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Stroboscopic Scanning Probe Microscopy and Time-Resolved Molecular-Scale Imaging of Photoexcited Carriers

Research Project

Project/Area Number 16310074
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nanostructural science
Research InstitutionOsaka University

Principal Investigator

MATSUMOTO Takuya  Osaka University, The Institute of Scientific and Industrial Research, Associate Professor, 産業科学研究所, 助教授 (50229556)

Co-Investigator(Kenkyū-buntansha) TANIGUCHI Masateru  Osaka University, The Institute of Scientific and Industrial Research, Research Associates, 産業科学研究所, 助手 (40362628)
Project Period (FY) 2004 – 2006
Project Status Completed (Fiscal Year 2006)
Budget Amount *help
¥15,200,000 (Direct Cost: ¥15,200,000)
Fiscal Year 2006: ¥3,800,000 (Direct Cost: ¥3,800,000)
Fiscal Year 2005: ¥5,300,000 (Direct Cost: ¥5,300,000)
Fiscal Year 2004: ¥6,100,000 (Direct Cost: ¥6,100,000)
KeywordsStroboscopic probe / Photo-excited charge transfer / Time-resolved measurement / Electrostatic field calculation / Kelvin force microscopy / Electrostatic force microscopy / ストロボスコピック・プローブ顕微鏡
Research Abstract

In this year, we demonstrated time-resolved force detection by using scanning force microscopy. In the dynamic-mode operation, the tip interacts with the surface only at the moment when the tip closes to the sample surface. The interactive duration can be estimated or less. Taking advantage of this short duration, submicrosecond-class time-resolved force detection has been achieved by the coincidence between photo-irradiation and cantilever motion.
Since the frequency of cantilever oscillation is modulated by the tip-sample force change during the scan, it is necessary that the timing of each laser pulse should be synchronized by each stroke of cantilever motion. We examined that the relationship between oscillation amplitude and the laser-pulse delay with various sample bias voltage. The sample was a Si(111) flushed in UHV condition. In usual, oscillation amplitude does not changed by bias voltage in non-contact region. Actually, in case of no laser irradiation, there is no bias effect. However, under the pulsed laser irradiation, the oscillation amplitude is dramatically changed as a function of both delay time and bias voltage. Furthermore, we found dead zone in delay time. These results indicate that the transient charge generated by pulsed laser irradiation can be detected with μs-class resolution.

Report

(4 results)
  • 2006 Annual Research Report   Final Research Report Summary
  • 2005 Annual Research Report
  • 2004 Annual Research Report
  • Research Products

    (23 results)

All 2007 2006 2005 2004

All Journal Article (22 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Tunnelling charge injection into a pentacene layer using dynamic-mode scanning force microscopy2007

    • Author(s)
      T.Kusaka, K.Ojima, T.Matsumoto, T.Kawai
    • Journal Title

      Nanotechnology 18

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Tunnelling charge injection into a pentacene layer using dynamic-mode scanning force microscopy2007

    • Author(s)
      Takao Kusaka, Kaoru Ojima, Takuya Matsumoto, Tomoji Kawai
    • Journal Title

      Nanotechnology 18

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Annual Research Report 2006 Final Research Report Summary
  • [Journal Article] Anchoring gold nanoparticles onto a mica surface by oxygen plasma ashing for sequential nanocomponent assembly.2007

    • Author(s)
      Akihiko Takagi, Kaoru Ojima, Eriko Mikamo, Takuya Matsumoto, Tomoji Kawai
    • Journal Title

      Appl. Phys. Left. 90

      Pages: 43122-43122

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Single molecular morphology of porphyrin / DNA complex2006

    • Author(s)
      C.Takatoh, T.Matsumoto, T.Kawai, T.Saitoh, K.Takeda
    • Journal Title

      Chem. Lett. 35

      Pages: 88-89

    • NAID

      10016907996

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Giant porphrin wheels with Large Electronic coupling as models of light harvesting photosynthetic antenna2006

    • Author(s)
      T.Hori, N.Aratani, A.Takagi, T.Matsumoto, T.Kawai, Min-Chul Yoon, Zin Seok Yoon, Sung Cho, Dongho Kim, A.Osuka
    • Journal Title

      Chem. Eur. J. 12

      Pages: 1319-1327

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Porphyrin molecules working as nanodevice on single-walled carbon nanotube wiring.2006

    • Author(s)
      Hirofumi Tanaka, T.Yajima, T.Matsumoto, Y.Otsuka, T.Ogawa
    • Journal Title

      Adv. Materals 18

      Pages: 1411-1415

    • NAID

      120004837470

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] A directly fused tetrameric porphyrin sheet and its unique electronic properties that arise from the planar yclooctatetraenecore.2006

    • Author(s)
      Y.Nnakamura, N.Aratani, H.Shinokubo, A.Takagi, T.Kawai, T.Matsumoto, Zin Seok Yoon, Deok Yun Kim, Tae Kyu Ahn, Dongho Kim, A.Muranaka, N.Kobayashi, A.Osuka
    • Journal Title

      J. Am. Chem. Soc. 128

      Pages: 4119-4127

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Single molecular morphology of porphyrin / DNA complex2006

    • Author(s)
      Chikako Takatoh, Takuya Matsumoto, Tomoji Kawai, Takayuki Saitoh, Kazuyoshi Takeda
    • Journal Title

