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2012 Fiscal Year Final Research Report

Study of topological order and detection of edge statein the spin liquid state realized in an organic material

Research Project

  • PDF
Project/Area Number 23684025
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Condensed matter physics II
Research InstitutionThe University of Tokyo

Principal Investigator

ITOU Tetsuaki  東京大学, 大学院・工学系研究科, 講師 (50402748)

Project Period (FY) 2011 – 2012
Keywords分子性固体・有機導体 / スピン液体
Research Abstract

I have confirmed that the organic triangular-lattice system EtMe_3Sb[Pd(dmit)_2]_2 has an spin-liquid ground state without antiferromagnetic ordering. The temperature dependence of the spin-lattice relaxation rate suggests that the spin state of this system undergoes an abrupt change at around 1 K. Although some theories had predicted that such an instability is accompanied by topological ordering, I have reached a conclusion that topological ordering is not likely to be realized in this system.
I have also clarified the electronic states which appear when this spin liquid state is destroyed by substituting the counter cation or applying pressure.

  • Research Products

    (12 results)

All 2013 2012 2011

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (9 results)

  • [Journal Article] Kato Nuclear magnetic resonance of the inequivalent carbon atoms in the organic spin-liquid material EtMe_3Sb[Pd(dmit)_2]_22011

    • Author(s)
      T.Itou,K.Yamashita,M.Nishiyama,A.Oyamada,S. Maegawa,K.Kubo,and R.
    • Journal Title

      Physical Review B

      Volume: 84 Pages: 1-5

    • DOI

      doi:10.1103/PhysRevB.84.094405

    • Peer Reviewed
  • [Journal Article] Ground state of the organic spin-liquid material EtMe_3Sb[Pd(dmit)2_]_22011

    • Author(s)
      T.Itou,A.Oyamada,S.Maegawa,and R.Kato
    • Journal Title

      Conference Series

      Volume: 320 Pages: 1-5

    • DOI

      doi:10.1088/1742-6596/320/1/012033

    • Peer Reviewed
  • [Journal Article] NMR study of quantum spin liquid and its phase transition in the organic spin-1/2 triangular lattice antiferromagnet EtMe_3 Sb[Pd(dmit)_2]_22011

    • Author(s)
      S.Maegawa, T.Itou, A.Oyamada, and R.Kato
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 320 Pages: 1-6

    • DOI

      doi:10.1088/1742-6596/320/1/012032

    • Peer Reviewed
  • [Presentation] 量子スピン液体物質EtMe_3Sb[Pd(dmit)_2]_2の圧力下13^C-NMR2013

    • Author(s)
      渡辺恵里
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(広島県)
    • Year and Date
      2013-03-28
  • [Presentation] Spin liquid, superconductivity, and Mott transition observed in the triangular-lattice organic system X[Pd(dmit)_2]_22013

    • Author(s)
      T.Itou
    • Organizer
      QS2C Theory Forum: International Symposium on "Strongly Correlated Quantum Science"
    • Place of Presentation
      University of Tokyo (Tokyo,Japan)
    • Year and Date
      2013-01-27
  • [Presentation] Spin liquid state in EtMe3Sb[Pd(dmit)_2]_22012

    • Author(s)
      T. Itou
    • Organizer
      studied by <13>^C-NMR measurementsTokyo workshop on spin/charge liquids near ordering
    • Place of Presentation
      University of Tokyo (Tokyo, Japan)
    • Year and Date
      2012-11-29
  • [Presentation] Quantum Spin Liquid State in the Triangular-Lattice Mott Insulator2012

    • Author(s)
      T. Itou
    • Organizer
      Observed by <13>^C-NMR International Conference on Science and Technology of Synthetic Metals 2012
    • Place of Presentation
      The Hyatt Regency Atlanta (Atlanta,America)
    • Year and Date
      2012-07-09
  • [Presentation] Low energy magnetic excitation in the organic spin liquid material EtMe_3Sb[Pd(dmit)_2]_22012

    • Author(s)
      T. Itou
    • Organizer
      observed by <13>^C-NMR International Conference on Highly Frustrated Magnetism 2012
    • Place of Presentation
      McMaster University (Hamilton, Canada)
    • Year and Date
      2012-06-06
  • [Presentation] 二次元面平行ないし面垂直の印加磁場下におけるEtMe_3Sb[Pd(dmit)_2]_2の単結晶13C-NMR2012

    • Author(s)
      伊藤哲明
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学(兵庫県)
    • Year and Date
      2012-03-24
  • [Presentation] (Me_4Sb)_x(EtMe_3Sb)_1-x[Pd(dmit)_2]_2混晶系の13^C-NMR2012

    • Author(s)
      渡辺恵里
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学(兵庫県)
    • Year and Date
      2012-03-24
  • [Presentation] NMRによるフラストレート三角格子X[Pd(dmit)_2]_2系における新奇磁性・超伝導の研究2011

    • Author(s)
      伊藤哲明
    • Organizer
      日本物理学会2011年秋季大会2011年度若手奨励賞受賞記念講演
    • Place of Presentation
      富山大学(富山)
    • Year and Date
      2011-09-23
  • [Presentation] NMRによるフラストレート三角格子X[Pd(dmit)_2]_2系における新奇磁性・超伝導の研究2011

    • Author(s)
      伊藤哲明
    • Organizer
      研究会:金属dmit錯体による磁性・伝導性研究の最前
    • Place of Presentation
      理化学研究所(埼玉)
    • Year and Date
      2011-05-13

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Published: 2014-08-29  

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