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Novel spin state in Co akermanite

Research Project

Project/Area Number 15K05145
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionOsaka University

Principal Investigator

AKAKI MITSURU  大阪大学, 理学研究科, 特任助教(常勤) (60610904)

Co-Investigator(Renkei-kenkyūsha) MASUDA Takatsugu  東京大学, 物性研究所, 准教授 (90313014)
KOHAMA Yoshimitsu  東京大学, 物性研究所, 准教授 (90447524)
KIHARA Takumi  東北大学, 金属材料研究所, 助教 (80733021)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2017: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2016: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2015: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywordsマルチフェロイック / 電気磁気効果 / パルス強磁場 / 電子スピン共鳴 / スピン四極子 / 強磁場 / 磁化 / 電気分極
Outline of Final Research Achievements

Exotic spin-multipolar ordering in spin transition metal insulators has so far eluded unambiguous experimental observation. A less studied, but perhaps more feasible fingerprint of multipole character emerges in the excitation spectrum in the form of quadrupolar transitions. Such multipolar excitations are desirable as they can be manipulated with the use of light or electric field and can be captured by means of conventional experimental techniques. Here we study single crystals of multiferroic Sr2CoGe2O7, and observe a two-magnon spin excitation appearing above the saturation magnetic field in electron spin resonance (ESR) spectra. Our analysis of the selection rules reveals that this spin excitation mode does not couple to the magnetic component of the light, but it is excited by the electric field only, in full agreement with the theoretical calculations. Due to the nearly isotropic nature of Sr2CoGe2O7, we identify this excitation as a purely spin-quadrupolar two-magnon mode.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (28 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (2 results) Journal Article (6 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 6 results,  Open Access: 2 results,  Acknowledgement Compliant: 3 results) Presentation (20 results) (of which Int'l Joint Research: 10 results)

  • [Int'l Joint Research] Inst. for Solid State Phys. and Optics,/Wigner Res. Centre for Phys(ハンガリー)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] ハンガリー科学アカデミー(ハンガリー)

    • Related Report
      2016 Research-status Report
  • [Journal Article] Magnetoelectric properties of Ca2CoSi2O7 studied by high-field electron spin resonance2018

    • Author(s)
      M. Akaki, K. Kanaida and M. Hagiwara
    • Journal Title

      Journal of Physics: Conf. Series

      Volume: 969 Pages: 012102-012102

    • DOI

      10.1088/1742-6596/969/1/012102

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Direct observation of spin-quadrupolar excitations in Sr2CoGe2O7 by high field ESR2017

    • Author(s)
      Mitsuru Akaki, Daichi Yoshizawa, Akira Okutani, Takanori Kida, Judit Romhanyi, Karlo Penc, and Masayuki Hagiwara
    • Journal Title

      Phys. Rev. B

      Volume: 96 Issue: 21 Pages: 214406-214406

    • DOI

      10.1103/physrevb.96.214406

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Magnetoelectric Behavior from the S=1/2 Asymmetric Square Cupolas2017

    • Author(s)
      Y. Kato, K. Kimura, A. Miyake, M. Tokunaga, A. Matsuo, K. Kindo, M. Akaki, M. Hagiwara, M. Sera, T. Kimura, and Y. Motome
    • Journal Title

      Phys. Rev. Lett

      Volume: 118 Issue: 10 Pages: 1076011-5

    • DOI

      10.1103/physrevlett.118.107601

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Magnetic Structure and Dielectric State in the Multiferroic Ca2CoSi2O72017

    • Author(s)
      M. Soda, S. Hayashida, T. Yoshida, M. Akaki, M. Hagiwara, M. Avdeev, O. Zaharko, and T. Masuda
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 印刷中

    • NAID

      210000134400

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Magnetic-Field-Induced Polar Phase in Chiral Magnet CsCuCl32015

    • Author(s)
      A. Miyake, J. Shibuya, M. Akaki, H. Tanaka, and M. Tokunaga
    • Journal Title

      Physical Review B

      Volume: 92 Issue: 10

    • DOI

      10.1103/physrevb.92.100406

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Impurity Substitution Effect on Magnetoelectric Properties of CaBaCo4O7 Crystals2015

    • Author(s)
      R. Oda, R. Kajihara, K. Nishina, M. Akaki, H. Kuroe, and H. Kuwahara
    • Journal Title

      Physics Procedia

      Volume: 75 Pages: 303-308

    • DOI

      10.1016/j.phpro.2015.12.036

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Presentation] Sr2CoGe2O7におけるスピン四極子励起の観測(実験)2018

    • Author(s)
      赤木暢, 吉澤大智, 奥谷顕, 木田孝則, J. Romhanyi, K. Penc, 萩原政幸
    • Organizer
      日本物理学会 第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Observation of spin-quadrupolar excitations in Sr2CoGe2O7 (Theory)2018

    • Author(s)
      Mitsuru Akaki, Daichi Yoshizawa, Akira Okutani, Takanori Kida, Judit Romhanyi, Karlo Penc, and Masayuki Hagiwara
    • Organizer
      日本物理学会 第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] オケルマナイト酸化物Ca2CoSi2O7のパルス強磁場ESR2017

    • Author(s)
      赤木暢, 金井田小夏, 萩原政幸
    • Organizer
      日本物理学会 第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] Magnetoelectric properties of Ca2CoSi2O7 studied by high-field electron spin resonance2017

