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2017 Fiscal Year Annual Research Report

trial of the model free-observation of anomalous electron-phonon coupling

Research Project

Project/Area Number 26400322
Research InstitutionKwansei Gakuin University

Principal Investigator

水木 純一郎  関西学院大学, 理工学部, 教授 (90354977)

Co-Investigator(Kenkyū-buntansha) 藤田 全基  東北大学, 金属材料研究所, 教授 (20303894)
町田 昌彦  国立研究開発法人日本原子力研究開発機構, システム計算科学センター, 研究主席 (60360434)
Project Period (FY) 2014-04-01 – 2018-03-31
Keywords強相関電子 / 高温超伝導体 / 非弾性X線散乱 / 中性子非弾性散乱 / 格子振動 / 電子励起
Outline of Annual Research Achievements

物性や機能発現の主役である格子振動エネルギー領域(100meV以下の低エネルギー領域)での電荷の動的相関、特に電子‐格子相互作用の直接観察により、銅酸化物高温超伝導体における格子振動の役割を明らかにすることを目的に研究を進めている。2017年度は、J-PARCでの中性子非弾性散乱実験(INS)が2016年度終了間際に実行されたため、そのデータ解析を中心に研究を行った。試料は、LaSrCuO系では最高の超伝導転移温度を持つ組成の、[100]方向に進むCu-Oボンドストレッチ縦波光学格子振動に注目し、非弾性X線散乱(IXS)による格子振動スペクトルと中性子非弾性散乱によるそれとを比較することによって電子‐格子相互作用の異常を観測することを試みた。これは、注目する格子振動が電子との相互作用が異常に強いため、電子の動きを観るX線と原子核の動きを観る中性子で異なったスペクトル形状が観測されると期待した。結果は、IXSで観測される逆格子ベクトルQ=0.3近傍のボンドストレッチ縦波光学格子振動のスペクトル幅がINSで観測されるそれと比較して1.5倍程度大きいことが解析され、超伝導発現に関わる電子‐格子相互作用の異常を観測したと考えている。
また、、銅酸化物超伝導体に関して、(1)T’構造Pr1.4La0.6CuO4の頂点酸素量を制御した単結晶による磁気励起の観測により、頂点酸素がスピン相関を劇的に誘起させることを発見した。(2)FeSe系超伝導体で高圧誘起超伝導発現(SC-II相)に注目し、FeSe層間にアンモニア分子を挿入した試料の高圧下発光分光法、X線回折法、放射光メスバウアー分光法により電子状態、磁性状態、結晶構造を解析することができ、SC-II発現にスピン相関が誘起した軌道揺らぎが関わっているモデルを提唱した。(論文投稿中)

  • Research Products

    (19 results)

All 2018 2017 Other

All Int'l Joint Research (6 results) Journal Article (6 results) (of which Int'l Joint Research: 5 results,  Peer Reviewed: 6 results,  Open Access: 6 results) Presentation (7 results) (of which Int'l Joint Research: 5 results,  Invited: 3 results)

  • [Int'l Joint Research] The University of Texas at Austin/Brookhaven National Laboratory/Carnegie Institution of Washington(米国)

    • Country Name
      U.S.A.
    • Counterpart Institution
      The University of Texas at Austin/Brookhaven National Laboratory/Carnegie Institution of Washington
  • [Int'l Joint Research] NSRRC(Taiwan)

    • Country Name
      その他の国・地域
    • Counterpart Institution
      NSRRC
  • [Int'l Joint Research] Center for High Pressure Sci. Tech./Univ. Chinese Academy of Sciences(China)

    • Country Name
      China
    • Counterpart Institution
      Center for High Pressure Sci. Tech./Univ. Chinese Academy of Sciences
  • [Int'l Joint Research] University of Genova(Italy)

    • Country Name
      Italy
    • Counterpart Institution
      University of Genova
  • [Int'l Joint Research] Vienna University of(Austria)

    • Country Name
      Austria
    • Counterpart Institution
      Vienna University of
  • [Int'l Joint Research]

    • # of Other Countries
      1
  • [Journal Article] Reentrant valence transition in YbCu4:5 under pressure2018

    • Author(s)
      H. Yamaoka, N. Tsujii, Y. Yamamoto, Y. Michiue, J.-F. Lin, N. Hiraoka, H. Ishii, K.-D. Tsuei, J. Mizuki
    • Journal Title

      Physical Review B

      Volume: 97 Pages: 085106

    • DOI

      10.1103/PhysRevB.97.085106

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Electronic structures and spin states of BaFe2As2 and SrFe2As2 probed by x-ray emission spectroscopy at Fe and As K-absorption edges2017

    • Author(s)
      H. Yamaoka, Y. Yamamoto, J.-F. Lin, J. J. Wu, X. Wang, C. Jin, M. Yoshida, S. Onari, S. Ishida, Y. Tsuchiya, N. Takeshita, N. Hiraoka, H. Ishii, K.-D. Tsuei, P. Chow, Y. Xiao, and J. Mizuki,
    • Journal Title

      Physical Review B

      Volume: 96 Pages: 085129 (1-2)

    • DOI

      10.1103/PhysRevB.96.085129

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Observation of momentum-dependent charge excitations in hole-doped cuprates using resonant inelastic x-ray scattering at the oxygen K edge2017

