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Development of nonlinear near-field scanning optical microscope and its application to the study of optical nonlinearlties of semiconductor quantum structures

Research Project

Project/Area Number 13640340
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionKanagawa Academy of Science and Technology

Principal Investigator

MATSUDA Kazunari  Near-field optics group, Special Research Laboratory for Optical Science, Researcher, 光科学重点研究室・近接場光学グループ, 研究員 (40311435)

Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2003: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 2002: ¥1,200,000 (Direct Cost: ¥1,200,000)
Fiscal Year 2001: ¥1,100,000 (Direct Cost: ¥1,100,000)
Keywordsnear-field scanning optical microscope / semiconductor quantum dot / many body effect / 半導体量子構造 / 非線形光学分光 / 非線形光学効果
Research Abstract

With combination of near-field scanning optical microscope and ultra-fast laser pulses, we can create the strong electric field in time and spatial domain around the aperture of the near-field fiber probe. Using this advantage, the nonlinear optical response can be easily induced in the materials. We have developed the new type of optical microscope (nonlinear near-field scanning optical microscope) and investigated the nonlinear-behavior of the optical response in semiconductor quantum structures. The results of this research project are as follows.
1.I have added the compensate system of group velocity dispersion of the pulse to the near-field scanning optical microscope. The nonlinear near-field scanning optical microscope has been constructed due to reduction of the optical pulse broadening in the fiber probe.
2.The double tapered fiber probe with a 20-30 nm aperture can be fabricated using pounding method. The high spatial resolution of 30 nm in the measurement of semiconductor quantum structures has been achieved owing to the high performance of this near-filed fiber probe.
3.The Coulomb interaction is enhanced in a semiconductor quantum dot, because the carriers are confined in a nanometer space. I expect that the nonlinear optical response can be easily induced, if only a few carriers are generated in a semiconductor quantum dot. I investigated the photoluminescence spectrum of a single InGaAs quantum dot at room temperature in the higher excitation conditions. The many body effects and the decrease of phase relaxation time due to Auger scattering process in a quantum dot have been found.
4.I have demonstrated the real-space mapping of exciton wave function confined in a GaAs quantum dot using the near-field scanning optical microscope with a 30 nm spatial resolution.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (57 results)

All Other

All Publications (57 results)

