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2012 Fiscal Year Final Research Report

Study of energy loss mechanisms in organic thin film solar cells by using quantum beam based analytical techniques

Research Project

  • PDF
Project/Area Number 23760276
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Electronic materials/Electric materials
Research InstitutionUniversity of Tsukuba

Principal Investigator

SAKURAI Takeaki  筑波大学, 数理物質系, 講師 (00344870)

Project Period (FY) 2011 – 2012
Keywords太陽電池 / 有機/金属界面 / ドーピング / 量子ビーム計測
Research Abstract

In this research, we have investigated
(1) electronic properties of electrode buffer layers by means of ultraviolet photoelectron spectroscopy
and (2) the charge transfer speed at molecule/electrode interfaces by means of photoelectron spectroscopy and core-hole clock spectroscopy.
It was found that electrondoping from metal to molecule results in effective electrode contact; that is, the high speed charge transfer of less than 10 fs happens at electrode interfaces. Moreover, it became clear that the electrondoping affected energy level alignment of two or more organic layers. Thus, control of electron doping at organic/metal interface is indispensable to selection of the optimal device structure, and it became clear to become a key to highly efficient OSCs.

  • Research Products

    (31 results)

All 2013 2012 2011 Other

All Journal Article (5 results) (of which Peer Reviewed: 5 results) Presentation (24 results) Book (1 results) Remarks (1 results)

  • [Journal Article] Energy band bending induced charge accumulation at fullerene/bathocuproine heterojunction interface2012

    • Author(s)
      S.Wang, T.Sakurai, R.Kuroda, K.Akimoto
    • Journal Title

      Applied Physics Letters

      Volume: 100 Pages: Art.243302

    • DOI

      DOI:10.1063/1.4728996

    • Peer Reviewed
  • [Journal Article] Energy level alignment at interfaces between 3-(4-biphenylyl)-4-phenyl-5-(4-tert -butyl phenyl)-1, 2, 4-triazole (TAZ) and metals (Ca, Mg, Ag, and Au): experiment and theory2012

    • Author(s)
      B.M. Datt, A. Baba, T. Sakurai, K. Akimoto
    • Journal Title

      Journal of Solid State Electrochemistry

      Volume: 3 Pages: 1141-1149

    • DOI

      DOI:10.1007/s10008-011-1497-2

    • Peer Reviewed
  • [Journal Article] Energy level alignment of C60/Ca interface with bathocuproine as a interlayer studied by ultraviolet photoelectron spectroscopy2012

    • Author(s)
      S.Wang, T.Sakurai, R.Kuroda, H.Kato, K.Akimoto
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 51 Pages: 10NE32

    • DOI

      DOI:10.1143/JJAP.51.10NE32

    • Peer Reviewed
  • [Journal Article] Structural control of organic solar cells based on nonplanar metallophthalocyanine/C60 heterojunctions using organic buffer layers2011

    • Author(s)
      T. Sakurai, T. Ohashi, H. Kitazume, M. Kubota, T. Suemasu, K. Akimoto
    • Journal Title

      Organic Electronics

      Volume: 12 Pages: 966

    • DOI

      DOI:10.1016/j.orgel.2011.03.016

    • Peer Reviewed
  • [Journal Article] Effect of Ag-doped bathocuproine on the recombination properties of exciton in fullerene

    • Author(s)
      Shenghao Wang, Takeaki Sakurai, Keiichirou Komatsu, Katsuhiro Akimoto
    • Journal Title

      Journal of Crystal Growth

      Volume: (in press)

    • DOI

      DOI:10.1016/j.jcrysgro.2012.12.126

    • Peer Reviewed
  • [Presentation] 有機半導体/金属界面電子準位接続と分子構造の相関2013

    • Author(s)
      櫻井岳暁,王生浩,付巍,間瀬一彦,秋本克洋
    • Organizer
      平成25年春季 第60回応用物理学関係連合講演会
    • Place of Presentation
      神奈川工科大学
    • Year and Date
      20130327-30
  • [Presentation] 紫外光電子分光による有機へテロ界面の電子準位接続に関する研究2013

