Study on novel magnetic order and transport properties in pyrochlore iridium oxides
Project/Area Number |
15H03692
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Research Category |
Grant-in-Aid for Scientific Research (B)
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Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Condensed matter physics II
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Research Institution | Kyushu Institute of Technology |
Principal Investigator |
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Co-Investigator(Kenkyū-buntansha) |
富安 啓輔 株式会社日産アーク(マテリアル解析部、デバイス機能解析部), マテリアル解析部,デバイス機能解析部, 主任研究員 (20350481)
渡邊 功雄 国立研究開発法人理化学研究所, 仁科加速器科学研究センター, 専任研究員 (40260195)
小野田 繁樹 国立研究開発法人理化学研究所, 開拓研究本部, 専任研究員 (70455335)
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Project Period (FY) |
2015-04-01 – 2019-03-31
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Project Status |
Completed (Fiscal Year 2018)
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Budget Amount *help |
¥16,640,000 (Direct Cost: ¥12,800,000、Indirect Cost: ¥3,840,000)
Fiscal Year 2018: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2017: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2016: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2015: ¥7,280,000 (Direct Cost: ¥5,600,000、Indirect Cost: ¥1,680,000)
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Keywords | パイロクロア / イリジウム酸化物 / 中性子散乱 / ミュオンスピン緩和 / 第一原理電子状態計算 / 金属絶縁体転移 / パイロクロア酸化物 / 磁気構造解析法 / 偏極中性子散乱 / 第一原理計算 / 強相関電子系 / フラストレート系 / パイロクロア型酸化物 / 磁気秩序 / 中性子回折 / パイロクア型酸化物 |
Outline of Final Research Achievements |
The metal-insulator transition of pyrochlore iridates was researched in conjunction with various measurement methods and a theoretical method based on first principles calculation. The magnetic structure of pyrochlore iridates was clarified from polarized neutron diffraction and muon spin relaxation, which can microscopically measure the spin state of electrons. The first-principles calculations on the electronic state revealed that increasing the on-site Coulomb interaction U changes from paramagnetic semimetal to antiferromagnetic semimetal, from antiferromagnetic semimetal to antiferromagnetic insulator.
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Academic Significance and Societal Importance of the Research Achievements |
本研究の学術的な意義は,スピン軌道相互作用が大きい5d遷移金属酸化物であるイリジウム酸化物において,幾何学的なフラストレーションを示すパイロクロア型構造を有する物質の基底状態の磁気構造を実験的に解明することができたことである。また,第一原理電子状態計算からも,実験結果と対応するようにオンサイトクーロン相互作用Uにより基底状態が変化することを理論的に解明したことは,学術的に大きな成果と考えられる。
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Report
(5 results)
Research Products
(93 results)
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[Journal Article] Magnetic Properties of Hole-Doped Pyrochlore Iridate (Y1-x-yCuxCay)2Ir2O72019
Author(s)
Julia Angel, Retno Asih, Hironori Nomura, Tomoya Taniguchi, Kazuyuki Matsuhira, Muhammad Redo Ramadhan, Irwan Ramli, Makoto Wakeshima, Yukio Hinatsu, Mohamed Ismail Mohamed-Ibrahim, Shukri Sulaiman and Isao Watanab
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Journal Title
Key Engineering Materials
Volume: 印刷中
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Quantum paramagnet near spin-state transition2018
Author(s)
K. Tomiyasu, N. Ito, R. Okazaki, Y. Takahashi, M. Onodera, K. Iwasa, T. Nojima, T. Aoyama, K. Ohgushi, Y. Ishikawa, T. Kamiyama, S. Ohira-Kawamura, M. Kofu and S. Ishihara
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Journal Title
Advanced Quantum Technology
Volume: 2018
Issue: 3
Pages: 1800057-1800057
DOI
Related Report
Peer Reviewed / Open Access
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[Journal Article] Excitonic dispersion of the intermediate spin state in LaCoO3 revealed by resonant inelastic x-ray scattering2018
Author(s)
Ru-Pan Wang, Atsushi Hariki, Andrii Sotnikov, Federica Frati, Jun Okamoto, Hsiao-Yu Huang, Amol Singh, Di-Jing Huang, Keisuke Tomiyasu, Chao-Hung Du, Jan Kune?, and Frank M. F. de Groot
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Journal Title
Phys. Rev. B
Volume: 98
Issue: 3
Pages: 35149-35149
DOI
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Chiral-crystal-structure transformations and magnetic states of R3Rh4Sn13 (R=La and Ce)2018
Author(s)
Kazuya Suyama, Kazuaki Iwasa, Yuka Otomo, Keisuke Tomiyasu, Hajime Sagayama, Ryoko Sagayama, Hironori Nakao, Reiji Kumai, Yoshinori Kitajima, Fran?oise Damay, Jean-Michel Mignot, Akira Yamada, Tatsuma D. Matsuda, and Yuji Aoki
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Journal Title
Phys. Rev. B
Volume: 97
Issue: 23
Pages: 231538-231538
DOI
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Magnetic moments and ordered states in pyrochlore iridates Nd2Ir2O7 and Sm2Ir2O7 studied by muon-spin relaxation2017
Author(s)
R. Asih, N. Adam, S. S. M. Tajudin, D. P. Sarid, K. Matsuhira, H. Guo, M. Wakeshima, Y. Hinatsu, T. Nakano, Y. Nozue, S. Sulaiman, M. I. M. Ibrahim, P. K. Biswas, I. Watanabe
