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Study on Accumulation and Transportation of Refractory Organic Materials in Terrestrial Area

Research Project

Project/Area Number 15310002
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionHOKKAIDO UNIVERSITY

Principal Investigator

NAGAO Seiya  Hokkaido Univ., Fac.of Environ.Earth Sci., Asso.Prof., 大学院・地球環境科学研究院, 助教授 (20343014)

Co-Investigator(Kenkyū-buntansha) YAMAMOTO Masanobu  Hokkaido Univ., Fac.of Environ.Earth Sci., Asso.Prof., 大学院・地球環境科学研究院, 助教授 (60332475)
FUJITAKE Nobuhide  Kobe Univ., Fac.of Agr., Asso.Prof., 農学部, 助教授 (50243332)
IRINO Tomohisa  Hokkaido Univ., Fac.of Environ.Earth Sci., Inst., 大学院・地球環境科学研究院, 助手 (70332476)
KODAMA Hiroki  Kyoto Pref.Univ., Fac.of Agr., Inst., 農学部, 助手 (60305563)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥15,500,000 (Direct Cost: ¥15,500,000)
Fiscal Year 2005: ¥2,400,000 (Direct Cost: ¥2,400,000)
Fiscal Year 2004: ¥4,200,000 (Direct Cost: ¥4,200,000)
Fiscal Year 2003: ¥8,900,000 (Direct Cost: ¥8,900,000)
KeywordsRiver / Dissolved organic matter / Suspended solids / Carbon Cycle / Carbon isotopes / Humic substances / Radiocarbon / Snow melt / 粒子態有機物 / 土壌有機物 / 降雨 / 難分解性有機物 / フミン酸 / フルボ酸 / 溶存有機炭素 / 河川水 / 移行動態
Research Abstract

An important part of global organic carbon cycle is the flux of terrestrial organic carbon from the continents to the oceans. The potential importance of coastal systems in global and regional organic budgets is still unclear because of the inherent complexity and variability of rivers, estuaries and coastal zones. Therefore, it is important to understand the organic matter cycling in estuaries and coastal systems, especially characteristics and dynamics of river DOM and POM. But the DOM and POM is not homogeneous in terms of size or chemical characteristics so that we can't evaluate the linkage of terrestrial and coastal environments. The objective of this study is to understand the transport behavior of dissolved and particulate organic matter from terrestrial region to ocean. This study used carbon isotopic ratios (Δ^<14>C and δ^<13>C values) as tracers of organic carbon because the simultaneous use of these values adds a second dimension to isotopic studies of carbon cycling in surface aquatic environments.
Refractory organic materials, humic substances, were isolated from the river waters in Scotland, Ukraine, Japan and Indonesia by the XAD extraction. The Δ^<14>C values of dissolved humic substances ranged from -316‰ to +209‰, indicating spatial and temporal distribution.
To understand transport of POM in river systems, we selected three river systems (Tokachi, Ishikari and Kuji River systems) with different watershed conditions and carried out the observation at a fixed point in each river. The Δ^<14>C values range from -111 to -286‰ for the Tokachi River in northeast Hokkaido, -103〜-364‰ for the Ishikari River in southeast Hokkaido and -18.7〜-94.4‰ for the Kuji River in Kanto area in Japan. The paired Δ^<14>C vs. δ^<13>C distributions vary with rivers and seasons. These results suggest that the difference in paired Δ^<14>C vs. δ^<13>C distributions may reflect the water discharge and watershed environments.

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (24 results)

All 2006 2005 2004 2003 Other

All Journal Article (18 results) Book (1 results) Publications (5 results)

  • [Journal Article] Distribution and sources of organic matter in surface sediments on the shelf and slope off Tokachi,western North Pacific,inferred from C and N stable isotopes and C/N ratios2006

    • Author(s)
      T.Usui et al.
    • Journal Title

      Marine Chemistry 98

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Effects of operational conditions for extraction and sample storage on the structural properties of water-extractable humic substances in soil2006

    • Author(s)
      D.Asakawa et al.
    • Journal Title

      Humic Substances Research (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Changes in elemental composition,molecular weight,and 1HNMR spectrum of water-extractable hydrophobic acids in Cambisols with season and soil depth2006

    • Author(s)
      D.Asakawa et al.
    • Journal Title

      Soil Science Plant Nutrition (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Distribution and sources of organic matter in surface sediments on the shelf and slope off Tokachi, western North Pacific, inferred from C and N stable isotopes and C/N ratios2006

