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Fundamental physical properties of Mn system alloys with platinum group element

Research Project

Project/Area Number 13450255
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical properties of metals
Research InstitutionTohoku University

Principal Investigator

FUKAMACHI Kazuaki  Tohoku University, Graduate School of Engineering, Professor, 大学院・工学研究科, 教授 (00005969)

Co-Investigator(Kenkyū-buntansha) SAKUMA Akimasa  Tohoku University, Graduate School of Engineering, Professor, 大学院・工学研究科, 教授 (30361124)
UMETSU Rie  Tohoku University, Graduate School of Engineering, JSPS Postdoctoral Fellow, 大学院・工学研究科, 日本学術振興会特別研究員
笹尾 和宏  東北大学, 大学院・工学研究科, 博士後期課程・日本学術振興会特別研究員
佐々間 昭正  日立金属(株), 磁性材料研究所, 主任研究員
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥14,700,000 (Direct Cost: ¥14,700,000)
Fiscal Year 2003: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2002: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 2001: ¥11,600,000 (Direct Cost: ¥11,600,000)
KeywordsMn system alloys / Neel temperature / band structures / magnetic structure / electronic specific heat coefficient / electrical resistivity / 結晶歪み
Research Abstract

The fundamental physical properties of γ-Mn and LI_0-type Mn system alloys have been investigated. The main results are listed as follows:
1.It becomes clear that the antiferromagnetic stability of Mn_3Rh ordered alloy is related to the formation of the dip around the Fermi level in their electronic structures.
2.The magnetic phase diagram of γ-MnIr disordered alloy system was investigated and it was revealed from the theoretical and experimental investigations that the magnetic structure closely correlate to the lattice distortion, however the magnetic transition temperature from the fct to fcc structures dos not necessarily accord with the magnetic transition temperatures from the 2Q to 3Q structures.
3.It was clarified from the theoretical and the experimental investigations that the characteristic electronic structures having a pseudo-gap around the Fermi level are common future among the LI_0-type MnTM(TM=Ni, Pd and Pt) system alloys and closely correlate to the very high antiferromagnetic stability.
4.The magnetic, electrical and the low-temperature specific heat measurements were carried out and further the band calculations were made for the LI_0-type MnIr alloy. It was clarified that the alloy behaves pseudo-gap type antiferromagnet in analogy with other LI_0-type MnTM alloys. It also became clear that the LI_0-type MnIr exhibits the highest Neel temperature among te Mn system alloys.
5.The exchange coupling between the ferromagnetic layer and the antiferromagnetic layer, such as the γ-Mn and LI_0-type Mn system alloys, was investigated from using the classical Heisenberg model.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (52 results)

All Other

All Publications (52 results)