    • Author(s)
      付巍,王生浩,櫻井岳暁,間瀬一彦,秋本克洋
    • Organizer
      平成25年春季 第60回応用物理学関係連合講演会
    • Place of Presentation
      神奈川工科大学
    • Year and Date
      20130327-30
  • [Presentation] Chemical interaction at the interfacesbetween bathocuproine and Mg2013

    • Author(s)
      Shenghao Wang, Takeaki Sakurai, Kazuhiko Mase, Katsuhiro Akimoto
    • Organizer
      7^<th>International conference on Molecular Electronics and Bioelectronics
    • Place of Presentation
      福岡 E-P19
    • Year and Date
      20130317-19
  • [Presentation] Role of electrode buffer layers in organic solar cells2013

    • Author(s)
      T.Sakurai, S.Wang, S.Toyoshima, K.Akimoto
    • Organizer
      IEEE international renewable and sustainable energy conference
    • Place of Presentation
      Ourazazate, Morocco. S-1(oral)
    • Year and Date
      20130307-09
  • [Presentation] The effect of bathocuproine on the recombination of exciton in fullerene2012

    • Author(s)
      Shenghao Wang, Takeaki Sakurai, Keiichirou Komatsu, Katsuhiro Akimoto
    • Organizer
      The 17th International Conference on Molecular Beam Epitaxy
    • Place of Presentation
      奈良,MoP-46
    • Year and Date
      20120923-28
  • [Presentation] Study on the interaction between Bathocuproine and Mg by Photoemission Spectroscopy2012

    • Author(s)
      王生浩,櫻井岳暁,付巍,秋本克洋
    • Organizer
      平成22年秋季 第71回応用物理学会学術講演会,平成24年秋季 第73回応用物理学会学術講演会
    • Place of Presentation
      愛媛大学
    • Year and Date
      20120911-14
  • [Presentation] Core-hole clock分光によるカルバゾール化合物/金属界面電荷移動の評価2012

    • Author(s)
      櫻井岳暁,王生浩,付巍,間瀬一彦,秋本克洋
    • Organizer
      平成24年秋季 第73回応用物理学会学術講演会
    • Place of Presentation
      愛媛大学
    • Year and Date
      20120911-14
  • [Presentation] Gap states induced energy level alignment of fullerene (C_60)/bathocuproine (BCP) heterojunction interface2012

    • Author(s)
      王生浩,櫻井岳暁,黒田龍介,豊島晋,加藤博雄,秋本克洋
    • Organizer
      平成24年春季 第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学
    • Year and Date
      20120315-18
  • [Presentation] 分子構造の異なるカルバゾール系化合物における有機/金属界面電子物性2012

    • Author(s)
      櫻井岳暁, 王生活, 黒田龍介, 間瀬一彦, 秋本克洋
    • Organizer
      平成24年春季 第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学
    • Year and Date
      20120315-18
  • [Presentation] Role of cathode buffer layer in organic solar cells2012

    • Author(s)
      T.Sakurai
    • Organizer
      2012 Energy Materials Nanotechnology (EMN) Fall meeting
    • Place of Presentation
      Las Vegas, USA.
    • Year and Date
      2012-11-30
  • [Presentation] 放射光光電子分光による有機太陽電池モデル系の界面電子物性評価2012

    • Author(s)
      櫻井岳暁
    • Organizer
      表面科学会学術講演会シンポジウム「放射光表面化学研究の最前線」(
    • Place of Presentation
      東北大学
    • Year and Date
      2012-11-22
  • [Presentation] 有機薄膜太陽電池における電極界面電子状態の放射光解析2012

    • Author(s)
      櫻井岳暁
    • Organizer
      UVSOR 研究会「UVSOR有機固体専用ラインの今後の展開」
    • Place of Presentation
      分子科学研究所
    • Year and Date
      2012-09-25
  • [Presentation] 低分子系有機薄膜太陽電池の界面物性評価2012

    • Author(s)
      櫻井岳暁
    • Organizer
      太陽電池材料開発の現在と未来 -第4回半導体若手ワークショップ
    • Place of Presentation
      東北大学
    • Year and Date
      2012-07-30
  • [Presentation] 有機薄膜太陽電池における界面物性評価とその制御2012

    • Author(s)
      櫻井岳暁
    • Organizer
      第3回つくばグリーンイノベーションフォーラム「有機電子・光機能材料の最前線
    • Place of Presentation
      筑波大学
    • Year and Date
      2012-05-25
  • [Presentation] 有機薄膜太陽電池における界面物性2012