    • Author(s)
      K. Ishii, T. Tohyama, S. Asano, K. Sato, M. Fujita, S. Wakimoto, K. Tustsui, S. Sota, J. Miyawaki, H. Niwa, Y. Harada, J. Pelliciari, Y. Huang, T. Schmitt, Y. Yamamoto, and J. Mizuki,
    • Journal Title

      Physical Review B

      Volume: 96 Pages: 115148 (1-8)

    • DOI

      10.1103/PhysRevB.96.115148

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Pressure-induced anomalous valence crossover in cubic YbCu5-based compounds2017

    • Author(s)
      H. Yamaoka, N. Tsujii, M. Suzuki, Y. Yamamoto, I. Jarrige, H. Sato, J.-F. Lin, T. Mito, J. Mizuki, H. Sakurai, O. Sakai, N. Hiraoka, H. Ishii, K.-D. Tsuei, M. Giovannini and E. Bauer,
    • Journal Title

      Scientific Reports

      Volume: 7 Pages: 5846

    • DOI

      10.1038/s41598-017-06190-3

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Electronic structure of ferromagnetic heavy fermion, YbPdSi, YbPdGe, and YbPtGe studied by photo-electron spectroscopy, x-ray emission spectroscopy, and DFT+DMFT calculations2017

    • Author(s)
      H. Yamaoka, P. Thunstrom, N. Tsujii, K. Katoh, Y. Yamamoto, E. F. Schwier, K. Shimada, H. Iwasawa, M. Arita, I. Jarrige, N. Hiraoka, H. Ishii, K.-D. Tsuei and J. Mizuki,
    • Journal Title

      J. Physics: Condenst Matter

      Volume: 29 Pages: 475502-475510

    • DOI

      10.1088/1361-648X/aa8b98

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Observation of momentum-dependent charge excitations in hole-doped cuprates using resonant inelastic x-ray scattering at the oxygen K edge2017

    • Author(s)
      M. Taguchi, H. Yamaoka, Y. Yamamoto, H. Sakurai, N. Tsujii, M. Sawada, H. Daimon, K. Shimada, J. Mizuki
    • Journal Title

      Physical Review B

      Volume: 96 Pages: 245113 (1-6)

    • DOI

      10.1103/PhysRevB.96.245113

    • Peer Reviewed / Open Access
  • [Presentation] Resonant Inelastic X-ray Scattering study in Materials science2018

    • Author(s)
      Jun'ichiro Mizuki
    • Organizer
      6th Annual Conference of Analytix 2018
    • Int'l Joint Research / Invited
  • [Presentation] Electronic Excitations of Copper- and Iron-based Superconductors Studied by Resonant and Non-Resonant Inelastic X-ray Scattering2017

    • Author(s)
      Jun'ichiro Mizuki
    • Organizer
      International Conference on Advanced Materials 2017
    • Int'l Joint Research / Invited
  • [Presentation] Electronic Excitation of Cuprates and Iron-based Superconductors Studies by Inelastic X-ray Scattering2017

    • Author(s)
      Jun'ichiro Mizuki
    • Organizer
      4th Annual Global Congress of Knowledge Economy-2017
    • Int'l Joint Research / Invited
  • [Presentation] Origin of the pressure-induced second superconducting phase of (NH3)yCs0.4FeSe with double-dome superconductivity2017

    • Author(s)
      Y. Yamamoto, H. Yamaoka, M. Yoshida, R. Tanaka, S. Shonai, N. Hirao, S. Imada, Y. Oishi, L. Zheng, Xiao Mio, Y. Kubozono, S. Onari, J.-F. Lin, N. Hiraoka, H. Ishii, K.-D. Tuei, J. Mizuki
    • Organizer
      The 10th international conference on Inelastic X-ray Scattering (IXS)
    • Int'l Joint Research
  • [Presentation] In Situ Observation of Electronic State Related to Adsorption State on Pt/C Surface by X-ray Absorption Spectroscopy2017

    • Author(s)
      S. Kusano, D. Matsumura, H. Kishi, T. Sakamoto, S. Yamaguchi, K. Ishii, H. Tanaka, J. Mizuki
    • Organizer
      国際シンポジウム“Future Earth”エネルギー課題に資する新奇なナノ物質・触媒・表面
    • Int'l Joint Research
  • [Presentation] 鉄系超伝導体LnFeAsO1-xHxの高圧下でのX線発光分光、吸収分光、X線回折測定2017

    • Author(s)
      川井拓真, 山本義哉, 山岡人志, 吉田雅洋, 石井啓文, 平岡望, Ku-Ding TsueiC, Jung-Fu Lin, 山浦淳一, 飯村壮史, 松村聡, 細野秀雄, 水木純一郎
    • Organizer
      日本物理学会秋季大会
  • [Presentation] 鉄系超伝導体KxFe2-ySe2の高圧下メスバウアー分光測定2017

    • Author(s)
      山本義哉,三井隆也,北尾真司,瀬戸誠,溝畑尚幸,尾崎壽紀,山岡人志,水木純一郎
    • Organizer
      日本物理学会秋季大会

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Published: 2018-12-17   Modified: 2022-08-18  

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