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Quantum Manipulation of Nuclear Spin of Ortho-H2 Molecule in Solid Hydrogen

Research Project

Project/Area Number 15340131
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 原子・分子・量子エレクトロニクス・プラズマ
Research InstitutionThe University of Electro-Communications

Principal Investigator

HAKUTA Kohzo  UEC, Faculty of Electro-Communications, Professor, 電気通信学部, 教授 (80164771)

Co-Investigator(Kenkyū-buntansha) SUZUKI Masaru  UEC, Faculty of Electro-Communications, Professor, 電気通信学部, 教授 (20196869)
KATSURAGAWA Masayuki  UEC, Faculty of Eelctro-Communications, Associate Professor, 電気通信学部, 助教授 (10251711)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥16,500,000 (Direct Cost: ¥16,500,000)
Fiscal Year 2005: ¥4,000,000 (Direct Cost: ¥4,000,000)
Fiscal Year 2004: ¥4,800,000 (Direct Cost: ¥4,800,000)
Fiscal Year 2003: ¥7,700,000 (Direct Cost: ¥7,700,000)
KeywordsSolid Hydrogen / Nuclear Spin / Quantum Coherence / Near Field / Optical Nanofiber / ナノファイバー / 超微細光ファイバー / 極細光ファイバー
Research Abstract

We carried out the researches to establish a basis for manipulating nuclear-spin quantum-coherence of ortho-hydrogen molecule in solid hydrogen. Simultaneously, we developed a method to manipulate optical processes using optical nanofiber ; it was originally proposed to introduce a strong light into the solid hydrogen.
Regarding the ortho-hydrogen project, we developed a highly-stable single-frequency cw laser at 2.4 μm wavelength using doubly-resonant OPO-technique. Ortho-hydrogen infrared transition (v=1-0, J=1-1) was measured systematically. We showed that the transition reveals an ultra-narrow spectral width of 1.6 MHz HWHM. This width is the narrowest width observed just using simple absorption spectroscopy, without using any nonlinear laser-spectroscopic method. Although density of ortho-hydrogen is very low 40 ppm, the peak absorption of 1-cm solid hydrogen crystal reaches to 60% ; it is due to the ultra-narrow spectral feature. We demonstrated also that the vibration-rotation sp … More ectrum splits into three components with splittings of about 10 MHz. The origin of the splitting may be understood due to breaking of magnetic degeneracy of J=1 state into three sublevels via crystal field. The observations have demonstrated that the ortho-hydrogen embedded in solid-parahydrogen is a unique system for realizing quantum coherence control in solid. The observed degeneracy breaking may open a new possibility to realize a new Raman three level scheme without magnetic field.
Regarding the nanofiber, we established a method to produce nanofibers with diameter from 1μm to 400 nm with transmission of 80%. We showed theoretically a unique possibility to develop optical processes using nanofibers, very different from those in free space ; a key point is to confine both optical field and atoms/molecules into a submicron space around a nanofiber. We can manipulate single atom/molecule transition just using single photon. Moreover, spontaneous emission of atom/molecule near the nanofiber is strongly modified to emit photons into a guided mode of a nanofiber. We have observed experimentally the unique features of confinement in February of 2006. The observations imply that the nanofiber technique may open a new category of quantum optics. Less

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (51 results)

All 2006 2005 2004 2003 Other

All Journal Article (40 results) Book (4 results) Publications (7 results)

  • [Journal Article] Scattering of an evanescent probe light field on a single cesium atom near a nanofiber2006

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Physical Review A 73

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Scattering of an evanescent probe light field on a single cesium atom near a nanofiber2006

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Physical Review A Vol.73

      Pages: 13819-13819

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Nanofiber-mediated radiative transfer between teo distant atoms2005

    • Author(s)
      Fam Le Kien, S.Dutta Gupta, K.P.Nayak, K.Hakuta
    • Journal Title

      Physical Review A 72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spontaneous emission of cesium atom near a subwavelength-diameter fiber2005