    • Author(s)
      櫻井岳暁
    • Organizer
      神奈川技術アカデミー 有機薄膜太陽電池セミナー
    • Place of Presentation
      神奈川技術アカデミー(川崎市)
    • Year and Date
      2012-03-08
  • [Presentation] ENERGY LEVEL ALIGNMENT OF Ca/BCP/C60 INTERFACES2011

    • Author(s)
      S. Wang, T. Sakurai, R. Kuroda, H. Kato and K. Akimoto
    • Organizer
      21^<st>International Photovoltaic Science and Engineering Conference
    • Place of Presentation
      福岡, 4D-5P-27
    • Year and Date
      20111128-1202
  • [Presentation] Study on the electronic properties of C_60and bathocuproine interface using ultraviolet photoelectron spectroscopy2011

    • Author(s)
      S. Wang, T. Sakurai, R. Kuroda, S. Toyoshima, H. Kato and K. Akimoto
    • Organizer
      The 6th Japan-Sweden Workshop on Advanced Spectroscopy of Organic Materials for Electronic Applications (ASOMEA-VI)
    • Place of Presentation
      加賀温泉, P-6
    • Year and Date
      20111124-26
  • [Presentation] 紫外光電子分光によるC60/BCP 界面の電子構造に関する研究2011

    • Author(s)
      黒田龍介,王生浩,豊島 晋,櫻井岳暁,加藤博雄,秋本克洋
    • Organizer
      平成23年秋季 第72回応用物理学会学術講演会
    • Place of Presentation
      山形大学
    • Year and Date
      20110829-0902
  • [Presentation] Theoretical study of interaction between bathocuproine and various types of metals2011

    • Author(s)
      M.D.Bhatt, T.Sakurai, S.Suzuki, K.Akimoto
    • Organizer
      E-MRS 2011 Spring Meeting
    • Place of Presentation
      Nice, France, N-15.11
    • Year and Date
      20110509-13
  • [Presentation] 有機薄膜太陽電池における界面物性2011

    • Author(s)
      櫻井岳暁, 秋本克洋
    • Organizer
      第21回日本MRS学術シンポジウム(MRS-J)【セッションA】先端プラズマ技術が拓くナノマテリアルズフロンティア
    • Place of Presentation
      横浜開港記念会館(横浜市)
    • Year and Date
      2011-12-21
  • [Presentation] 有機薄膜太陽電池の物性評価2011

    • Author(s)
      櫻井岳暁
    • Organizer
      電子情報技術産業協会(JEITA)電子材料・デバイス技術専門委員会太陽電池技術分科会 第5回委員会
    • Place of Presentation
      JEITA(東京)
    • Year and Date
      2011-12-19
  • [Presentation] CIGS太陽電池ならびに有機薄膜太陽電池のエネルギー損失に関する研究2011

    • Author(s)
      櫻井岳暁
    • Organizer
      第3回半導体デバイス若手ワークショップ(ホテルメリージュ
    • Place of Presentation
      宮崎
    • Year and Date
      2011-11-11
  • [Presentation] 有機薄膜太陽電池における界面制御と評価2011

    • Author(s)
      櫻井岳暁
    • Organizer
      表面技術協会 第42回『ナノテク部会』研究会「クリーンエネルギー創製のためのナノ材料開発」
    • Place of Presentation
      産業技術総合研究所 臨海副都心センター別館(東京)
    • Year and Date
      2011-08-22
  • [Presentation] Interface control of smallmolecule-based organic solar cells2011

    • Author(s)
      Takeaki Sakurai
    • Organizer
      2011 Workshops on Nanotechnology and Solar Cells & Green Chemical Processes and Materials
    • Place of Presentation
      Taisan, Taiwan
    • Year and Date
      2011-06-18
  • [Book] 有機薄膜太陽電池における界面電子構造評価2012

    • Author(s)
      櫻井岳暁
    • Total Pages
      154-164
    • Publisher
      CMC 出版
  • [Remarks] ホームページ

    • URL

      http://www.bk.tsukuba.ac.jp/~semicon

URL: 

Published: 2014-09-25  

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