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1989 Fiscal Year Final Research Report Summary

Study for Isotopic Analysis of Plutonium in the Environment by Internal Conversion Electron and alpha-ray Spectrometry

Research Project

Project/Area Number 63580170
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field Nuclear engineering
Research InstitutionTOHOKU UNIVERSITY

Principal Investigator

SHIOKAWA Yoshinobu  Tohoku University, Institute For Materials Research, Research Associate, 金属材料研究所, 助手 (50111307)

Co-Investigator(Kenkyū-buntansha) HARA Mitsuo  Tohoku University, Institute For Materials Research, Research Associate, 金属材料研究所, 助手 (90005918)
Project Period (FY) 1988 – 1989
KeywordsIsotope analysis / Internal Conversion Electron / Alpha ray / Plutonium / Curium / Actinide
Research Abstract

The isotopic ratios ^<240>Pu/^<239>Pu in plutonium samples purified freshly and allowed to stand for a long time were determined by using a high resolution internal conversion electron spectrometer. As a result, it was proved that the above ratios can be determined accurately and precisely. The method was also examined further through a similar determination with curium samples. It was demonstrated that ^<244>Cm was effectively determined by a comparative measurement. On the other hand, the conversion electron intensities of ^<243>Cm were re-evaluated. Furthermore, a technique coupled with alpha-ray spectrometry, in order to determine the isotopic ratio in samples with low-level radioactivity, was also examined.

  • Research Products

    (14 results)

All Other

All Publications (14 results)

  • [Publications] Y.Shiokawa,K.Suzuki,M.Yagi,S.Suzuki: "A New Internal Conversion Electron Spectrometer and its application to determine the ^<240>Pu to ^<239>Pu Isotope Ratio" J.Radioanal.Nucl.Chem.130. 55-62 (1989)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yagi,Y.Shiokawa,S.Suzuki,M.Hara,I.Satoh,K.Masumoto,T.Mitsugashira: "Measurement of Neutron Emission from a Ti-D_2 System" J.Radioanal.Nucl.Chem.Letters. 137. 411-420 (1989)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Yagi,T.Mitsugashira,I.Satoh,M.Hara,Y.Shiokawa,K.Inoue,K.Masumoto,S.Suzuki: "Measurement of Neutron Emission from a SiO_2-D_2 System" J.Radioanal.Nucl.Chem.Letters. 137. 421-429 (1989)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Shiokawa,K.Suzuki,S.Suzuki,M.Yagi: "Determination of Isotopic Ratios of Plutonium and Curium by Internal Conversion Electron Spectrometry" J.Radioanal.Nucl.Chem.

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Shiokawa,K.Suzuki,S.Suzuki,M.Yagi: "A New Internal Conversion Spectrometer and Its Characteristics" J.Radioanal.Nucl.Chem.

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Shiokawa,M.Yagi: "Isotopic Analysis of ^<243>Cm and ^<244>Cm by High Resolution Internal Conversion Electron Spectrometer" J.Radioanal.Nucl.Chem.

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Shiokawa, K.Suzuki, M.Yagi, S.Suzuki: "A New Internal Conversion Electron Spectrometer and Its Application to Determine the ^<240>Pu to ^<239>Pu Isotope Ratio" J.Radioanal.Nucl.Chem., 130, 55-62(1989).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yagi, Y.Shiokawa, S.Suzuki, M.Hara, I.Satoh, K.Masumoto, T.Mitsugashira: "Measurement of Neutron Emission from a Ti-D_2 System" J.Radioanal.Nucl.Chem.Letters, 137, 421-429(1989).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Yagi, T.Mitsugashira, I.Satoh, M.Hara, Y.Shiokawa, K.Inoue, K.Masumoto, S.Suzuki: "Measurement of Neutron Emission from a SiO_2-D_2 System" J.Radioanal.Nucl.Chem.Letters, 137, 421-429(1989).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Shiokawa, K.Suzuki, S.Suzuki, M.Yagi: "Determination of Isotopic Ratios of Plutonium and Curium by Internal Conversion Electron Spectrometry" J.Radioanal.Nucl.Chem.

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Shiokawa, K.Suzuki, S.Suzuki, M.Yagi: "A New Internal Conversion Spectrometer and Its Characteristics" J.Radioanal.Nucl.Chem.

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Shiokawa, M.Yagi: "Isotopic Analysis of ^<243>Cm and ^<244>Cm by High Resolution Internal Conversion Electron Spectrometer" J.Radioanal.Nucl.Chem.

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Shiokawa, R.Amano, M.Yagi, A.Nomura: "Micropreparation Technique for Actinide Compounds by Chemical Vapor Deposition Using beta-diketone Chelates: Preparation of oxide" J.Less-Common Metals.

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] R.Amano, Y.Shiokawa, M.Yagi: "Micropreparation Technique for Lanthanide and Actinide Compounds by Chemical Vapor Deposition Using beta-diketone Chelates: Preparation of Sulfide" J.Less-Common Metals.

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1993-03-26  

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