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Theoretical Research of Optical Pulse Response of Quantum Confined Excitons

Research Project

Project/Area Number 09640396
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionOsaka University

Principal Investigator

ISHIHARA Hajime  Graduate School of Engineering Science, Osaka University, Assoc. Prof., 基礎工学研究科, 助教授 (60273611)

Co-Investigator(Kenkyū-buntansha) AJIKI Hiroshi  Graduate School of Engineering Science, Osaka University, Research assist., 基礎工学研究科, 助手 (60283735)
CHO Kikuo  Graduate School of Engineering Science, Osaka University, Prof., 基礎工学研究科, 教授 (60013489)
Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥3,200,000 (Direct Cost: ¥3,200,000)
Fiscal Year 1999: ¥400,000 (Direct Cost: ¥400,000)
Fiscal Year 1998: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 1997: ¥1,900,000 (Direct Cost: ¥1,900,000)
KeywordsNonlinear Optics / Optical Pulse / Excitons / Polaritons / Ultra fast response / Mesoscopic systems / Nano-scale matters / Thin film / パルス応答
Research Abstract

We have developed the theory for the optical response of the ultra short pulse in which the nanoscale spatial structure of the response field in the media is correctly considered. This theory has following features.
The nonlocal response is considered.
The microscopic position dependences of the induced current density and the response field are correctly taken into account.
The self-consistency of the induced current density and the response field are taken into account.
Nonlinear response can be treated.
We take the method such that the simultaneous equations of Maxwell eq. and the equation for the density matrix of the matter system are numerically solved. Taking the rotating wave approximation and slowly varing envelope approximation in time, and reducing the number of the exctitonic states as bases, we make this calculation feasible. Appling this method to the ultra thin film confining excitons, we have clarified the following points.
1.The remarkable nanoscale spatial structure of the response field appears even for the short pulse of several hundreds femto second, and the selection rule that should hold in the case of long wavelength is broken for both the linear and nonlinear regimes. We understand that our approach is essentially necessary in such conditions.
2.We elucidate, for the first time, the real time characteristics of the internal field by the short pulse undergoing multiple reflection.
3.The time characteristics of the nonlinear signal reflects the above mentioned motion of the internal field in time, thus, the nano-scale spatial structure of the internal field takes a important role in the time characteristics of the nonlinear response. It is also clarified that if we neglect this spatial structure of the internal field, we can not describe the correct time variation of the nonlinear signal at all.

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] H. Ishihara: "Manipulation of Nonlinear Response via Nanoscale Spatial Structure of Resonant Internal Field"Material Science & Engineering B. 48. 75-82 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Enhancement of Nonlinear Optical Response due to Cavity-induced Double Resonance in a Semiconductor Ultrathin Film"Appl. Phys. Lett.. 71. 3036-3038 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Enhancement of the-third nonlinear optical response of quantum wells in a Semiconductor microcavity"Appl. Phys. Lett.. 73. 1478-1480 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Theory of the th-rd-order Nonlinear Optical Response of Exciton-Microcavity Coupled System"Phys. Stat. Sol. (a). 170. 301-306 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "A super coupling of radiation field and excitons confined in spatiallyperiodic structure"Physica E. (to be published).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Size dependence of degenerate four wave mixing signal due to enhancement of internal field in mesoscopic systems"J. Luminesc. (to be published).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Theory of transient pulse response including the effect of nanoscale spatial variation of resonant internal field"J. Luminesc. (to be published).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Manipulation of Nonlinear Response via Nanoscale Spatial Structure of Resonant Internal Field"Material Science & Engineering B. vol.48. 75-82 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Enhancement of Nonlinear Optical Response due to Cavity-induced Double Resonance in a Semiconductor Ultrathin Film"Appl. Phys. Lett.. vol.71. 3036-3038 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Enhancement of the third-order nonlinear optical response of quantum wells in a semiconductor microcavity"Appl. Phys. Lett.. vol.73. 1478-1480 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Theory of the Third-Order Nonlinear Optical Response of Exciton-Microcavity Coupled Syetem"phys. stat. sol. (a). vol.170. 301-306 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "A super coupling of radiation field and excitons confined in spatiallyperiodic structure"Physica E. (to be published). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Size dependence of degenerate four wave mixing signal due to enhancement of internal field in mesoscopic systems"J. Luminesc.. (to be published). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Ishihara: "Theory of transient pulse response including the effect of nanoscale spatial variation of resonant internal field"J. Luminesc.. (to be published). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Ishihara: "Size dependence of degenerate four wave mixing signal due to enhancement of internal field in mesoscopic systems"Luminescence and Optical Spectroscopy of Condensed Matter "Osaka 1999, in J. Luminesc.. (to be published).

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Ishihara: "Theory of transient pulse response including the effect of nanoscale spatial variation of resonant internal field"Luminescence and Optical Spectroscopy of Condensed Matter" Osaka 1999, in J. Luminesc.. (to be published).

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Ishihara: "A super coupling of radiation field and excitons confined in spatially periodic structure"Proc. Int. Conf. On "Modulated Semiconductor Structures" Fukuoka 1999, in Physica E.. (to be published).

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Ishihara: "Enhancement of the Third-Order Nonlinear Optical Response of Quantum Wells in a Semiconductor Microcavity" Appl. Phys.lett.73. 1478-1480 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Ishihara: "Theory of the Third-Order Nonlinear Optical Response of Exction-Microcavity Coupled System" Phys. stat. sol. (a). 170. 301-306 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 天方智成: "閉じ込め励起子系における四光波混合信号のサイズ依存性" 光物性研究会'98論文集. 239-242 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Hajime Ishihara: "Manipulation of Nonlinear Response via Nanoscale Spatial Structure of Resonant Internal Field" Material Science & Engineering B. 48. 75-82 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Hajime Ishihara: "Enhancement of Nonlinear Optical Response due to Cavity-Induced Double Resonance in a Semiconductor Ultrathin Film" Appl.Phys.Letters. 71. 3036-3038 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] 張紀久夫: "メゾスコピック系における非局所光学応答" 日本物理学会誌. 52. 343-349 (1997)

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2020-05-15  

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