    • Author(s)
      Fam Le Kien, S.Dutta Gupta, V.I.Balykin, K.Hakuta
    • Journal Title

      Physical Review A 72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Manipulating Light with Quantum Coherence in Solid Hydrogen2005

    • Author(s)
      K.Hakuta
    • Journal Title

      Advances in Phtonics and Applications IWPA2004

      Pages: 36-42

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] State insensitive trapping and guiding of Cesium atoms using a two-color evanescent field around a sub-wavelength diameter fiber2005

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 910-917

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Nanofiber-mediated radiative transfer between two distant atoms2005

    • Author(s)
      Fam Le Kien, S.Dutta Guta, K.P.Nayak, K.Hakuta
    • Journal Title

      Physical Review A Vol.72

      Pages: 63815-63815

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spontaneous emission of cesium atom near a subwavelength-diameter fiber2005

    • Author(s)
      Fam Le Kien, S.Dutta Gupta, V.I.Balykin, K.Hakuta
    • Journal Title

      Physical Review A Vol.72

      Pages: 32509-32509

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] State insensitive trapping and guiding of Cesium atoms using a two-color evanescent field around a sub-wavelength diameter fiber2005

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Journal of the Physical Society of Japan Vol.74

      Pages: 910-917

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Manipulating Light with Quantum Coherence in Solid Hydrogen2005

    • Author(s)
      K.Hakuta
    • Journal Title

      Proceedings of the International Workshop on Photonica and Applications, Hanoi, Vietnam, published in March

      Pages: 36-42

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Nanofiber-mediated radiative transfer between two distant atoms2005

    • Author(s)
      Fam Le Kien, S.Dutta Gupta, K.P.Nayak, K.Hakuta
    • Journal Title

      Physical Review A 72

    • Related Report
      2005 Annual Research Report
  • [Journal Article] State insensitive trapping and guiding of Cesium atoms using a two-color evanescent field around a sub-wavelength diameter fiber2005

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Journal of the Physical Society of Japan (in press)

      Pages: 910-917

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Manipulating Light with Quantum Coherence in Solid Hydrogen2005

    • Author(s)
      K.Hakuta
    • Journal Title

      Proceeding of the International Workshop on Photonics and Applications (in press)

      Pages: 36-42

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Pbservation of multiorder coherent Raman sidebands in solid hydrogen film2004

    • Author(s)
      Geon Joon Lee, K.Hara, M.Katsuragawa, K.Hakuta
    • Journal Title

      Journal of the Physical Society of Japan 45

      Pages: 75-79

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Atom trap and waveguide using a two-color evanescent light field around a subwavelength-diameter optical fiber2004

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Physical Review A 70

      Pages: 63403-63403

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Field intensity distribution and polarization orientration in a vacuum-clad subwavelength-diameter optical fiber2004

    • Author(s)
      Fam Le Kien, J.Q.Liang, K.Hakuta, V.I.Balykin
    • Journal Title

      Optics Communications 242

      Pages: 445-455

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Atom trapping and guiding with a subwavelength-diameter optical fiber2004

    • Author(s)
      V.I.Balykin, K.Hakuta, Fam Le Kien, J.Q.Liang, M.Morinaga
    • Journal Title

      Physical Review A 70

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] 電気通信大学の21世紀COEプログラム「コヒーレント光科学の展開」2004

    • Author(s)
      白田耕蔵
    • Journal Title

      電気通信大学紀要 16

      Pages: 95-98

    • NAID

      120006315558

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Resonantly enhanced four-wave mixing in a modified double-A scheme : Effect of the decay of the upper level2004

    • Author(s)
      Fam Le Kien, K.Hakuta
    • Journal Title

      Physical Review A 69

      Pages: 43811-43811

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Manipulating the retrieval of the stored light pulses2004