  • [Publications] M.Miyakawa: "Specific Heat and Thermal Expansion Characteristics Related to Spin Fluctuations in Antiferromagnetic β-MnOs Alloys"J.Phys.Condens.Matter. 13. 3809-3816 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Sasao: "Atomic Site Preference, the Neel Temperature and specific Heat of β-Mn_<1-x>Ru_x Alloys"J.Alloy and Compd.. 325. 24-28 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Electrical and Calorimetric Evidence of a Pseudo-gap in Antiferromagnetic Equiatomic MnPd Alloy"J.Magn.Magn.Mater.. 239. 530-532 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Concentration Dependence of Magnetic and Electrical Properties of Gap-type antiferromagnetic MnPt Alloys"J.Appl.Phys.. 91. 8873-8875 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Sakuma: "Magnetic structures and Their Stability in Mn_3Rh Ordered and Disordered Alloys"Phys.Rev.B. 66. 014432 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Sasao: "Lattice Distortions and Phase Diagram of Antiferromagnetic γ-MnIr Disordered Alloy System"J.Alloys and Comp.. 352. 21-25 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Sakuma: "First-principles Study on the Magnetic Structures of Ordered and Disordered Mn-Ir Alloy"Phys.Rev.B. 67. 024420 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Magnetovolume Effects and Spin Fluctuations in Mn_<3+x>Rh_<1-x> Alloys"J.Phys.Condens.Matter. 15. 4589-4606 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] C.Mitsumata: "Mechanism of the Exchange Bias Field in Ferromagnetic and Antiferromagnetic Bilayer"Phys.Rev.B. 68. 0144437 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] C.Mitsumata: "Influence of the Spin Structure on the Exchange Bias of Antiferromagnetic and Ferromagnetic Bilayer"IEEE Trans.Magn.MAG. 39. 2738-2740 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Miyakawa: "Antiferromagnetism and Low Temperature Specific Heat of β-Mn_<1-x>Ir_x Alloys"J.Phys.Condens.Matter. 15. 4605-4612 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Miyakawa: "Thermal Expansion Characteristics Related to Spin Fluctuations and the Pressure Effect on the Neel Temperature of β-MnOs Alloys"J.Phys.Condens.Matter. 15. 4817-4825 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Magnetic and Electrical Properties, and Mechanism of Exchange Bias-field of γ-phase and L1_0-type Antiferromagnetic Mn Alloys"J.Magn.Soc.Jpn.. 3. 59-94 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Pseudogap in the Density of States and the High Neel Temperature of L1_0-type MnIr Alloy System"Phys.Rev.B. 69. 104411 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Very High Antiferromagnetic Stability of L1_0-type MnIr Alloys"J.Magn.Magn.Mat.. (印刷中). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Hama: "^<55>Mn NMR/NQR Study in β-MnOs Alloys"J.Magn.Magn.Mat.. (印刷中). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Magnetic Properties and Electronic Structures of L1_0-type MnTM (TM = Ir, Pt, Pd and Ni) Alloy Systems"Metals Materials and Processes. (印刷中). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 藤田麻哉: "最新熱測定「熱膨脹測定の応用」"アグネ技術センター. 39-48 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Miyakawa, R.Y.Umetsu, K.Fukamichi: "Specific Heat and Thermal Expansion Characteristics Related to Spin Fluctuations in Antiferromagnetic β-Mn_<1-x>Ru_x Alloys"J.Phys.Condens. Matter. 13. 3809-3816 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Sasano, R.Y.Umetsu, K.Fukamichi: "Atomic Site Preference, the Neel Temperature and specific Heat of β-Mn_<1-x>Ru_x Alloys"J. Alloy and Compd.. 325. 24-28 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, K.Fukamichi, A.Sakuma: "Electrical and Calorimetric Evidence of a Pseudo-gap in Antiferromagnetic Equiatomic MnPd Alloy"J.Magn.Magn.Mater.. 239. 530-532 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, K.Fukamichi, A.Sakuma: "Concentration Dependence of Magnetic and Electrical Properties of Gap-type antiferromagnetic MnPt Alloys"J.Appl.Phys.. 91. 8873-8875 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Sakuma, R.Y.Umetsu, K.Fukamichi: "Magnetic structures and Their Stability in Mn_3Rh Ordered and Disordered Alloys"Phys.Rev. B. 66. 014432 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Sasao, R.Y.Umetsu, K.Fukamichi, A.Sakuma: "Lattice Distortions and Phase Diagram of Antiferromagnetic γ-MnIr Disordered Alloy System"J. Alloys and Comp.. 352. 21-25 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Sakuma, R.Y.Umetsu, K.Fukamichi: "First-principles Study on the Magnetic Structures of Ordered and Disordered Mn-Ir Alloys"Phys.Rev. B. 67. 024420 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, K.Fukamichi, Y.Fujinaga, A.Sakuma: "Magnetovolume Effects and Spin Fluctuations in Mn_<3+x>Rh_<1-x> Alloys"J.Phys.Condens. Matter. 15. 4589-4604 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] C.Mitsumata, A.Sakuma, K.Fukamichi: "Mechanism of the Exchange Bias Field in Ferromagnetic and Antiferromagnetic Bilayar"Phys.Rev. B. 68. 