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2013 Fiscal Year Final Research Report

Synthesis of high purity hBN crystals and realization for their new functions

Research Project

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Project/Area Number 23246116
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionNational Institute for Materials Science

Principal Investigator

TANIGUCHI Takashi  独立行政法人物質・材料研究機構, 先端材料プロセスユニット, グループリーダー (80354413)

Co-Investigator(Kenkyū-buntansha) WATANABE Kenji  物質・材料研究機構, 光・電子材料ユニット 光電機能グループ, 主席研究員 (20343840)
KAWAMURA Fumio  物質・材料研究機構, 先端材料プロセスユニット 超高圧グループ, 主任研究員 (80448092)
MIYAKAWA Masashi  物質・材料研究機構, 超伝導物性ユニット強相関物質探索グループ, 主任研究員 (40552667)
OBA Fumiyasu  京都大学, 大学院工学研究科 材料工学専攻, 准教授 (90378795)
YAMADA Takatoshi  (独)産業技術総合研究所, ナノチューブ応用研究センター, 主任研究員 (30306500)
NAKAYAMA Atsuko  新潟大学, 研究推進機構 超域学術院, 准教授 (50399383)
Project Period (FY) 2011-04-01 – 2014-03-31
Keywords六方晶窒化ホウ素単結晶 / 遠紫外線発光 / グラフェン基板
Research Abstract

Purposes of this study are synthesis of high purity hBN crystals and realization for their new functions. Band gap of hBN crystal and effect of carbon impurity on intense band edge far-ultraviolet emission of hBN were experimentally clarified. For applications as substrates for graphene, function of hBN graphene layered structure as well as hBN MoS2 structures were investigated on the basis with international collaborations. Fundamental research to understand doping mechanism of large size mismatch system were carried out in the system of Ce doped cBN and AlN.

  • Research Products

    (34 results)

All 2014 2013 2012 2011 Other

All Journal Article (17 results) (of which Peer Reviewed: 17 results) Presentation (14 results) (of which Invited: 14 results) Book (1 results) Remarks (1 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Tunable symmetry breaking and helical edge transport in a graphene quantum spin Hall state2014

    • Author(s)
      A.F.Young, J.D.Sanchez-Yamagishi, B.Hunt, S.H.Choi, K.Watanabe, T.Taniguchi, R.C.Ashoori, and P.Jarillo-Herrero
    • Journal Title

      Nature

      Volume: 505 Pages: 528-532

    • DOI

      10.1038/nature12800

    • Peer Reviewed
  • [Journal Article] Tunable Phonon Polaritons in Atomically Thin van der Waals Crystals of Boron Nitride2014

    • Author(s)
      S.Dai, Z.Fei, Q.Ma, A.S.Rodin, M.Wagner, A.S.McLeod, M.K.Liu, W.Gannett, W.Regan, K.Watanabe, T.Taniguchi, M.Thiemens, G.Dominguez, A.H.C.Neto, A.Zettl, F.Keilmann, P.Jarillo-Herrero, M.M.Fogler, and D.N.Basov
    • Journal Title

      Science

      Volume: 343 Pages: 1125-1129

    • DOI

      10.1126/science.1246833

    • Peer Reviewed
  • [Journal Article] Atomic structure of luminescent centers in high-efficiency Ce-doped w-AlN single crystal2014

    • Author(s)
      R.Ishikawa, A.R.Lupini, F.Oba, S.D.Findlay, N.Shibata, T.Taniguchi, K.Watanabe, H.Hayashi, T.Sakai, I.Tanaka, Y.Ikuhara, and S.J.Pennycook
    • Journal Title

      Scientific Reports

      Volume: 4 Pages: 3778-1-5

    • DOI

      10.1038/srep03778

    • Peer Reviewed
  • [Journal Article] Screening Charged Impurities and Lifting the Orbital Degeneracy in Graphene by Populating Landau Levels2014

