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2011 Fiscal Year Final Research Report

Pressure enhanced self catalytic decomposition of alginic acid in high temperature high pressure water

Research Project

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Project/Area Number 22760586
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Reaction engineering/Process system
Research InstitutionTohoku University

Principal Investigator

AIDA Taku  東北大学, 大学院・環境科学研究科, 助教 (00466541)

Project Period (FY) 2010 – 2011
Keywords新規反応場 / 超高圧水 / アルギン酸 / 精密分解 / 分子量制御 / 自己触媒効果 / 生体材料 / 組成制御
Research Abstract

Alginate is a biocompatible polymer that has high potential in medical uses such as vessels for drug delivery systems. However, for more specialized uses, the molecular weight needs to be controlled to around ~ 10^3 g/mol. In this work, we investigated the decomposition of alginate in high temperature high pressure water. Under the experimental conditions examined, the decomposition of alginate can be achieved to molecular weights above ~ 10^3g/mol in short reaction times (<1s)without any addition of catalysts, compared to conventional decomposition methods which require addition of acid or base catalyst and long reaction times (hours). Also, we found reaction condition dependencies in the monomer content of the product alginate.

  • Research Products

    (5 results)

All 2012 2011 2010

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (2 results)

  • [Journal Article] Production of organic acids from alginate in high temperature water2012

    • Author(s)
      T. M. Aida, T. Yamagata, C. Abe, H. Kawanami, M. Watanabe, R. L. Smith Jr.
    • Journal Title

      The Journal of Supercritical Fluids

      Volume: 65 Pages: 39-44

    • Peer Reviewed
  • [Journal Article] Reaction kinetics of D-xylose in sub-and supercritical water2010

    • Author(s)
      T. M. Aida, N. Shiraishi, M. Kubo, M. Watanabe and R. L. Smith
    • Journal Title

      The journal of Superctical Fluids

      Volume: 55 Pages: 208-216

    • Peer Reviewed
  • [Journal Article] Depolymerization of Sodium alginate under hydrothermal conditions2010

    • Author(s)
      T. M. Aida, T. Yamagata, M. Watanabe, R. L. Smith
    • Journal Title

      Carbohydrate Polymers

      Volume: 80 Pages: 296-302

    • Peer Reviewed
  • [Presentation] ecomposition Kinetics of Sodium Alginate and Production of Organic Acids In High Temperature Water2011

    • Author(s)
      T. M. Aida, C. Abe, T. Yamagata, K. Oshima, M. Watanabe, H. Kawanami, R. L. Smith Jr.
    • Organizer
      AIChE Annual Meeting
    • Place of Presentation
      Minneapolis, USA
    • Year and Date
      2011-11-19
  • [Presentation] 熱水中におけるアルギン酸分解反応の圧力効果2010

    • Author(s)
      阿部ちひろ, 相田卓, 渡邉賢, R. L. Smith
    • Organizer
      化学工学会第42回秋季大会
    • Place of Presentation
      京都
    • Year and Date
      2010-09-08

URL: 

Published: 2013-07-31  

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