0144437 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] C.Mitsumata, A.Sakuma, K.Fukamichi: "Influence of the Spin Structure on the Exchange Bias of Antiferromagnetic and Ferromagnetic Bilayer"IEEE Trans.Magn. MAG. 39. 2738-2740 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] B.M.Miyakawa, R.Y.Umetsu, K.Sasao, K.Fukamichi: "Antiferromagnetism and Low Temperature Specific Heat of β-Mn_<1-x>Ir_x Alloys"J.Phys.Condens. Matter. 15. 4605-4612 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Miyakawa, R.Y.Umetsu, K.Fukamichi, H.Yoshida, T.Matsubara: "Thermal Expansion Characteristics Related to Spin Fluctuations and the Pressure Effect on the Neel Temperature of β-MnOs Alloys"J.Phys.Condens. Matter. 15. 4817-4825 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, C.Mitsumata, A.Sakuma, K.Fukamichi: "Magnetic and Electrical Properties, and Mechanism of Exchange Bias-field of γ-phase and LI_0-tyoe Antiferromagnetic Mn Alloys"Trans.Mag.Soc.Jpn.. 3. 59-94 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, M.Miyakawa, K.Fukamichi, A.Sakuma: "Pseudogap in the Density of States and the High Neel Temperature of LI_0-type MnIr Alloy System"Phys.Rev. B. 69. 104411 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, Y.Okamoto, M.Miyakawa, K.Sasao, K.Fukamichi, A.Sakuma: "Very-High Antiferromagnetic Stability of LI_0-tyoe MnIr alloys"J.Magn.Magn.Mat.. (in press). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Hama, M.Mitsumura, H.Yamagata, M.Miyakawa, R.Y.Umetsu, K.Fukamichi: "^<55>Mn NMR/NQR study in β-MnOs Alloys"J.Magn.Magn.Mat.. (in press). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu, K.Fukamichi, A.Sakuma: "Magnetic Properties and Electronic Structures of LI_0-type MnTM(TM=Ir, Pt, Pd and Ni) Alloy System"Metals Materials and Processes. (in press). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] R.Y.Umetsu: "Magnetovolume Effects and Spin Fluctuations in Mn_<3+x>Rh_<1-x> Alloys"J.Phys.Condens.Matter. 15. 4589-4604 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Miyakawa: "Antiferromagnetism and Low Temperature Specific Heat of β-Mn_<1-x>Ir_x Alloys"J.Phys.Condens.Matter. 15. 4605-4612 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Miyakawa: "Thermal Expansion Characteristics Related to Spin Fluctuations and the Pressure Effect on the Neel Temperature of β-MnOs Alloys"J.Phys.Condens.Matter. 15. 4817-4825 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.Y.Umetsu: "Very High Antiferromagnetic Stability of L1_0-type MnIr Alloys"J.Magn.Magn.Mat.. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Hama: "^<55>Mn NMR/NQR Study in β-MnOs Alloys"J.Magn.Magn.Mat.. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.Y.Umetsu: "High Neel Temperature and Low Density of States of L1_0-type MnIr Alloy System"Phys.Rev.B. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.Y.Umetsu: "Magnetic and Electrical Properties, and Mechanism of Exchange Bias-field of γ-phase and L1_0-type Antiferromagnetic Mn Alloy"Trans.Mag.Soc.Jpn.. 27. 59-94 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 梅津理恵: "L1_0型 Mn合金の電子構造と磁気的・電気的性質"日本応用磁気学会誌. 1. 5-14 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.Y.Umetsu: "Magnetic Properties and Electronic Structures of L1_0-type MnTM(TM=Ir, Pt, Pd and Ni)Alloy Systems"Metals Materials and Processes. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] 藤田麻哉: "最新熱測定「熱膨張測定の応用」39-48"アグネ技術センター. (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.Y.Umetsu: "Electrical and Calorimetric Evidence of a Pseudo-gap in Antiferromagnetic Equiatomic MnPd Alloy"J. Magn. Magn. Mater.. 239. 530-532 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] R.Y.Umetsu: "Concentration Dependence of Magnetic and Electrical Properties of Gaptype antiferromagnetic MnPt Alloys"J. Appl. Phys.. 91. 8873-8875 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Sakuma: "Magnetic structures and Their Stability in Mn_3Rh Ordered and Disordered Alloys"Phys. Rev. B. 66. 0144321-0144326 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Sakuma: "First-principles Study on the Magnetic Structures of Ordered and Disordered Mn-Ir Alloys"Phys. Rev. B. 67. 0244201-0244207 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Sasao: "Lattice distortions and phase diagram of antiferromagnetic γ-MnIr disordered alloy system"J. Alloys and Compds. 352. 21-25 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] R.Y.Umetsu: "Electrical and Calorimetric Evidence of a Pseudo-gap in Antiferromagnetic Equiatomic MnPd Alloy"J. Magn. Magn. Mater.. (印刷中).

    • Related Report
      2001 Annual Research Report
  • [Publications] R.Y.Umetsu: "Concentration Dependence of Magnetic and Electrical Properties of Gap-type antiferromagnetic MnPt Alloys"J. Appl. Phys.. (掲載決定).

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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