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Plasmon-enhanced photoelectrochemical energy conversion on Au nanoparticles loaded titanium dioxide thin film

Research Project

Project/Area Number 15K20833
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Physical chemistry
Nanostructural physics
Research InstitutionHokkaido University

Principal Investigator

Shi Xu  北海道大学, 電子科学研究所, 助教 (20749113)

Project Period (FY) 2015-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2016: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2015: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordsplasmon resonance / water splitting / strong coupling / titanium dioxide / thin film solar cell / Plasmon resonance / Coupling / Cavity mode / Water splitting / Plasmon / Titanium Dioxide / Gold Nanoparticles / Water Oxidation
Outline of Final Research Achievements

In this study, the plasmon-induced water oxidation process was investigated via a in-situ SERS measurement. The interfacial structure effect on the charge separation was determined at the atomic layer scale. A tight contact between the metal nanoparticles and its support metal oxide is highly demanded for efficient plasmon-induced charge separation. Based on the understanding of the plasmon-induced water oxidation process and the interfacial structure effect on the charge separation, we successfully constructed a novel plasmonic structure, which shows strong light absorption, for broadband plasmon-enhanced solar energy conversion.

Report

(3 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • Research Products

    (8 results)

All 2017 2016

All Journal Article (4 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 4 results,  Open Access: 4 results,  Acknowledgement Compliant: 4 results) Presentation (4 results) (of which Int'l Joint Research: 2 results)

  • [Journal Article] Plasmon-induced photoelectrochemical biosensor for in situ real-time measurement of biotin-streptavidin binding kinetics under visible light irradiation2017

    • Author(s)
      J. Guo, T. Oshikiri, K. Ueno, Xu Shi, H. Misawa
    • Journal Title

      Anal. Chim. Acta.

      Volume: 957 Pages: 70-75

    • DOI

      10.1016/j.aca.2016.12.025

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Highly Sensitive Aluminum-Based Biosensors using Tailorable Fano Resonances in Capped Nanostructures2017

    • Author(s)
      K.-L. Lee, H.-U. Hsu, M.-L. You, C.-C. Chang, M.-Y. Pan, X. Shi, K. Ueno, H. Misawa, and P.-K. Wei
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 44104-44104

    • DOI

      10.1038/srep44104

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Water splitting using a three-dimensional plasmonic photoanode with titanium dioxide nano-tunnels2017

    • Author(s)
      R. Takakura, T. Oshikiri, K. Ueno, X. Shi, T. Kondo, H. Masuda and H. Misawa
    • Journal Title

      Green Chemistry

      Volume: 印刷中 Issue: 10 Pages: 2398-2405

    • DOI

      10.1039/c6gc03217f

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Cobalt Oxide (CoOx) as an Efficient Hole-extracting Layer for High-performance Inverted Planar Perovskite Solar Cells2016

    • Author(s)
      A. E. Shalan, T. Oshikiri, S. Narra, M. M. Elshanawany, K. Ueno, H.-P. Wu, K. Nakamura, X. Shi, E. W.-G. Diau, H. Misawa
    • Journal Title

      ACS Appl. Mater. Interfaces

      Volume: 8 Issue: 49 Pages: 33592-33600

    • DOI

      10.1021/acsami.6b10803

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Presentation] Plasmon-induced photocurrent generation using coupling between localized surface plasmon resonance and cavity mode2017

    • Author(s)
      Xu Shi, Tomoya Oshikiri, Kosei Ueno, Keiji Sasaki, Hiroaki Misawa
    • Organizer
      The 97th CSJ Annual Meeting
    • Place of Presentation
      Hiyoshi Campus, Keio University, Yokohama, Japan
    • Year and Date
      2017-03-16
    • Related Report
      2016 Annual Research Report
  • [Presentation] Observation of charge separation between gold nanoparticles and titanium dioxide using surface plasmon spectroscopy2016

    • Author(s)
      X. Shi, K. Ueno, T. Oshikiri, H. Misawa
    • Organizer
      The International Chemical Congress of Pacific Basin Societies (PACHIFICHEM) 2015
    • Place of Presentation
      Honolulu, USA
    • Year and Date
      2016-12-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Plasmon-induced photocurrent generation system using metal-semiconductor-metal nanostructured perfect absorber2016

    • Author(s)
      Xu Shi, Kosei Ueno, Tomoya Oshikiri, Hiroaki Misawa
    • Organizer
      Annual meeting on Photochemistry 2016
    • Place of Presentation
      Komaba I Campus, The University of Tokyo
    • Year and Date
      2016-09-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] Improvement of Plasmon-Enhanced Photocurrent Generation by Interference of Titanium Dioxide Thin-film2016

    • Author(s)
      X. Shi, K. Ueno, T. Oshikiri, H. Misawa
    • Organizer
      27th International Conference on Photochemistry (ICP2015)
    • Place of Presentation
      Jeju Island, Korea
    • Year and Date
      2016-06-28
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research

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Published: 2015-04-16   Modified: 2018-03-22  

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