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Journal Title
J. Phys. Soc. Jpn.
Volume: 86
Issue: 2
Pages: 0247051-7
DOI
NAID
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Journal Article] Possible Tomonaga-Luttinger spin liquid state in the spin-1/2 inequilateral diamond-chain compound K3Cu3AlO2(SO4)42017
Author(s)
M. Fujihala, H. Koorikawa, S. Mitsuda, K. Morita, T. Tohyama, K. Tomiyasu, A. Koda, H. Okabe, S. Itoh, T. Yokoo, S. Ibuka, M. Tadokoro, M. Itoh, H. Sagayama, R. Kumai, and Y. Murakami
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Journal Title
Scientific Reports
Volume: 7
Issue: 1
DOI
Related Report
Peer Reviewed
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[Journal Article] Coulomb Correlations Intertwined with Spin and Orbital Excitations in LaCoO32017
Author(s)
K. Tomiyasu, J. Okamoto, H. Y. Huang, Z. Y. Chen, E. P. Sinaga, W. B. Wu, Y. Y. Chu, A. Singh, R.-P. Wang, F. M. F. de Groot, A. Chainani, S. Ishihara, C. T. Chen, and D. J. Huang
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Journal Title
Phys. Rev. Lett.
Volume: 119
Issue: 19
DOI
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Microscopic Examinations of Co Valences and Spin States in Electron-Doped LaCoO32016
Author(s)
Keisuke Tomiyasu, Syun-Ichi Koyama, Masanori Watahiki, Mika Sato, Kazuki Nishihara, Yuki Takahashi, Mitsugi Onodera, Kazuaki Iwasa, Tsutomu Nojima, Hiroyuki Nojiri, Jun Okamoto, Di-Jing Huang, Yuuichi Yamasaki, Hironori Nakao, and Youichi Murakami
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Journal Title
Journal of the Physical Society of Japan
Volume: 85
Issue: 9
Pages: 094702-094702
DOI
NAID
Related Report
Peer Reviewed / Int'l Joint Research
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[Presentation] μSR Study on Magnetic Ordering in (Eu,Ca)2Ir2O72019
Author(s)
U. Widyaiswari, J. Angel, H. Nomura, T. Taniguchi, K. Matsuhira, B. Kurniawan, I. Watanabe
Organizer
International Workshop on Topological Quantum Materials, NCKU, Tainan, Taiwan
Related Report
Int'l Joint Research
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[Presentation] Magnetic Properties of Hole-doped Pyrochlore Iridate (Y1-x-yCuxCay)2Ir2O72018
Author(s)
J. Angel, R. Asih, H. Nomura, T. Taniguchi, K. Matsuhira, M. Redo Ramadhan, Irwan Ramli, M. Wakeshima, Y. Hinatsu, M. Ismail Mohamed-Ibrahim, S. Sulaiman, I. Watanabe
Organizer
4th International Conference for Functional Materials Science 2018, Sanur, Bali, Indonesia
Related Report
Int'l Joint Research
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[Presentation] Magnetic ordered states of hole doped pyrochlore iridates (Nd1-xCax)2Ir2O7 studied by μSR2017
Author(s)
R. Asih, J. Angel, S. Maeda, D. P. Sari, F. Astuti, K. Matsuhira, M. Wakeshima, Y. Hinatsu, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
日本物理学会第72回年次大会
Place of Presentation
大阪大学(豊中市)
Year and Date
2017-03-18
Related Report
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[Presentation] μSR study on magnetic ordered states of pyrochlore iridates Nd2Ir2O7 and Sm2Ir2O72017
Author(s)
R. Asih, S. S. Mohd-Tajudin, F. Astuti, S. Maeda, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
The 37th REIMEI Workshop on Frontiers of Correlated Quantum Matters and Spintronics The DMREF-FCMP Symposium on Mott Transitions and Computational Approaches
Place of Presentation
Conference Hall at Advanced Science Research Center JPARC, iVil Hall- Tokai, and Takeda Hall in Univ. of Tokyo
Year and Date
2017-01-13
Related Report
Int'l Joint Research
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[Presentation] Magnetic ordered states of hole doped pyrochlore iridates (Nd1-xCax)2Ir2O7 studied by μSR2017
Author(s)
R. Asih, S. Maeda, D. P. Sari, J. Angel, F. Astuti, K. Matsuhira, M. Wakeshima, Y. Hinatsu, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
nternational Workshop on Organic Molecular Systems,Penang, Malaysia
Related Report
Int'l Joint Research
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[Presentation] Magnetic ordered states of hole-doped pyrochlore (Nd1-xCax)2Ir2O7 studied by μSR2017
Author(s)
R. Asih, J. Angel, S. Maeda, D. P. Sari, F. Astuti, K. Matsuhira, M. Wakeshima, Y. Hinatsu, I. Watanabe, T. Nakano and Y. Nozue
