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Spatial and temporal spectroscopy of the luminescence generated by hot carriers in narrow-gap-semiconductor quantum dots

Research Project

Project/Area Number 14350355
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionToyo University

Principal Investigator

WADA Noboru  Toyo University, Engineering, Professor, 工学部, 教授 (40256772)

Co-Investigator(Kenkyū-buntansha) HANAJIRI Tatsuro  Toyo University, Engineering, Associate Professor, 工学部, 助教授 (30266994)
TOYABE Tohru  Toyo University, Engineering, Professor, 工学部, 教授 (20266993)
ISHIBASI Kouji  RIKEN, Full time researcher, 理化学研究所, 専任研究員 (30211048)
Project Period (FY) 2002 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥6,500,000 (Direct Cost: ¥6,500,000)
Fiscal Year 2004: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 2003: ¥1,300,000 (Direct Cost: ¥1,300,000)
Fiscal Year 2002: ¥3,800,000 (Direct Cost: ¥3,800,000)
Keywordsnarrow-gap semiconductor / hot carrier / luminescence spectroscopy / nanowires / InAs / InSb / quantum dot / hot luminescence / 近接場ナノフォトニクス / 量子細線 / 微小ギャップ半導
Research Abstract

The dynamics of hot carriers in semiconductors has been an intensive research subject for some decades. From a fundamental point of view, the behavior of highly excited, almost free carriers and their interactions with other carriers, phonons, photons and so on is of great interest. Application-wise, understanding the hot carrier dynamics is essential in advancing nano-scale semiconductor devices, where a small voltage easily generates hot carriers in nano-scale dimensions. Intense femto-second laser pulses (λ=780 nm) were used to generate hot carriers in bulk InAs, where not only Stokes luminescence, but also surprisingly strong anti-Stokes luminescence were observed. Moreover, a periodic intensity variation found in the anti-Stokes spectrum was found and may be attributed to two-LO-phonon cascade emission by the hot carriers. Hot carries produced in two-photon absorption process may generate several pairs of LO phonons before they emit a photon by recombination.
The luminescence spatial extent was also probed in InAs and InSb. It was several times larger than the laser spot size (〜2 μ m). Our results suggest that hot carriers in the narrow-gap semiconductors may travel ballistically over a surprisingly long distance. It is also noted that the luminescence intensity exhibited large non-linearity with the excitation laser energy.
In addition, fabrication of the double structured (core-shell and axial superlattice) nanowires with some dots was conducted with FIB apparatus and a furnace. The double structured nanowires consist of crystalline InSb and In_2O_3. The method is simple and can be used to mass-produce compound semiconductor nanowires. Manipulation of Ga-ion beams in nanoscale may enable us to fabricate nanoelectronics devices and nanophotodevices. The detailed conditions and mechanism for creating such novel nanostructures are not clear at this time, but we hope these findings may invoke more interests in compound semiconductor nanowire research.

Report

(4 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • Research Products

    (9 results)

All 2005 2004 Other

All Journal Article (8 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] 酸化インジウムナノ細線の構造解析及び電気抵抗測定2005

    • Author(s)
      石塚雅朗, 和田昇
    • Journal Title

      日本物理学会講演概要集 第60巻第1号第4分冊

      Pages: 643-643

    • Related Report
      2004 Annual Research Report
  • [Journal Article] FIBを用いた化合物半導体量子細線の自己形成による生成2005

    • Author(s)
      堀内照正, 和田昇
    • Journal Title

      第5回工業技術研究所講演会予稿集 2005年2月24日、東洋大学

      Pages: 39-40

    • Related Report
      2004 Annual Research Report
  • [Journal Article] InSb量子細線の作成とその電気伝特性2004

    • Author(s)
      山本健仁, 和田昇, 中島義賢, 花尻達郎
    • Journal Title

      日本物理学会講演概要集 第59巻第1号第4分冊

      Pages: 693-693

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 自己形成成長によるInSb量子ドット、量子細線の作成2004

    • Author(s)
      石塚雅朗, 和田昇
    • Journal Title

      日本物理学会講演概要集 第59巻第1号第4分冊

      Pages: 693-693

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 集束イオンビーム装置で加工したSi基板上へのInSb量子ドット作製2004

    • Author(s)
      石塚雅朗, 和田昇, 中島義賢, 花尻達郎
    • Journal Title

      第3回工業技術研究所講演会予稿集 2004年2月26日、東洋大学

      Pages: 145-146

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Anti-Stokes and Stokes Hot Luminescence from Bulk InAs and InSb

    • Author(s)
      N.Wada, A.C.H.Rowe, S.A.Solin
    • Journal Title

      Proceedings of the 27^<th> International Conference on the Physics of Semiconductors (published by AIP) (In press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Anti-Stokes and Stokes Hot Luminescence from Bulk InAs and InSb

    • Author(s)
      N.Wada, A.C.H.Rowe, S.A.Solin
    • Journal Title

      Proceedings of the 27^<th> International Conference on the Physics of Semiconductors (AIP) (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Anti-Stokes and Stokes Hot Luminescence from Bulk InAs and InSb

    • Author(s)
      Noboru Wada, A.C.H.Rowe, S.A.Solin
    • Journal Title

      Proceedings of the 27^<th> International Conference on the Physics of Semiconductors (published by AIP) (in press)

      Pages: 2-2

    • Related Report
      2004 Annual Research Report
  • [Patent(Industrial Property Rights)] 特許2004

    • Inventor(s)
      和田昇, 石塚雅朗
    • Industrial Property Rights Holder
      東洋大
    • Filing Date
      2004-02-27
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary

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Published: 2002-04-01   Modified: 2016-04-21  

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