    • Author(s)
      T.Usui et al.
    • Journal Title

      Marine Chemistry 98

      Pages: 241-259

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Distribution and sources of organic matter in surficial sediments on the shelf and slope off Tokachi, western North Pacific, inferred from C and N stable isotopes and C/N ratios2006

    • Author(s)
      T.Usui, S.Nagao, M.Yamamoto, K.Suzuki, I.Kudo, S.Montani, A.Noda, M.Minagawa
    • Journal Title

      Marine Chemistry 98

      Pages: 241-259

    • NAID

      120000955221

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Combined use of Δ^<14>C and δ^<13>C values to trace transportation and deposition processes of terrestrial particulate organic matter in coastal marine environments2005

    • Author(s)
      Nagao et al.
    • Journal Title

      Chemical Geology 218

      Pages: 63-72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Combined use of Δ14C and d13C values to trace transportation and deposition processes of terrestrial particulate organic matter in coastal marine environments2005

    • Author(s)
      Nagao et al.
    • Journal Title

      Chemical Geology 218

      Pages: 63-72

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Combined use of delta C-14 and delta C-13 values to trace transportation and deposition processes of terrestrial particulate organic matter in coastal marine environments2005

    • Author(s)
      S.Nagao, T.Usui, M.Yamamoto, M.Minagawa, T.Iwatsuki, A, Noda
    • Journal Title

      Chemical Geology 218

      Pages: 63-72

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 水中腐植物質の溶存形態解析2004

    • Author(s)
      長尾 誠也
    • Journal Title

      日本水環境学誌 27・2

      Pages: 92-95

    • NAID

      10012049441

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Radiocarbon of dissolved humic substances in river waters from the Chernobyl area2004

    • Author(s)
      S.Nagao et al.
    • Journal Title

      Nuclear Instruments and Method B 223-224

      Pages: 848-853

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Association of dissolved radionuclides released by the Chernobyl accident with colloidal materials in surface water2004

    • Author(s)
      T.Matsunaga et al.
    • Journal Title

      Applied Geochemistry 19

      Pages: 1581-1599

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Analysis of dissolved forms and characteristics of humic substances (in Japanese)2004

    • Author(s)
      S.Nagao
    • Journal Title

      Journal of Japan Society on Water Environment 27

      Pages: 92-95

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Characteristics of humic substances in the Kuji River waters as determined by high-performance size exclusion chromatography with fluorescence detection2003

    • Author(s)
      S.Nagao et al.
    • Journal Title

      Water Research 37

      Pages: 4159-4170

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] 環境中での腐植物質の存在意義とその機能2003

    • Author(s)
      長尾 誠也
    • Journal Title

      日本土壌肥料学雑誌 74・3

      Pages: 371-376

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Recent trend and view of studies on humic substances in Japan (in Japanese)2003

    • Author(s)
      S.Nagao
    • Journal Title

      Journal of Soil Science and Plant Nutrition 74

      Pages: 371-376

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Effects of operational conditions for extraction and sample storage on the structural properties of water-extractable humic substances in soil

    • Author(s)
      D.Asakawa et al.
    • Journal Title

      Humic Substances Research (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Changes in elemental composition, molecular weight, and 1H NMR spectrum of water-extractble hudrophobic acids in cambisols with season and soil depth

    • Author(s)
      D.Asakawa et al.
    • Journal Title

      Soil Science Plant Nutrition (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Combined use of delta 14C and delta 13C values to trace transportation and deposition processes of terrestial

    • Author(s)
      S.Nagao et al.
    • Journal Title

      Chemical Geology (印刷中)

    • Related Report
      2004 Annual Research Report
  • [Book] 水の分析2005

    • Author(s)
      長尾誠也(分担執筆)
    • Total Pages
      472
    • Publisher
      化学同人
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Publications] S.Nagao et al.: "Characteristics of humic substances in the Kuji River waters as determined by high-performance size exclusion chromatography with fluorescence detection"Water Research. 37. 4159-4170 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 長尾 誠也: "環境中での腐植物質の存在意義とその機能"日本土壌肥料学雑誌. 74・3. 371-376 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 長尾 誠也: "水中腐植物質の溶存形態解析"日本水環境学誌. 27・2. 92-95 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Nagao et al.: "Radiocarbon of dissolved the humic substances in river waters from Chernobyl area"Nuclear Instruments and Method B. (in print).

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Matsunaga, S.Nagao et al.: "Association of dissolved radionuclides released by the Chernobyl accident with colloidal materials in surface water"Applied Geochemistry. (in print).

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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