    • Author(s)
      A.Luican-Mayer, M.Kharitonov, G.Li, C.-P.Lu, I.Skachko, A.-M.B.Goncalves, K.Watanabe, T.Taniguchi, and E.Y.Andrei
    • Journal Title

      Phys. Rev. Lett

      Volume: 112 Pages: 036804

    • DOI

      10.1103/PhysRevLett.112.036804

    • Peer Reviewed
  • [Journal Article] Reconfigurable p-n junction diodes and the photovoltaic effect in exfoliated MoS2 films2014

    • Author(s)
      S.Sutar, P.Agnihotri, E.Comfort, T.Taniguchi, K.Watanabe, and L.Ung, Ji
    • Journal Title

      Appl. Phys. Lett

      Volume: 104 Pages: 122104

    • DOI

      10.1063/1.4870067

    • Peer Reviewed
  • [Journal Article] Local environment of silicon in cubic boron nitride2013

    • Author(s)
      H.Murata, T.Taniguchi, S.Hishita, T.Yamamoto, F.Oba, and I.Tanaka
    • Journal Title

      Journal ofApplied Physics

      Volume: 114 Pages: 233502-1-4

    • DOI

      10.1063/1.4849015

    • Peer Reviewed
  • [Journal Article] Functional complex point-defect structure in a huge-size-mismatch system2013

    • Author(s)
      R.Ishikawa, N.Shibata, F.Oba, T.Taniguchi, S.D.Findlay, I.Tanaka, and Y.Ikuhara
    • Journal Title

      Physical Review Letters

      Volume: 110 Pages: 065504-1-5

    • DOI

      10.1103/PhysRevLett.110.065504

    • Peer Reviewed
  • [Journal Article] Thermal Conductivity and Phonon Transport in Suspended Few-Layer Hexagonal Boron Nitride2013

    • Author(s)
      I.Jo, M.T.Pettes, J.Kim, K.Watanabe, T.Taniguchi, Z.Yao, and L.Shi
    • Journal Title

      Nano Letters

      Volume: 13 Pages: 550-554

    • DOI

      10.1021/nl304060g

    • Peer Reviewed
  • [Journal Article] Photovoltaic infrared photoresponse of the high-mobility graphene quantum Hall system due to cyclotron resonance2013

    • Author(s)
      S.Masubuchi, M.Onuki, M.Arai, T.Yamaguchi, K.Watanabe, T.Taniguchi, and T.Machida
    • Journal Title

      Phys. Rev. B

      Volume: 88 Pages: 121402

    • DOI

      10.1103/PhysRevB.88.121402

    • Peer Reviewed
  • [Journal Article] Electrically tunable transverse magnetic focusing in graphene2013

    • Author(s)
      T.Taychatanapat, K.Watanabe, T.Taniguchi, P.Jarillo-Herrero
    • Journal Title

      Nat. Phys

      Volume: 9[4] Pages: 225-229

    • DOI

      10.1038/NPHYS2549

    • Peer Reviewed
  • [Journal Article] One-dimensional electrical contact to a two-dimensional material2013

    • Author(s)
      L.Wang, I.Meric, P.Huang, Q.Gao, Y.Gao, H.Tran, T.Taniguchi, K.Watanabe, L.M.Campos, D.Muller, J.Guo, P.Kim, J.Hone, K.Shepard, C.Dean
    • Journal Title

      Science

      Volume: 342 Pages: 614-617

    • DOI

      10.1126/science.1244358

    • Peer Reviewed
  • [Journal Article] Massive Dirac Fermions and Hofstadter Butterfly in a van der Waals Heterostructure2013

    • Author(s)
      B.Hunt, J.D.Sanchez-Yamagishi, A.F.Young, M.Yankowitz, B.J.LeRoy, K.Watanabe, T.Taniguchi, P.Moon, M.Koshino, P.Jarillo-Herrero, and R.C.Ashoori
    • Journal Title

      Science

      Volume: 340 Pages: 1427-1430

    • DOI

      10.1126/science.1237240

    • Peer Reviewed
  • [Journal Article] Hofstadter's butterfly and the fractal quantum Hall effect in moire superlattices2013

