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Detection of transient low frequency mode by time-resolved far-infrared spectroscopy with a coherent radiation.

Research Project

Project/Area Number 04555009
Research Category

Grant-in-Aid for Developmental Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field 物理計測・光学
Research InstitutionTOHOKU UNIVERSITY

Principal Investigator

KONDO Yasuhiro  Tohoku University, Faculty of Engineering, Applied Physics, Associated Professor, 工学部, 助教授 (20013534)

Co-Investigator(Kenkyū-buntansha) SUZUKI Yoshiro  Tohoku University, Faculty of Engineering, Applied Physics, Research Associate, 工学部, 助手 (80133932)
Project Period (FY) 1992 – 1994
Project Status Completed (Fiscal Year 1994)
Budget Amount *help
¥9,100,000 (Direct Cost: ¥9,100,000)
Fiscal Year 1994: ¥400,000 (Direct Cost: ¥400,000)
Fiscal Year 1993: ¥400,000 (Direct Cost: ¥400,000)
Fiscal Year 1992: ¥8,300,000 (Direct Cost: ¥8,300,000)
KeywordsTime-resolved spectroscopy / far-infrared / transient absorption / coherent radiation / synchrotron radiation / multichannel detector / array detector / 放射光 / 遠赤外分光 / マルチャンネル検出器 / 加速器 / アルカリハライド / 緩和励起子
Research Abstract

Recent research in Tohoku University revealed that a high energy electron pulse generates intense far-infrared radiation when it passes through magnetic field or thin metal foils. This radiation is an intense CW radiation ranging 30 -40 cm^<-1> with a time width of less than several ps, suggesting that it can be used as a probe light for the transient absorption spectroscopy. In alkali halide crystals, electronic excitation induces defect formation due to recombination of a self-trapped exciton, STE.A recent research using ps laser photolysis has suggested that the STE in NaCl may have the low-frequency vibration which is infrared active.
The aim of this project is (1) to build a system for the far-infrared transient spectroscopy, (2) to detect the low-frequency mode, and (3) to detect THz radiation from laser-excited semiconductor suefaces. In this system, a crystal is excited by the electron pulses and the induced transient states are probed by the far-infrared pulses which was genera … More ted by the electron pulses. For this purpose we make a ten-channel far-infrared polychromator-detector by which the induced absorption spectrum can be measured with single electron pulse.
Results :
(1). A 10-channel polychromator-detector consists of ten InSb hot-electron bolometers and concave gratings were built. This polychromator-detector can detect far-infrared radiation ranging from 4 to 30 cm^<-1>. The detector performance for the pulsed radiation was confirmed by using 300 MeV linac in Tohoku University. For cw far-infrared radiation, a ten-channel lock-in amplifier was made by this project.
(2). The transient absorption measurements were made on several NaCl single crystals at LHeT.However, measured transient spectra showed no definite absorption band due to the low-frequency mode.
(3). By using this system, far-infrared radiation from a fs-laser pulse irradiated GaAs crystal surface was also measured. The dependence of the radiation on the incident angle, polarization, and the intensity of the fs laser pulses were determined. Less

Report

(4 results)
  • 1994 Annual Research Report   Final Research Report Summary
  • 1993 Annual Research Report
  • 1992 Annual Research Report
  • Research Products

    (11 results)

All Other

All Publications (11 results)

  • [Publications] 近藤泰洋: "コヒーレント放射光による遠赤外パルスラジオリシス" 核理研研究報告. 25. 131-135 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] 近藤泰洋: "多チャンネル遠赤外配列検出器によるコヒーレント放射光の検出" 核理研研究報告. 26. 323-329 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] 近藤泰洋: "多チャンネル配列検出器による遠赤外パルスラジオリシス" 核理研研究報告. 27. 15-21 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] YASUHIRO KONDO: "Far-Infrared Pulse Radiolysis by Using a Coherent Synchrotron Radiation (I)" Research Report of Laboratory of Nuclear Science, Tohoku University. Vol 25. 131-135 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] YASUHIRO KONDO: "Detection of Coherent Radiation by a Multichannel Far-Infrared Array Detector" Research Report of Laboratory of Nuclear Science, Tohoku University. Vol 26. 323-329 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] YASUHIRO KONDO: "Far-Infrared Pulse Radiolysis by Using a Multichannel Array Detector" Research Report of Laboratory of Nuclear Science, Tohoku University. Vol 27. 15-21 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] 近藤泰洋: "コヒーレント放射光による遠赤外パルスラジオリシス" 核理研研究報告. 25. 131-135 (1992)

    • Related Report
      1994 Annual Research Report
  • [Publications] 近藤泰洋: "多チャンネル遠赤外配列検出器によるコヒーレント放射光の検出" 核理研研究報告. 26. 323-329 (1993)

    • Related Report
      1994 Annual Research Report
  • [Publications] 近藤泰洋: "多チャンネル配列検出器による遠赤外パルスラジオリシス" 核理研研究報告. 27. 15-21 (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] 近藤泰洋: "多チャンネル遠赤外配列検出器によるコヒーレント放射光の検出" 核理研研究報告. 26. 323-329 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] 中里俊晴: "コヒーレント放射によるバンチ長計測(I)" 核理研研究報告. 26. 297-303 (1993)

    • Related Report
      1993 Annual Research Report

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Published: 1992-04-01   Modified: 2016-04-21  

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