Organizer
The 3rd Emallia Conference, 釜山、韓国
Related Report
Int'l Joint Research
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[Presentation] フラストレートスピン1/2ラダーRb2Cu2Mo3O12に現れるスピン1ハルデンギャップと強誘電性2017
Author(s)
上田宏, 小野田繁樹, 山口泰弘, 木村剛, 吉澤大智, 森岡俊晶, 萩原政幸, 萩原雅人, 左右田稔, 益田隆嗣, 榊原俊郎, 富安啓輔, 河村聖子, 中島健次, 梶本亮一, 中村充孝, 稲村泰弘, 長谷正司, 安井幸夫
Organizer
日本物理学会第73回年次大会, 東京理科大(野田キャンパス)
Related Report
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[Presentation] Investigation of magnetic ordered states in the pyrochlore iridates (Nd1-xCax)2Ir2O72016
Author(s)
R. Asih, N. Adam, S. S. Mohd-Tajudin, S. Maeda, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
Emallia Conference
Place of Presentation
Graduate School of Science, Hokkaido University, Sapporo
Year and Date
2016-12-19
Related Report
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[Presentation] μSR study on the magnetic ordered states of (Nd1-xCax)2Ir2O72016
Author(s)
R. Asih, S. S. Mohd-Tajudin, F. Astuti, S. Maeda, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
日本物理学会2016年秋季大会
Place of Presentation
金沢大学(金沢市)
Year and Date
2016-09-14
Related Report
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[Presentation] Magnetic ordered states in pyrochlore iridates Nd2Ir2O7 and Sm2Ir2O7 studied by μSR2016
Author(s)
R. Asih, N. Adam, S.S. Mohd-Tajudin, D.P. Sari, K. Matsuhira, H. Guo, M. Wakeshima, Y. Hinatsu, T. Nakano, Y. Nozue, S. Sulaiman, M.I. Mohamed-Ibrahim, P.B. Kumar, and I. Watanabe
Organizer
The 8th International Conference on Highly Frustrated Magnetism (HFM 2016)
Place of Presentation
NTU Convention Center, Taipei, Taiwan
Year and Date
2016-09-07
Related Report
Int'l Joint Research
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[Presentation] Magnetic ordered states in pyrochlore iridates R2Ir2O7 (R = Nd and Sm) investigated by μSR2016
Author(s)
R. Asih, N. Adam, S.S. Mohd-Tajudin, D.P. Sari, K. Matsuhira, H. Guo, M. Wakeshima, Y. Hinatsu, T. Nakano, Y. Nozue, S. Sulaiman, M.I. Mohamed-Ibrahim, P.B. Kumar, and I. Watanabe
Organizer
Rare Earth Conferences 2016
Place of Presentation
Conference Hall, Hokkaido University
Year and Date
2016-06-05
Related Report
Int'l Joint Research
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[Presentation] Investigation of magnetic ordered states in the (Nd1-xCax)2Ir2O7 probed by μSR2016
Author(s)
R. Asih, N. Adam, S. S. Mohd-Tajudin, S. Maeda, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
Hokkaido University-RIKEN symposium
Place of Presentation
Graduate School of Science, Hokkaido University, Sapporo
Year and Date
2016-05-25
Related Report
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[Presentation] Effect of Ca-substitution on the magnetic ordered state of (Na1-xCax)2Ir2O7 studied by μSR2016
Author(s)
R. Asih, S. S. Mohd-Tajudin, S. Maeda, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, and Y. Nozue
Organizer
日本物理学会第71回年次大会
Place of Presentation
東北学院大学(仙台市)
Year and Date
2016-03-21
Related Report
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[Presentation] μSR Study on the Pyrochlore Iridates R2Ir2O7 (R= Nd,Sm)2015
Author(s)
R. Asih, N. Adam, S. S. Mohd-Tajudin, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, Y. Nozue
Organizer
International Symposium on Present and Future of Material Sciences
Place of Presentation
大阪大学(豊中市)
Year and Date
2015-11-17
Related Report
Int'l Joint Research
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[Presentation] μSR Study on the Pyrochlore Iridates R2Ir2O7 (R= Nd,Sm)2015
Author(s)
R. Asih, N. Adam, S. S. Mohd-Tajudin, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, Y. Nozue
Organizer
東大物性研短期研究会「スピン系物理の深化と最前線」
Place of Presentation
東京大学物性研(千葉県柏市)
Year and Date
2015-11-16
Related Report
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[Presentation] Investigation of Magnetic Ordered State in the Pyrochlore Iridates R2Ir2O7 (R= Nd,Sm) probed by μSR2015
Author(s)
R. Asih, N. Adam, S. S. Mohd-Tajudin, K. Matsuhira, M. Wakeshima, Y. Hinatsu, A. Miyake, M. Tokunaga, I. Watanabe, T. Nakano, Y. Nozue
Organizer
日本物理学会2015年秋季大会
Place of Presentation
関西大学(吹田市)
Year and Date
2015-09-18
Related Report
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