    • Author(s)
      C.R.Dean, L.Wang, P.Maher, C.Forsythe, F.Ghahari, Y.Gao, J.Katoch, M.Ishigami, P.Moon, M.Koshino, T.Taniguchi, K.Watanabe, K.L.Shepard, J.Hone, and P.Kim
    • Journal Title

      Nature

      Volume: 497 Pages: 598-602

    • DOI

      10.1038/nature12186

    • Peer Reviewed
  • [Journal Article] Quantum Hall Effect Screening and Layer-Polarized Insulating States in Twisted Bilayer Graphene2012

    • Author(s)
      J.Sanchez-Yamagishi, T.Taychatanapat, K.Watanabe, T.Taniguchi, A.Yacoby and P.Jarillo-Herrero
    • Journal Title

      Phys. Rev. Lett

      Volume: 108[7] Pages: 076601-1

    • DOI

      10.1103/PhysRevLett.108.076601

    • Peer Reviewed
  • [Journal Article] Long-Wavelength Local Density of States Oscillations Near Graphene Step Edges2012

    • Author(s)
      J.Xue, J.Sanchez-Yamagishi, K.Watanabe, T.Taniguchi, P.Jarillo-Herrero and B.LeRoy
    • Journal Title

      Phys. Rev. Lett

      Volume: 108[1] Pages: 016801-1

    • DOI

      10.1103/PhysRevLett.108.016801

    • Peer Reviewed
  • [Journal Article] Hunting for Monolayer Boron Nitride : Optical and Raman Signatures2011

    • Author(s)
      R.V.Gorbachev, I.Riaz, R.R.Nair, R.Jalil, L.Britnell, B.D.Belle, E.W.Hill, K.S.Novoselov, K.Watanabe, T.Taniguchi, A.K.Geim and P.Blake
    • Journal Title

      Small

      Volume: 7[4] Pages: 465-468

    • DOI

      10.1002/smll.201001628

    • Peer Reviewed
  • [Journal Article] Exciton optical transitions in a hexagonal boron nitride single crystal2011

    • Author(s)
      L.Museur, G.Brasse, A.Pierret, S.Maine, B.Attal-Tretout, F.Ducastelle, A.Loiseau, J.Barjon, K.Watanabe, T.Taniguchi and A.Kanaev
    • Journal Title

      Phys. Status Solidi-Rapid Res. Lett

      Volume: 5[5-6] Pages: 214-216

    • DOI

      10.1002/pssr.201105190

    • Peer Reviewed
  • [Presentation] Band alignment of zinc-blende and chalcopyrite semiconductors : Effects of misfit dislocations2014

    • Author(s)
      F.Oba
    • Organizer
      APS March Meeting 2014
    • Place of Presentation
      Denver
    • Year and Date
      2014-03-03
    • Invited
  • [Presentation] Synthesis of high purity hBN single crystals by using solvent growth process2013

    • Author(s)
      T.Taniguchi, K.Watanabe
    • Organizer
      5th Inter. Conf on Recent Progress in Graphene Res
    • Place of Presentation
      Tokyo
    • Year and Date
      20130909-13
    • Invited
  • [Presentation] Luminescence image of cleaved crystal in hexagonal boron nitride grown by temperature gradient method2013

    • Author(s)
      渡邊賢司
    • Organizer
      第32回電子材料シンポジウム
    • Place of Presentation
      滋賀県守山市
    • Year and Date
      20130710-12
    • Invited
  • [Presentation] Optical Properties of Boron Nitride Single Crystals2013

    • Author(s)
      K.Watanabe
    • Organizer
      CLEO-PR 2013
    • Place of Presentation
      京都
    • Year and Date
      20130630-0704
    • Invited
  • [Presentation] Point defects in oxide and nitride semiconductors : Understanding and prediction toward material screening2013

