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2012 Fiscal Year Final Research Report

Development of a spatio-time-resolved cathodoluminescence spectroscopy technique applicable for wide bandgap semiconductors through the generation and focusing of high-brightness femtosecond pulsed photoelectron beams

Research Project

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Project/Area Number 23656206
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Electronic materials/Electric materials
Research InstitutionTohoku University

Principal Investigator

CHICHIBU Shigefusa  東北大学, 多元物質科学研究所, 教授 (80266907)

Co-Investigator(Renkei-kenkyūsha) HAZU Kouji  東北大学, 多元物質科学研究所, 助教 (30367057)
Project Period (FY) 2011 – 2012
Keywords電気・電子材料 / 高輝度フェムト秒収束電子線 / ワイドバンドギャップ半導体 / 時間空間同時分解計測 / 結晶評価
Research Abstract

To probe local carrier dynamics in wide bandgap semiconductors such as AlN and high AlN mole fraction AlGaN alloys, the use of spatio-time-resolved cathodoluminescence (STRCL) technique offering high spatial and temporal resolutions is preferred, becauseelectron beams can be focused and implanted into sub-micrometer to nanometer regions of interest. In this study, we succeeded in developing a novel front-excitation type high-brightness pulsed photoelectron (PE)- gun driven by femtosecond laser pulses, and the STRCL measurement system equipped with this PE-gun was used to measure the local emission dynamics in GaN, AlN, and high AlN mole fraction AlGaN alloys.

  • Research Products

    (20 results)

All 2013 2012 2011 Other

All Journal Article (7 results) (of which Peer Reviewed: 7 results) Presentation (9 results) Book (1 results) Remarks (3 results)

  • [Journal Article] Impacts ofSi-doping and resultant cation vacancy formation on the luminescence dynamics for the near-band-edge emission of Al_<0.6>Ga_<0.4>N films grown on AlN templates by metalorganic vapor phase epitaxy2013

    • Author(s)
      S. F. Chichibu, H. Miyake, Y. Ishikawa, M. Tashiro, T. Ohtomo, K. Furusawa, K. Hazu, K. Hiramatsu, and A. Uedono
    • Journal Title

      Journal of Applied Physics

      Volume: Vo. 113

    • Peer Reviewed
  • [Journal Article] Spatio-time-resolved cathodoluminescence studies on freestanding GaN substrates grown by hydride vapor phase epitaxy2013

    • Author(s)
      S. F. Chichibu, Y. Ishikawa, M. Tashiro, K. Hazu, K. Furusawa, H. Namita, S. Nagao, K. Fujito, and A. Uedono
    • Journal Title

      Electrochemical Society Transactions

      Volume: Vol. 50, No.42 Pages: 1-8

    • Peer Reviewed
  • [Journal Article] Time-resolved luminescence studies on AlN and high AlN mole fractionAlGaN alloys2013

    • Author(s)
      S. F. Chichibu, T. Onuma, K. Hazu, and A. Uedono
    • Journal Title

      Physica Status Solidi (c)

      Volume: Vol. 10, No. 3 Pages: 501-506

    • DOI

      DOI:10.1002/pssc.201200676

    • Peer Reviewed
  • [Journal Article] Local lifetime and luminescence efficiency for the near band edge emission of freestanding GaN substrates determined using spatio time resolved cathodoluminescence2012

    • Author(s)
      Y. Ishikawa, M. Tashiro, K. Hazu, K. Furusawa, H. Namita, S. Nagao, K. Fujito, and S. F. Chichibu
    • Journal Title

      Applied Physics Letters

      Volume: Vol. 101, No. 21,212106 Pages: 1-4

    • DOI

      DOI:10.1063/1.4767357

    • Peer Reviewed
  • [Journal Article] Femtosecond-laser-driven photoelectron-gun for time-resolved cathodoluminescence measurement of GaN2012

    • Author(s)
      T. Onuma, Y. Kagamitani, K. Hazu, T. Ishiguro, T. Fukuda, and S. F. Chichibu
    • Journal Title

      Review of Scientific Instruments

      Volume: Vol. 83, No. 4, 043905 Pages: 1-7

    • DOI

      DOI:10.1063/1.3701368

    • Peer Reviewed
  • [Journal Article] Advantages and remaining issues of state-of-the-art m-plane freestanding GaN substrates grown by halide vapor phase epitaxy for m-plane InGaN epitaxial growth2012

    • Author(s)
      S. F. Chichibu, M. Kagaya, P. Corfdir, J. D. Ganiere, B. Deveaud-Pledran, N. Grandjean, S. Kubo, and K. Fujito
    • Journal Title

      Semiconductor Science and Technology

      Volume: Vol. 27,024008 Pages: 1-7

    • DOI

      DOI:10.1088/0268-1242/27/2/024008

    • Peer Reviewed
  • [Journal Article] Collateral evidence for an excellent radiative performance of AlxGa1-xN alloy films of high AlN mole fractions2011

    • Author(s)
      S. F. Chichibu, K. Hazu, T. Onuma, and A. Uedono
    • Journal Title

      Applied Physics Letters

      Volume: Vol. 99, No. 5, 051902 Pages: 1-3

    • DOI

      DOI:10.1063/1.3615681

    • Peer Reviewed
  • [Presentation] 高輝度表面入射型パルス電子銃を搭載した時間空間分解カソードルミネッセンス装置によるHVPE成長GaN基板の評価2013