    • Author(s)
      A.K.Patnaik, Fam Le Kien, K.Hakuta
    • Journal Title

      Physical Review A 69

      Pages: 35803-35803

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Nonlinear frequency conversion by Raman coherence prepared in solid hydrogen film2004

    • Author(s)
      Geon Joon Lee, K.Hara, M.Katsuragawa, K.Hakuta
    • Journal Title

      Journal of Nonlinear Optical Physics & Materials Vol.13(3-4)

      Pages: 433-437

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Atom trap and waveguide using a two-color evanescent light field around a subwavelength-diameter optical fiber2004

    • Author(s)
      Fam Le Kien, V.I.Balykin, K.Hakuta
    • Journal Title

      Phys.Rev.A, LANL Archives, quant-ph/047107 Vol.70

      Pages: 63403-63403

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Field intensity distribution and polarization orientation in a vacuum-clad subwavelength-diameter optical fiber2004

    • Author(s)
      Fam Le Kien, J.Q.Liang, K.Hakuta, V.I.Balykin
    • Journal Title

      Optics Communications Vol.242,Issues4-6,8Pages

      Pages: 445-455

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Observation of multiorder coherent Raman sidebands in solid hydrogen film2004

    • Author(s)
      Geon Joon Lee, K.Hara, M.Katsuragawa, K.Hakuta
    • Journal Title

      Journal of the Korean Physical Society vol.45,no.1

      Pages: 75-79

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Atom trapping and guiding with a subwavelength-diameter optical fiber2004

    • Author(s)
      V.I.Balykin, K.Hakuta, Fam Le Kien, J.Q.Liang, M.Morinaga
    • Journal Title

      Physical Review A Vol.70

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Resonantly enhanced four-wave mixing in a modified double-Λ scheme : Effect of the decay of the upper level2004

    • Author(s)
      Fam Le Kien, K.Hakuta
    • Journal Title

      Physical Review A Vol.69

      Pages: 43811-43811

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Manipulating the retrieval of the stored light pulses2004

    • Author(s)
      A.K.Patnaik, Fam Le Kien, K.Hakuta
    • Journal Title

      Physical Review A Vol.69

      Pages: 35803-35803

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Observation of multiorder coherent Raman sidebands in solid hydrogen film2004

    • Author(s)
      Geon Joon Lee, K.Hara, M.Katsuragawa, K.Hakuta
    • Journal Title

      Journal of the Korean Physical Society 45

      Pages: 75-79

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Field intensity distribution and polarization orientation in a vacuum-clad subwavelength-diameter optical fiber2004

    • Author(s)
      Fam Le Kien, J.Q.Liang, K.Hakuta, V.I.Balykin
    • Journal Title

      Optics Communications 242

      Pages: 445-455

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 電気通信大学の21世紀COEプログラム「コヒーレント光科学の展開」2004

    • Author(s)
      白田耕藏
    • Journal Title

      電気通信大学紀要 16

      Pages: 95-98

    • NAID

      120006315558

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Resonantly enhanced four-wave mixing in a modified double-Λ scheme : Effect of the decay of the upper level2004

    • Author(s)
      Fam Le Kien, K.Hakuta
    • Journal Title

      Physical Review A 69

      Pages: 43811-43811

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Stimulated Raman scattering in vapor-deposited hydrogen film2003

    • Author(s)
      G.J.Lee, K.HARA, M.Katsuragawa, K.Hakuta
    • Journal Title

      Japanese Journal of Applied Physics 42

      Pages: 6450-3

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Multiorder coherent Raman scattering of a quantum probe field2003

    • Author(s)
      Fam Le Kien, A.K.Patnaik, K.Hakuta
    • Journal Title

      Physical Review A 68

      Pages: 63803-63803

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Engineering the dispersion of a fiber mode via molecular coherence2003

    • Author(s)
      A.K.Patnaik, J.Q.Liang, K.Hakuta
    • Journal Title

      Journal of Modern Optics 50

      Pages: 2595-2604

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Parametric beating of a quantum probe field with a prepared Raman coherence2003