    • Author(s)
      M. Akaki, K. Kanaida and M. Haagiwara
    • Organizer
      28th International Conference on Low Temperature Physics (LT28)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electric(magnetic)-field control of magnetization(electric polarization) in CaBaM4O7 (M=Co,Fe) single crystals2017

    • Author(s)
      H. Kuwahara, M. Noda, Y. Ebukuro, M. Akaki, and H. Kuroe
    • Organizer
      28th International Conference on Low Temperature Physics (LT28)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Magneto-electric spin excitations in forced-ferromagnetic state of Sr2CoSi2O7」2017

    • Author(s)
      M. Akaki, Y. Aoki and M. Hagiwara
    • Organizer
      The 9th APCTP Workshop on Multiferroics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Magnetic field induced polar phase in the chiral magnet CsCuCl32017

    • Author(s)
      A. Miyake, J. Shibuya, M. Akaki, H. Tanaka, and M. Tokunaga
    • Organizer
      The 9th APCTP Workshop on Multiferroics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of a nonreciprocal signal in ferromagnetic resonance in multiferroic GaFeO32017

    • Author(s)
      T. Omi, M. Akaki, N. Abe, Y. Tokunaga, S. kimura, M. Hagiwara, and T. Arima
    • Organizer
      The 9th APCTP Workshop on Multiferroics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Magnetoelectric effects in Ba2CuGe2O7 beyond the saturation field2017

    • Author(s)
      M. Tokunaga, Y. sato, A. Miyake, M. Akaki, M. Hagiwara, and H. Kuwahara
    • Organizer
      The 9th APCTP Workshop on Multiferroics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 強磁場電子スピン共鳴測定によるスピン四極子励起の観測2017

    • Author(s)
      赤木暢, 吉澤大智, 奥谷顕, 木田孝則, J. Romhanyi, K. Penc, 萩原政幸
    • Organizer
      強磁場コラボラトリーが拓く未踏計測領域への挑戦と物質・材料科学の最先端
    • Related Report
      2017 Annual Research Report
  • [Presentation] Sr2CoGe2O7におけるパルス強磁場ESR測定2016

    • Author(s)
      赤木暢
    • Organizer
      量子スピン系研究会
    • Place of Presentation
      福井大学
    • Year and Date
      2016-12-02
    • Related Report
      2016 Research-status Report
  • [Presentation] 強磁場下におけるBa2CuGe2O7の電気磁気効果2016

    • Author(s)
      徳永将史, 佐藤由昌, 赤木暢, 三宅厚志, 萩原政幸, 桑原英樹
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] Studies on magnetoelectric properties of Sr2CoGe2O7 by high-field electron spin resonance2016

    • Author(s)
      M. Akaki, D. Yoshizawa, A. Okutani, T. Kida, and M. Hagiwara
    • Organizer
      Multiferroic & Magnetoelectric Materials Gordon Research Conference
    • Place of Presentation
      Lewiston, USA
    • Year and Date
      2016-08-07
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] マルチフェロイック物質Ca2CoSi2O7の磁気構造2016

    • Author(s)
      左右田稔, 吉田俊, 赤木暢, 萩原政幸, Oksana Zaharko, Maxim Avdeev, 伊藤晋一, 横尾哲也, 益田隆嗣
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] Sr2CoGe2O7におけるパルス強磁場ESR測定2016

    • Author(s)
      赤木暢, 青木勇磨, 奥谷顕, 吉澤大智, 木田孝則, 萩原政幸
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] High Field ESR in the akermanite Sr2CoSi2O72015

    • Author(s)
      Y. Aoki, M. Akaki, T. Kida, A. Okutani, D. Yoshizawa, T. Morioka, and M. hagiwara
    • Organizer
      International Symposium on Present and Future of Material Sciences
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2015-11-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] High-field electron spin resonance in Sr2CoGe2O7 single crystal2015

    • Author(s)
      M. Akaki, Y. Aoki, D. Yoshizawa, A. Okutani, T. Kida, and M. Hagiwara
    • Organizer
      International Symposium on Present and Future of Material Sciences
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2015-11-17
    • Related Report
      2015 Research-status Report
  • [Presentation] オケルマナイト型化合物(Ca1-xSrx)2CoSi2O7の強磁場物性2015

    • Author(s)
      青木勇磨, 赤木暢, 木田孝則, 奥谷顕, 吉澤大智, 森岡俊晶, 萩原政幸
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] Magnetic properties of quasi one-dimensional antiferromagnet BaCo2Si2O72015

    • Author(s)
      M. Akaki, A. Okutani, D. Yoshizawa, H. Kuwahara, and M. Hagiwara
    • Organizer
      20th International Conference on Magnetism (ICM2015)
    • Place of Presentation
      Barcelona, Spain
    • Year and Date
      2015-07-05
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] High-field magnetic properties of akermanite (Ca1-xSrx)2CoSi2O7 single crystals2015

    • Author(s)
      M. Akaki, Y. Aoki, D. Yoshizawa, A. Okutani, and M. Hagiwara
    • Organizer
      11th International Conference on Research in High Magntic Fields (RHMF2015)
    • Place of Presentation
      Grenoble, France
    • Year and Date
      2015-07-01
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research

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Published: 2015-04-16   Modified: 2020-05-15  

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