  • [Publications] K.Matsuda et al.: "Near-field photoluminescence imaging spectroscopy of an n-type modulation-doped quantum well with a lateral periodic potential"Nanotechnology. 15. S345-S348 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Saiki et al.: "Nano-optical probing of exciton wave-functions confined in a GaAs quantum dot"Journal of Electron Microscopy. (in print). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Near-field optical mapping of exciton wave functions in a GaAs quantum dot"Physical Review Letters. 91. 177401-1-177401-4 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Carrier-carrier interaction in single InGaAs quantum dots at room temperature investigated by near-field scanning optical microscope"Applied Physic Letters. 83. 2250-2252 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Real-space mapping of exciton wavefunctio in aGaAs quantum dot by near-field optical imaging spectroscopy"Physica Status Solidi (b). 238. 235-238 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Near-field photoluminescence imaging of single semiconductor quantum constituents with a spatial resolution of 30 nm"Applied Physic Letters. 81. 141-143 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Kanemitsu et al.: "Photoluminescence spectrum of highly excited single CdS nanocrystals studied by a scanning near-field optical microscope"Applied Physics Letters. 81. 141-143 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Kanemitsu et al.: "Photoluminescence spectrum and dynamics of single CdS nanocrystals studied by scanning near-field optical microscopy"Phys.State Solidi (c). 190. 537-539 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nomura et al.: "Near-field scanning optical microscopy of quantum dot arrays"Japanese Journal of Applied Physics. 41. 2668-2670 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Near-field photoluminescence study of GaNAs alloy epilayer at room temperature and cryogenic temperature"Applied Physic Letters. 78. 1508-1510 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Ikeda et al.: "Near-field spectroscopy of single quantum dots at room temperature"Journal of Microscopy. 202. 209-211 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Homogeneous linewidth broadening in a In0.5Ga0.5As/GaAs single quantum dot at room temperature investigated using a highly sensitive near-field scanning optical microscope"Physical Review B. 63. 121304(R)-1-121304(R)-4 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Ando et al.: "Sharp photoluminescence of CdS nanocrystals in Al2O3 matrices formed by sequential ion implantation"Applied Physic Letters. 79. 539-541 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Takahashi et al.: "Observation of compositional fluctuations in GaNAs alloys grown by metalorganic vapor-phase epitaxy"Journal of Crystal Growth. 221. 461-466 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 斎木敏治他: "ナノの光によって電子の波を操る"化学. 58. 30-33 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 松田一成他: "近接場光学顕微鏡の高分解能化とナノイメージング分光への応用"光アライアンス. 14. 15-20 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 斎木敏治他: "近接場ナノイメージング分光技術の高分解能化とアクティブ操作"まてりあ. 41. 189-193 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 松田一成他: "近接場光学顕微鏡によるナノイメージング分光計測"材料科学. 39. 189-193 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 松田一成他: "高分解能近接場光学顕微鏡による単一半導体量子構造イメージング/分光の新展開"光学. 31. 732-737 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 松田一成他: "ナノ光工学ハンドブック"朝倉書店. 583 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki, S.Nomura, Y.Aoyagi: "Near-field photoluminescence imaging spectroscopy of an n-type modulation-doped quantum well with lateral periodic potentia"Nanotechnology. 15. S345-S348 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Saiki, K.Matsuda, T.Saiki, S.Nomura, M.Mihara, Y.Aoyagi, S.Nair, T.Takagahara: "Nano-optical probing of exciton wave functions confined in a GaAs quantum do"Applied Physics Letters. (in printing). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki, S.Nomura, M.Mihara, Y.Aoyagi, S.Nair, T.Takagahara: "Near-field optical mapping of exciton wave functions in a GaAs quantum do"Physical Review Letters. 91. 177401-1-17401-4 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, K.Ikeda, T.Saiki, H.Saito, K.Nishi: "Carrier-carrier interaction in single InGaAs quantum dots room temperature investigated by near-field scanning optical microscope"Applied Physics Letters. 83. 2250-2252 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki, S.Nomura, M.Mihara, Y.Aoyagi: "Real-space mapping of exciton wave function in GaAs quantum dot by near-field imaging spectroscopy"Physica Status Solidi (b). 238, No.2. 235-238 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki S.Nomura, M.Mihara, Y.Aoyagi: "Near-field photoluminescence imaging of single semiconductor quantum constituents with a spatial resolution of 30 nm"Applied Physics Letters. 81. 2291-2293 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Kanemitsu, T.Inagaki, M.Ando, K.Matsuda, T.Saiki, C.W.White: "Photoluminescence spectrum of highly excited single CdS nanocrystals studied by a scanning near-field optical microscope"Applied Physics Letters. 81. 141-143 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Kanemitsu, M.Ando, K.Matsuda, T.Saiki, C.W.White: "Photoluminescence spectrum and dynamics of single CdS nanocrystals studied by scanning near-field optical microscopy"Phys.State Solidi (c). 190. 537-539 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nomura, K.Matsuda, T.Saiki, Y.Aoyagi: "Near-field scanning optical microscopy of quantum dot arrays"Japanese Journal of Applied Physics. 