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Study on Exciton Interaction and Biexciton Formation Mechanism using Polarized Light

Research Project

Project/Area Number 07640443
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

HAYASHI Tetsusuke  Kyoto University, Department of Fundamental Sciences, Professor, 総合人間学部, 教授 (80026799)

Co-Investigator(Kenkyū-buntansha) ASHIDA Masaaki  Kyoto University, Department of Physics, Research Associate, 理学部, 助手 (60240818)
WATANABE Masayuki  Kyoto University, Department of Fundamental Sciences, Research Associate, 総合人間学部, 助手 (20240525)
Project Period (FY) 1995 – 1996
Project Status Completed (Fiscal Year 1996)
Budget Amount *help
¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 1996: ¥200,000 (Direct Cost: ¥200,000)
Fiscal Year 1995: ¥2,000,000 (Direct Cost: ¥2,000,000)
KeywordsSEMICONDUCTOR / EXCITON / POLARITON / BIEXCITON
Research Abstract

The purpose of this research project is to clarify the mechanism of biexciton formation through interaction of exciton polaritons in semiconductors such as PbI_2 and CuCl. The obtained results are as follows.
(1) Efficiency of biexciton formation through interaction of excitons has been compared in PbI_2 crystal and Pb_<1-x>Cd_xI_2 mixed crystals. In the mixed crystal, it was found that localized biexcitons are created and the formation efficiency of biexcitons increases by an order of magnitude from that in pure PbI_2 due to the confinement of excitons in the localized states.
(2) Spectrally-resolved four-wave mixing in the exciton resonance region has been investigated under various combination of two polarized lights from a sub-picosecond pulse laser. Coherent interaction of exciton polaritons was found to be dominated by the polarization selection rule for two-photon transition to the biexciton state.
(3) Dependence of biexciton formation on the crystal thickness has been investigated in CuCl thin crystals embedded in a cleaved wedge of NaF crystal. A huge increase in the biexciton luminescence was observed in a particular range of thickness, indicating the interference effect of polaritons.

Report

(3 results)
  • 1996 Annual Research Report   Final Research Report Summary
  • 1995 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] T.Makino: "Excitation Energy Dependence of Biexciton Formation Efficiency in PbI_2" Solid State Commun.93. 983-987 (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] T.Makino: "High Density Effect of Localized Excitons in Pb_<1-x>Cd_xI_2 Crystals : Formation of Localized Biexcitons" Proc.Int.Conf.on Excitonic Processes in Condensed Matter. 63-66 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Watanabe: "Coherent Optical Response of Excitons and Biexcitons in PbI_2 Studied by Femtosecond Four-wave Mixing Spectroscopy" Proc.Int.Conf.on Excitonic Processes in Condensed Matter. 83-86 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] T.Makino: "Luminescence of Localized Biexcitons in Pb_<1-x>Cd_xI_2 Mixed Crystals" J.Phys.Soc.Japan. 65. 3049-3055 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 渡辺雅之: "PbI_2における励起子と励起子分子の非線形光学応答" Proc.2nd Asia Symposium on Condensed Matter Photophysics. 181-184 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 牧野哲征: "PbI_2におけるポラリトン寿命の励起強度依存性" Proc.2nd Asia Symposium on Condensed Matter Photophysics. 185-188 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] T.Makino: "Excitation Energy Dependence of Biexciton Formation Efficiency in PbI_2" Solid State Commun. 93. 983-987 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] T.Makino: "High Density Effect of Localized Excitons in Pb_<1-x>Cd_xI_2 Crystals : Formation of Localized Biexcitons" Proc.Int.Conf.on Excitonic Prccesses in Condensed Matter. 63-66 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Watanabe: "Coherent Optical Response of Excitons and Biexcitons in PbI_2 Studied by Femtosecond Four-Wave Mixing Spectroscopy" Proc.Int.Conf.on Excitonic Prccesses in Condensed Matter. 83-86 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Makino: "Luminescence of Localized Biexcitons in Pb_<1-x>Cd_xI_2 Mixed Crystals" J.Phys.Soc.Japan. 65. 3049-3055 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Watanabe: "Nonlinear Optical Response of Excitons and Biexcitons in PbI_2" Proc.2^<nd> Asia Symposium on Condensed Matter Photophysics. 181-184 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] T.Makino: "Excitation Intensity Dependence of Polariton Lifetime in PbI_2" Proc.2^<nd> Asia Symposium on Condensed Matter Photophysics. 185-188 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] T.Makino: "High Density Effect of Localized Excitons in Pb_<1-x>Cd_xI_2 Crystals : Formation of Localized Biexcitons" Proc.Int.Conf.on Excitonic Processes in Condensed Matter. 63-66 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] M.Watanabe: "Coherent Optical Response of Excitons and Biexcitons in PbI_2 studied by Femtosecond Four-Wave Mixing spectroscopy" Proc.Int.Cont,on Excitonic Processes in Condensed Matter. 83-86 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] T.Makino: "Luminescence of Localized Biexcitons in Pb_<1-x>Cd_xI_2 Mixed Crystals" J.Phys.Soc.Jpn.65-9. 3049-3055 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 渡辺雅之: "PbI_2における励起子と励起子分子の非線形光学応答" Proc.2nd.Asia Symposium on Condensed Matter Photophysics. 181-184 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 牧野哲征: "PbI_2におけるポラリトン寿命の励起強度依存性" Proc.2nd.Asia Symposium on Condeused Matter Photophysics. 185-188 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 牧野哲征: "CuCl薄膜における励起子分子生成・効率の膜厚依存性" 日本物理学会 1997年年会講演概要集. 2(印刷中). (1997)

    • Related Report
      1996 Annual Research Report
  • [Publications] 牧野哲征: "Excitaion Energy Depeudeuce of Biexciton Formation Efficiency in PbI_2" Solid state Corxrmun. 93. 983-987 (1995)

    • Related Report
      1995 Annual Research Report
  • [Publications] 渡辺雅之: "反射型四光波混合による励起子ポラリトンの緩和時間の測定" 日本物理学会 1995年秋の分科会講演概要集. 2. 291 (1995)

    • Related Report
      1995 Annual Research Report
  • [Publications] 牧野哲征: "PbI_2における励起子分子生成レートの温度変化" Proceediugs of the ASIA Symposium on Solid State Photophysies. 167-170 (1995)

    • Related Report
      1995 Annual Research Report
  • [Publications] 牧野哲征: "PbI_2における励起子分子生成レートの温度変化" 日本物理学会 1996年年会講演概要集. 2. 220-220 (1996)

    • Related Report
      1995 Annual Research Report
  • [Publications] 渡辺雅之: "反射型四光波混合による励起子ポラリトンの緩和時間の測定 2" 日本物理学会 1996年年会講演概要集. 2. 220-220 (1996)

    • Related Report
      1995 Annual Research Report

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Published: 1995-04-01   Modified: 2020-05-15  

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