-03
  • [Presentation] ガラスは熱処理中に何が起きているのか?~ ナノ結晶化および相変態ダイナミクス2011

    • Author(s)
      高橋儀宏
    • Organizer
      日本セラミックス協会ガラス部会第43回ガラス部会夏季若手セミナー
    • Place of Presentation
      ホテルシーパレスリゾート(豊橋市)
    • Year and Date
      2011-08-26
  • [Presentation] ガラスの結晶化と非線形フォトニクス応用2010

    • Author(s)
      高橋儀宏, 井原梨恵, 藤原巧
    • Organizer
      日本光学会第118回微小光学研究会「最先端光材料と微小光学」
    • Place of Presentation
      東北大学電気通信研究所
    • Year and Date
      2010-12-03
  • [Book] 多様な配位多面体を有するチタン酸塩の発光-希土類フリー蛍光体として, ニューガラスフォーラム2012

    • Author(s)
      高橋儀宏, 藤原巧
    • Total Pages
      8-13
  • [Book] ボソンピークから見たガラス構造と結晶化過程2010

    • Author(s)
      高橋儀宏, 藤原巧
    • Total Pages
      38-42
  • [Remarks]

    • URL

      http://www.apph.tohoku.ac.jp/fujiwara-lab/

URL: 

Published: 2013-07-31  

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