    • Author(s)
      石川陽一,古澤健太郎,田代公則,羽豆耕治,長尾哲,池田宏隆,藤戸健史,秩父重英
    • Organizer
      2013年春季応用物理学会(30p-G21-3)
    • Place of Presentation
      神奈川工業大学,神奈川県
    • Year and Date
      2013-03-30
  • [Presentation] Impacts of point defects on the photoluminescence lifetime of Si-doped Al_<0.6>Ga_<0.4>N epilayers grown on an AlN template2012

    • Author(s)
      S. F. Chichibu, K. Hazu, Y. Ishikawa, M. Tashiro, H. Miyake, K. Hiramatsu, and A. Uedono
    • Organizer
      International Workshop on Nitride Semiconductors 2012 (IWN2012)
    • Place of Presentation
      Sapporo,Japan
    • Year and Date
      2012-10-17
  • [Presentation] Spatio-time-resolved cathodoluminescence studies on freestanding GaN substrates grown by hydride vapor phase epitaxy2012

    • Author(s)
      S. F. Chichibu, Y. Ishikawa, K. Hazu, M. Tashiro, K. Furusawa, H. Namita, S. Nagao, K. Fujito, and A. Uedono
    • Organizer
      Pacific Rim Meeting on Electrochemical and Solid-State Science (PRiME 2012), Session J3: Materials for Solid State Lighting, Hawaii Convention Center
    • Place of Presentation
      Honolulu, Hawaii, USA
    • Year and Date
      2012-10-08
  • [Presentation] 表面入射型パルス光電子銃を搭載した時間空間分解カソードルミネッセンス装置によるワイドバンドギャップ半導体の評価2012

    • Author(s)
      古澤健太郎,石川陽一,田代公則,羽豆耕治,秩父重英
    • Organizer
      2012年秋季応用物理学会(12p-H10-21)
    • Place of Presentation
      愛媛大学,愛媛県
    • Year and Date
      2012-09-12
  • [Presentation] Spatio-time-resolved cathodoluminescence study using a femtosecond focused electron beam on freestanding GaN substrates grown by hydride vapor phase epitaxy2012

    • Author(s)
      S. F. Chichibu, Y. Ishikawa, M. Tashiro, K. Hazu, K. Furusawa, S. Nagao, K. Fujito, and A. Uedono
    • Organizer
      The 39th International Symposium on Compound Semiconductors (ISCS 2012)
    • Place of Presentation
      Santa Barbara, CA, USA
    • Year and Date
      2012-08-29
  • [Presentation] Timeresolved luminescence studies on AlN and high AlN mole fraction AlGaN alloys, 招 待講演2012

    • Author(s)
      S. F. Chichibu and A. Uedono
    • Organizer
      The Fourth International Symposium on Growth of III-Nitrides (ISGN-4)
    • Place of Presentation
      St. Petersburg, Russia
    • Year and Date
      2012-07-18
  • [Presentation] III-V族窒化物半導体の欠陥評価最前線2012

    • Author(s)
      秩父重英,上殿明良
    • Organizer
      応用物理学会シリコンテクノロジー分科会第148回研究集会
    • Place of Presentation
      グランキューブ大阪(大阪国際会議場),大阪府,招待講演
    • Year and Date
      2012-06-14
  • [Presentation] Advantages and issues of m-plane freestanding GaN substrates grown by halide vapor phase epitaxy for InGaN and AlGaN epitaxial growth, 招待講演2012

    • Author(s)
      S. F. Chichibu, K. Hazu, P. Corfdir, J.-D. Ganiere, B. Deveaud-Pledran, N. Grandjean, S. Kubo, H. Namita, S. Nagao, K. Fujito, K. Shimoyama, and A. Uedono
    • Organizer
      German Physical Society (DPG) Spring Meeting, Technical University of Berlin
    • Place of Presentation
      Berlin, Germany
    • Year and Date
      2012-03-26
  • [Presentation] Time-resolved photoluminescence and time-resolved cathodoluminescence studies on AlN andhigh AlN mole fraction AlGaN alloys, 招待講演2011

    • Author(s)
      S. F. Chichibu, T. Onuma, K. Hazu, T. Sota, and A. Uedono
    • Organizer
      European Materials Research Society, 2011 Spring Meeting
    • Place of Presentation
      Session F, Nice, France
    • Year and Date
      2011-05-10
  • [Book] 「ワイドバンドギャップ半導体の新機能出現と時間空間分解分光計測」2011

    • Author(s)
      秩父重英,羽豆耕治
    • Total Pages
      273-276
    • Publisher
      マテリアルインテグレーション(特集:地域と世界に貢献する東北大学多元物質科学研究所)、第24巻,4,5月号
  • [Remarks] (1)国立大学法人東北大学産学連携推進本部「産学連携ものがたり」(2012年4月)p.26-27にSTRCL概念図等を掲載

  • [Remarks] (2)フェムト秒パルス電子線を用いたAlN・AlGaNの時間分解分光評価結果に関して2012年7月にSt.Petersburgで開催された第4回窒化物半導体結晶成長国際会議(ISGN-4)の招待講演で紹介した内容を表す図表が、会議のProceedingsであるPhysica Status Solidi(c)10(2013).の表紙に選定された。

    • URL

      http://onlinelibrary.wiley.com/doi/10.1002/pssc.201390004/abstract

  • [Remarks]

    • URL

      http://www.tagen.tohoku.ac.jp/labo/chichibu/Ronbun.html

URL: 

Published: 2014-09-25  

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