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Application to liquid phase chemical process of HO2 radical

Research Project

Project/Area Number 15K05963
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Power engineering/Power conversion/Electric machinery
Research InstitutionOsaka Institute of Technology

Principal Investigator

MIICHI TOMOAKI  大阪工業大学, 工学部, 准教授 (40368139)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2017: ¥130,000 (Direct Cost: ¥100,000、Indirect Cost: ¥30,000)
Fiscal Year 2016: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2015: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Keywords赤外吸収分光分析 / 水上直流コロナ放電 / 水処理 / 液中化学反応 / 活性酸素 / in-situ赤外吸収分光分析 / 液中化学プロセス
Outline of Final Research Achievements

The characteristics of acetic acid decomposition were investigated by a DC corona discharge over water. The corona discharge is 4 mm away from the water surface. Hence, this method does not directly treat water using discharge plasma. During corona processing, oxygen or ozone was supplied to the reactor. The optimal discharge treatment conditions were investigated by varying experimental condition. Results of treating aqueous solution of acetic acid with corona discharge showed that acetic acid can be decomposed, and that its decomposition amount heavily varies with pH of the solution. Next it was found that the decomposition rate of acetic acid increased when the gas flow rate was high at the same gaseous ozone concentration. Furthermore, as the gas flow rate increased, the concentration of the water vapor measured by infrared spectroscopy decreased. Our results indicate that ozone and the reactive oxygen species other than ozone are conveyed to water surface by a DC corona discharge.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (12 results)

All 2018 2017 2016 2015

All Journal Article (3 results) (of which Peer Reviewed: 2 results) Presentation (9 results) (of which Int'l Joint Research: 2 results)

  • [Journal Article] Advanced Oxidation Process using DC Corona Discharge Over Water2018

    • Author(s)
      見市 知昭、神澤 龍也
    • Journal Title

      IEEJ Transactions on Fundamentals and Materials

      Volume: 138 Issue: 2 Pages: 57-63

    • DOI

      10.1541/ieejfms.138.57

    • NAID

      130006329209

    • ISSN
      0385-4205, 1347-5533
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Advanced Oxidation Process using DC Corona Discharge over Water2018

    • Author(s)
      MIICHI TOMOAKI、KANZAWA RYUYA
    • Journal Title

      Electronics and Communications in Japan

      Volume: 101 Issue: 5 Pages: 65-72

    • DOI

      10.1002/ecj.12064

    • NAID

      130006329209

    • Related Report
      2017 Annual Research Report
  • [Journal Article] pH Dependence on Decomposition of Persistent Organic Compounds in Water Using a DC Corona Discharger2017

    • Author(s)
      T. Miichi
    • Journal Title

      International Journal of Plasma Environmental Science & Technology

      Volume: 11 Pages: 13-17

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] 水上直流コロナ放電を用いた水処理における気相オゾンの影響2017

    • Author(s)
      神澤龍也,見市知昭
    • Organizer
      平成29年電気学会全国大会
    • Place of Presentation
      富山大学 五福キャンパス
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] Effect of Gaseous Ozone Addition on Decomposition of Persistent Organic Compounds in Water using DC Corona Discharge2017

    • Author(s)
      T. Miichi, R. Kanzawa
    • Organizer
      International Symposium on Electrohydrodynamics 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 水上直流コロナ放電による液中生成活性種の計測2017

    • Author(s)
      神澤龍也,見市知昭
    • Organizer
      平成29年電気学会基礎・材料・共通部門大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 直流コロナ放電を用いた促進酸化処理の検討2017

    • Author(s)
      久保基,見市知昭
    • Organizer
      平成29年電気関係学会関西連合大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 水上コロナ放電を用いた水処理における放電生成物の影響2016

    • Author(s)
      神澤龍也,見市知昭
    • Organizer
      平成28年電気関係学会関西連合大会
    • Place of Presentation
      大阪府立大学 中百舌鳥キャンパス
    • Year and Date
      2016-11-22
    • Related Report
      2016 Research-status Report
  • [Presentation] 水上直流コロナ放電における放電生成物のin-situ計測2016

    • Author(s)
      神澤龍也,見市知昭
    • Organizer
      2016年度 第40回静電気学会全国大会
    • Place of Presentation
      群馬大学 桐生キャンパス
    • Year and Date
      2016-09-30
    • Related Report
      2016 Research-status Report
  • [Presentation] Discharge products measurement in a DC corona discharge over water by infrared spectroscopy2016

    • Author(s)
      T. Miichi
    • Organizer
      The 10th International Symposium on Non-Thermal/Thermal Plasma Pollution Control Technology and Sustainable Energy
    • Place of Presentation
      Slaviero Essential Florianopolis Ingleses Acquamar, Florianopolis, Brazil
    • Year and Date
      2016-08-01
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 水上コロナ放電における赤外分光法を用いた放電生成物の計測2016

    • Author(s)
      松實健司、見市知昭
    • Organizer
      2016年度静電気学会春期講演会
    • Place of Presentation
      東京大学 工学部
    • Year and Date
      2016-03-07
    • Related Report
      2015 Research-status Report
  • [Presentation] 水上放電におけるFTIRを用いたHO2ラジカルの測定2015

    • Author(s)
      松實健司、見市知昭
    • Organizer
      平成27年電気関係学会関西連合大会
    • Place of Presentation
      摂南大学 寝屋川キャンパス
    • Year and Date
      2015-11-14
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2019-03-29  

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