41. 2668-2670 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki, M.Takahashi, A.Moto, S.Takagishi: "Near-field photoluminescence study of GaNAs epilayer at room and cryogenic temperature"Applied Physics Letters. 78. (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Ikeda, K.Matsuda, H.Saito, K.Nishi, T.Saiki: "Near-field spectroscopy of single quantum dots at room temperature"Journal of Microscopy. 202. 209-211 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, K.Ikeda, T.Saiki, H.Tsuchiya, H.Saito, K.Nishi: "Homogeneous linewidth broadening in a In0.5Ga0.5 As/GaAs single quantum dot at room temperature investigated using a highly sensitive near-field scanning optical microscope"Physical Review B. 63. 121304(R)1-121304(R)-4 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Ando, Y.Kanemitsu, T.Kushida, K.Matsuda, T.Saiki, C.W.White: "Sharp photoluminescence of CdS nanocrystals in A12O3 matrices formed by sequential ion implantation"Applied Physics Letters. 79. 539-541 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Takahashi, A.Moto, S.Tanaka, T.Tanabe, S.Takagishi, K.Karatani, M.Nakayama, K.Matsuda, T.Saiki: "Observation of compositional fluctuations in GaN As alloys grown by metalorganic vapor-phase epitaxy"Journal of Crystal Growth. 221. 461-466 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Saiki, K.Matsuda: "Electron wave manipulation by nano-scale light"Kagaku. Vol.58, No.10. 30-33 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki: "High resolution near-field scanning optical microscope and its application to nanoimaging spaectrsocpy"Hikararaiansu. Vol.14, No.11. 15-20 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki: "A single semiconductor quantum constituent imaging/spectrosopcy by high resolution near-field scanning optical microscope"Kougaku. Vol.31, No.10. 732-737 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Saiki, K.Matsuda, N.Hosaka: "Optical near-field imaging technique for high spatial resolution and active manipulation"Materia. Vol.41, No.9. 610-615 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki: "Nano-imaging optical measurement by near-field scanning optical microscope"Zairyokagaku. 39. 189-193 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda, T.Saiki: "Low temperature technique"Handbook of Nano optics engineering (Asakura). 246-252 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Matsuda et al.: "Carrier-carrier interaction in single InGaAs quantum dots at room temperature in vestigated by near-field scanning optical microscope"Applied Physics Letters. 83. 2250-2252 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Matsuda et al.: "Near-field optical mapping of exciton wave functions in a GaAs quantum dot"Physical Review Letters. 91. 177401-1-177401-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Matsuda et al.: "Near-field photoluminescence imaging spectroscopy of an n-type modulation-doped quantum well with lateral periodic potential"Nanotechnology in printing. (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Matsuda et al.: "Real-space mapping of exciton wave function in GaAs quantum dot by near-field imaging spectroscopy"Physica Status Solidi. 238,2. 235-238 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 松田一成 他: "近接場光学顕微鏡の高分解能化とナノイメージング分光への応用"光アライアンス. 14,11. 15-20 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 斎木敏治 他: "ナノの光によって電子の波を操る"化学. 58,10. 30-33 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 松田一成 他: "光で見る半導体量子ドット中の波動関数"パリティ. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Matsuda et al.: "Near-field photoluminescence imaging of a single semiconductor quantum dot with a high spatial resolution of 30 nm"Applied Physics Letters. 81. 2291-2293 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Kanemitsu et al.: "Photoluminescence spectrum of highly excited single CdS nanocrystals"Applied Physics Letters. 81. 141-143 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Kanemitsu et al.: "Photoluminescence spectrum and dynamics of single CdS nanocrystal studied by scanning near-field optical microscopy"phys. state solidi. 190. 537-539 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] 松田一成 他: "高分解能近接場光学顕微鏡による単一半導体量子構造イメージング/分光の新展開"日本光学会誌. 32. 732-737 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] 松田一成 他: "近接場光学顕微鏡によるナノイメージング分光計測"材料科学. 39. 189-193 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Matsuda et al.: "Near-field photoluminescence study of GaNAs epilayer at room and cryogenic temperature"Applied Physics Letters. 79. 1508-1511 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Ando et al.: "Sharp photoluminescence of CdS nanocrystals in Al_2O_3 Matrices formed by sequential ion implantation"Applied.Physics.Letters. 79. 539-541 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Kanemitsu et al.: "Photoluminescence spectrum and dynamics of single CdS nanocrystal studied by scanning near-field optical microscopy"phys.state solidi. (in print).

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Ikeda et al.: "Near-field spectroscopy of single quantum dots at room temperature"Journal of Microscopy. 202. 209-211 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Matsuda et al.: "Homogeneous linewidth broadening in a InGaAs/GaAs single quantum dot at room temperature investigated using a highly sensitive near-field scanning optical microscope"Physical Review B. 63. 12304(R)1-12304(R)4 (2001)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2020-05-15  

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