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Temporal variation of nano-particle, elemental carbon and organic carbon in the urban atmosphere

Research Project

Project/Area Number 16310003
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionThe University of Tokyo

Principal Investigator

KOMAZAKI Yuichi  The University of Tokyo, Research Center for Advanced Science and Technology, Specially Appointed Associate Professor, 先端科学技術研究センター, 科学技術振興特任教員(特任助教授) (80286640)

Co-Investigator(Kenkyū-buntansha) KONDO Yutaka  The University of Tokyo, Research Center for Advanced Science and Technology, Professor, 先端科学技術研究センター, 教授 (20110752)
TAKEGAWA Nobuyuki  The University of Tokyo, Research Center for Advanced Science and Technology, Associate Professor, 先端科学技術研究センター, 助教授 (00324369)
KOIKE Makoto  The University of Tokyo, Graduate School of Science, Associate Professor, 大学院・理学系研究科, 助教授 (00225343)
宮崎 雄三  東京大学, 先端科学技術研究センター, 助手 (60376655)
Project Period (FY) 2004 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥16,000,000 (Direct Cost: ¥16,000,000)
Fiscal Year 2005: ¥4,600,000 (Direct Cost: ¥4,600,000)
Fiscal Year 2004: ¥11,400,000 (Direct Cost: ¥11,400,000)
KeywordsEnvironmental behavior / Urban atmophere / Nano-particle / Elemental carbon / Organic carbon / Carbon monoxide / 動態観測 / 粒径分布 / 季節変化 / 二次生成
Research Abstract

EC comprises a significant portion of nano-particles, which are harmful to human health. EC has also been identified as making important contributions to the radiative heating of the atmosphere. Mass concentrations of EC in fine mode and CO were measured in Tokyo. EC were measured using a semi-continuous thermal-optical analyzer. The mass concentrations of non-volatile fine-particle measured by the calibrated SMPS combined with a heated inlet agreed with the independent EC measurements, demonstrating that the mass concentrations of non-volatile particle well those for EC. EC mass concentration was in volume equivalent diameters between 50-200 nm, peaking at around 130 nm. The correlation of EC and CO was generally compact throughout the measurement period. The slope of the EC-CO correlation (ΔEC/ΔCO) is therefore a useful parameter in validating EC emission inventories. The EC concentration and ΔEC/ΔCO showed distinct diurnal variation. On weekdays, EC and ΔEC/ΔCO reached maximum values, respectively, in the early morning, when the traffic density of heavy-duty trucks with diesel engines was highest. In addition, these values were lower by a factor of 2 on Sundays. The heavy truck traffic showed similar diurnal and weekday/weekend variations, indicating that exhaust from diesel engines is an important source of EC. Monthly mean ΔEC/ΔCO showed a seasonal variation, reaching broad maximum values in spring-autumn and reaching minimum values in midwinter. More stringent regulation of emissions of particles from diesel cars started in the Tokyo metropolitan area in October 2003. The ΔEC/ΔCO values did not change significantly (10%) after one year from the start of the new regulations, when the temperature dependence is taken into account. This indicates that the regulation of particle emissions in the Tokyo Metropolitan Area was not effective in reducing the EC concentrations after one year.

Report

(3 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • Research Products

    (14 results)

All 2006 2005 2004 Other

All Journal Article (14 results)

  • [Journal Article] Temporal variations of elemental carbon in Tokyo2006

    • Author(s)
      Y.Kondo., Y.Komazaki, 他
    • Journal Title

      Journal of Geophysical Research (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Time-resolved measurements of water-soluble organic carbon in Tokyo2006

    • Author(s)
      Y.Miyazaki, Y.Komazaki, 他
    • Journal Title

      Journal of Geophysical Research (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Temporal variation of elemental carbon in Tokyo2006

    • Author(s)
      Y.Kondo, Y.Komazaki, et al.
    • Journal Title

      Journal of Geophysical Research (In press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Time-resolved measurements of water-soluble organic carbon in Tokyo2006

    • Author(s)
      Y.Miyazaki, Y.Komazaki, et al.
    • Journal Title

      Journal of Geophysical Research (In press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Temporal variations of elemental carbon in Tokyo2006

    • Author(s)
      Y.Kondo, Y.Komazaki 他
    • Journal Title

      Journal of Geophysical Research 111(印刷中)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Time-resolved measurements of water-soluble organic carbon in Tokyo2006

    • Author(s)
      Y.Miyazaki, Y.Komazaki 他
    • Journal Title

      Journal of Geophysical Research (印刷中)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Partitioning of HNO_3 and particulate nitrate over Tokyo : Effect of vertical mixing2006

    • Author(s)
      Y.Morino, Y.Komazaki 他
    • Journal Title

      Journal of Geophysical Research 111(印刷中)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Characterization of an Aerodyne Aerosol Mass Spectrometer (AMS) : Intercomparison with other aerosol instruments2005

    • Author(s)
      N.Takagawa, Y.Komazaki, 他
    • Journal Title

      Aerosol Science and Technology 39

      Pages: 760-770

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Characterization of an Aerodyne Aerosol Mass Spectrometer (AMS) : Intercomparison with other aerosol instruments2005

    • Author(s)
      N.Takegawa, Y.Komazaki, et al.
    • Journal Title

      Aerosol Science and Technology 39

      Pages: 760-770

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Characterization of an Aerodyne Aerosol Mass Spectrometer (AMS) : Intercomparison with other aerosol instruments2005

    • Author(s)
      N.Takegawa, Y.Komazaki 他
    • Journal Title

      Aerosol Science and Technology 39

      Pages: 760-770

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Composition and major sources of compound of aerosol particulate matter samples during the ACE-Asia campaign2004

    • Author(s)
      B.R.T.Simoneit, Y.Komazaki, 他
    • Journal Title

      Journal of Geophysical Research 109・D19

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Composition and major sources of compound of aerosol particulate matter sampled during the ACE-Asia campaign2004

    • Author(s)
      B.R.T.Simoneit, Y.Komazaki, et al.
    • Journal Title

      Journal of Geophysical Research 109 (D19)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Composition and major sources of compound of aerosol particulate matter sampled during the ACE-Asia campain2004

    • Author(s)
      Y.Komazaki他
    • Journal Title

      Journal of Geophysical Research 109

    • Related Report
      2004 Annual Research Report
  • [Journal Article] A chemical ionization mass spectrometer for ground-base measurement of nitric acid

    • Author(s)
      K.Kita, Y.Komazaki 他
    • Journal Title

      Journal of Atmospheric and Ocean Technology (印刷中)

    • Related Report
      2005 Annual Research Report

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Published: 2004-04-01   Modified: 2016-04-21  

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