    • Author(s)
      F.Oba
    • Organizer
      MRS Fall Meeting
    • Place of Presentation
      Boston
    • Year and Date
      2013-12-03
    • Invited
  • [Presentation] 高圧合成法による高純度窒化ホウ素単結晶研究の現状と新しい応用展開2013

    • Author(s)
      渡邊賢司
    • Organizer
      第15回応用物理学会プラズマエレクトロニクス分科会新領域研究会
    • Place of Presentation
      名古屋
    • Year and Date
      2013-11-22
    • Invited
  • [Presentation] Complex behavior of defects in oxide semiconductors : Insights from first-principles calculations2013

    • Author(s)
      F.Oba
    • Organizer
      International Symposium on Compound Semiconductors 2013 (ISCS2013)
    • Place of Presentation
      Kobe
    • Year and Date
      2013-05-21
    • Invited
  • [Presentation] 窒化ホウ素単結晶の高圧合成2012

    • Author(s)
      谷口 尚
    • Organizer
      第36回結晶成長討論会,日本結晶成長学会
    • Place of Presentation
      佐賀
    • Year and Date
      20120926-28
    • Invited
  • [Presentation] 高純度窒化ホウ素単結晶の高圧下フラックス成長2012

    • Author(s)
      谷口 尚
    • Organizer
      第7回日本フラックス成長研究発表会
    • Place of Presentation
      つくば
    • Year and Date
      2012-12-07
    • Invited
  • [Presentation] Complex behavior of point defects in oxide and nitride semiconductors : Insights from density functional calculations2012

    • Author(s)
      F.Oba
    • Organizer
      The 5th International Symposium on Designing, Processing and Properties of Advanced Engineering Materials (ISAEM-2012)
    • Place of Presentation
      Toyohashi
    • Year and Date
      2012-11-08
    • Invited
  • [Presentation] 酸化物・窒化物半導体における点欠陥の電子構造と機能2012

    • Author(s)
      大場史康
    • Organizer
      日本金属学会2012年秋期講演大会
    • Place of Presentation
      松山市
    • Year and Date
      2012-09-19
    • Invited
  • [Presentation] Synthesis of hBN single crystals under high pressure and high temperature2011

    • Author(s)
      T.Taniguchi
    • Organizer
      第7回日米セミナー Nanoscale Transport Phenomena, JSPS(Japan), NSF(USA), ONR (USA)
    • Place of Presentation
      Ise,Shima
    • Year and Date
      20111211-14
    • Invited
  • [Presentation] High purity boron nitride : synthesis under high pressure and 1atm, and their properties2011

    • Author(s)
      T.Taniguchi
    • Organizer
      NDNC2011
    • Place of Presentation
      Matsue
    • Year and Date
      20110516-20
    • Invited
  • [Presentation] 高純度窒化ホウ素単結晶及び焼結体の高圧合成と機能発現2011

    • Author(s)
      谷口 尚
    • Organizer
      先進セラミックス第124委員会 第136回会議,日本学術振興会
    • Place of Presentation
      東京
    • Year and Date
      2011-06-02
    • Invited
  • [Book] "Synthesis and Properties of Single Crystalline cBN and Its Sintered Body, In V.K.Sarin (Editor-in-Chief) & C.E. Nebel (Vol.Ed.), Comprehensive Hard Materials (vol.3) (ISBN: 9780080965277)2014

    • Author(s)
      T.Taniguchi
    • Total Pages
      587-605
    • Publisher
      Elsevier
  • [Remarks]

    • URL

      http://www.nims.go.jp/personal/BN_research/index-j_BNR.html

  • [Patent(Industrial Property Rights)] 紫外線発光六方晶窒化ホウ素結晶体の製造方法2013

    • Inventor(s)
      谷口 尚、渡邊賢司、窪田陽一、津田 統
    • Industrial Property Rights Holder
      潮田資勝
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      特許第5257995号
    • Acquisition Date
      2013-05-02

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Published: 2015-06-25   Modified: 2015-07-02  

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