    • Author(s)
      Fam Le Kien, K.Hakuta
    • Journal Title

      Physical Review A 67

      Pages: 33808-33808

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Temperature dependence of the Raman shift and width of solid paratydrogen : Effect of vibron-phonon scattering2003

    • Author(s)
      Fam Le Kien, A.Koreeda, K.Kuroda, M.Suzuki, K.Hakuta
    • Journal Title

      Japanese Journal of Applied Physics 42

      Pages: 3483-3489

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Stimulated Raman scattering in vapor-deposited solid hydrogen film2003

    • Author(s)
      G.J.Lee, K.Hara, M.Katsuragawa, K.Hakuta
    • Journal Title

      Japanese Journal of Applied Physics Vol.42

      Pages: 6450-6453

    • NAID

      10012449152

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Multiorder coherent Raman scattering of a quantum probe field2003

    • Author(s)
      Fam Le Kien, A.K.Patnaik, K.Hakuta
    • Journal Title

      Physical Review A Vol.68

      Pages: 63803-63803

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Engineering the dispersion of a fiber mode via molecular coherence2003

    • Author(s)
      A.K.Patnaik, J.Q.Liang, K.Hakuta
    • Journal Title

      Journal of Modern Optics Vol.50

      Pages: 2595-2604

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Parametric beating of a quantum probe field with a prepared Raman coherence2003

    • Author(s)
      Fam Le kien, K.Hakuta
    • Journal Title

      Physical Reiveiw A Vol.67

      Pages: 33808-33808

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Book] "量子干渉と量子コヒーレンス"、「光科学研究の最前線」2005

    • Author(s)
      白田耕蔵
    • Publisher
      強光子場科学研究懇談会
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Book] "光の自然放出と誘導放出、そして光応答の操作と制御"、「アインシュタインと21世紀の物理学」(日本物理学会編)2005

    • Author(s)
      白田耕蔵
    • Publisher
      日本評論社
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Book] "量子干渉と量子コヒーレンス"、光科学研究の最前線2005

    • Author(s)
      白田耕蔵
    • Publisher
      強光子場科学研究懇談会
    • Related Report
      2005 Annual Research Report
  • [Book] "光の自然放出と誘導放出、そして光応答の操作と制御"、アインシュタインと21世紀の物理学(日本物理学会編)2005

    • Author(s)
      白田耕蔵
    • Publisher
      日本評論社
    • Related Report
      2005 Annual Research Report
  • [Publications] Fam Le Kien, K.Hakuta: "Resonantly enhanced four-wave mixing in a modified double-Λ scheme : Effect of the decay of the upper level"Physical Review A. (in press).

    • Related Report
      2003 Annual Research Report
  • [Publications] G.J.Lee, K.Hara, M.Katsuragawa, K.Hakuta: "Stimulated Raman scattering in vapor-deposited solid hydrogen film"Japanese Journal of Applied Physics. 42. 6450-6453 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.K.Patnaik, Fam Le Kien, K.Hakuta: "Manipulating the retrieval of the stored light pulses"Physical Review A. (in press).

    • Related Report
      2003 Annual Research Report
  • [Publications] Fam Le Kien, A.K.Patnaik, K.Hakuta: "Multiorder coherent Raman scattering of a quantum probe field"Physical Review A. 68. 063803 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.K.Patnaik, J.Q.Liang, K.Hakuta: "Engineering the dispersion of a fiber mode via molecular coherence"Journal of Modern Optics. 50. 2595-2604 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Fam Le Kien, K.Hakuta: "Parametric beating of a quantum probe field with a prepared Raman coherence"Physical Review A. 67. 033808 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Fam Le Kien, A.Koreeda, K.Kuroda, M.Suzuki, K.Hakuta: "Temperature dependence of the Raman shift and width of solid parahydrogen : Effect of vibron-phonon scattering"Japanese Journal of Applied Physics. 42. 3483-3489 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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