      Chem.Lett. 35

      Pages: 88-89

    • NAID

      10016907996

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Giant porphrin wheels with Large Electronic coupling as models of light harvesting photosynthetic antenna2006

    • Author(s)
      Takaaki Hori, Naoki Aratani, Akihiko Takagi, Takuya Matsumoto, Tomoji Kawai, Min-Chul Yoon, Zin Seok Yoon, Sung Cho, Dongho Kim, Atsuhiro Osuka
    • Journal Title

      Chem.Eur.J. 12

      Pages: 1319-1327

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Porphyrin molecules working as nanodevice on single-walled carbon nanotube wiring.2006

    • Author(s)
      Hirofumi Tanaka, Takashi Yajima, Takuya Matsumoto, Yoichi Otsuka, Takuji Ogawa
    • Journal Title

      Adv.Materals 18

      Pages: 1411-1415

    • NAID

      120004837470

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] A directly fused tetrameric porphyrin sheet and its unique electronic properties that arise from the planar yclooctatetraene core.2006

    • Author(s)
      Yasuyuki Nnakamura, Naoki Aratani, Hiroshi Shinokubo, Akihiko Takagi, Tomoji Kawai, Takuya Matsumoto, Zin Seok Yoon, Deok Yun Kim, Tae Kyu Ahn, Dongho Kim, Atuya Muranaka, Nagao Kobayashi, Atsuhiro Osuka
    • Journal Title

      J.Am.Chem.Soc. 128

      Pages: 4119-4127

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Single molecular morphology of porphyrin/DNA complex2006

    • Author(s)
      Chikako Takatoh, Takuya Matsumoto, Tomoji Kawai, Takayuki Saitoh, Kazuyoshi Takeda
    • Journal Title

      Chem. Lett. 35

      Pages: 88-89

    • NAID

      10016907996

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Giant porphrin wheels with Large Electronic coupling as models of light harvesting photosynthetic antenna2006

    • Author(s)
      Takaaki Hori, Naoki Aratani, Akihiko Takagi, Takuya Matsumoto, Tomoji Kawai, Min-Chul Yoon, Zin Seok Yoon, Sung Cho, Dongho Kim, Atsuhiro Osuka
    • Journal Title

      Chem. Eur. J. 12

      Pages: 1319-1327

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Porphyrin molecules working as nanodevice on single-walled carbon nanotube wiring.2006

    • Author(s)
      Hirofumi Tanaka, Takashi Yajima, Takuya Matsumoto, Yoichi Otsuka, Takuji Ogawa
    • Journal Title

      Adv. Materals 18

      Pages: 1411-1415

    • NAID

      120004837470

    • Related Report
      2006 Annual Research Report
  • [Journal Article] A directly fused tetrameric porphyrin sheet and its unique electronic properties that arise from the planar yclooctatetraene core.2006

    • Author(s)
      Yasuyuki Nnakamura, Naoki Aratani, Hiroshi Shinokubo, Akihiko Takagi Tomoji Kawai, Takuya Matsumoto, Zin Seok Yoon, Deok Yun Kim, Tae Kyu Ahn, Dongho Kim, Atuya Muranaka, Nagao Kobayashi, Atsuhiro Osuka
    • Journal Title

      J. Am. Chem. Soc. 128

      Pages: 4119-4127

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Directly meso-meso linked porphyrin rings : synthesis, characterization, and efficient excitation energy hopping.2005

    • Author(s)
      Y.Nakamura, in-Wook Hwang, N.Aratani, Tae Kyu Ahn, Dah Mee Ko, A.Takagi, T.Kawai, T.Matsumoto, Dongho Kim, A.Osuka
    • Journal Title

      J. Am. Chem. Soc. 127

      Pages: 236-246

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Giant meso-meso-Linked Porphyrin Arrays of Micrometer Molecular Length and Their Fabrication.2005

    • Author(s)
      N.Aratani, A.Takagi, Y.Yanagawa, T.Matsumoto, T.Kawai, Zin Seok Yoon, Dongho Kim, A.Osuka
    • Journal Title

      Chem. A-Euro. J. 11

      Pages: 3389-3404

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Directly meso-meso linked porphyrin rings : synthesis, characterization, and efficient excitation energy hopping.2005

    • Author(s)
      Y Nakamura, in-Wook Hwang, N.Aratani, Tae Kyu Ahn, Dah Mee Ko, A.Takagi, T.Kawai, T.Matsumoto, Dongho Kim, A.Osuka
    • Journal Title

      J.Am.Chem.Soc. 127

      Pages: 236-246

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary
  • [Journal Article] Giant meso-meso-Linked Porphyrin Arrays of Micrometer Molecular Length and Their Fabrication.2005

    • Author(s)
      N.Aratani, A.Takagi, Y.Yanagawa, T.Matsumoto, T.Kawai, Zin Seok Yoon, Dongho Kim, A.Osuka
    • Journal Title

      Chem.A-Euro.J. 11

      Pages: 3389-3404

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2006 Final Research Report Summary 2005 Annual Research Report
  • [Journal Article] Directly meso-meso linked porphyrin rings : synthesis, characterization, and efficient excitation energy hopping.2005

    • Author(s)
      Y.Nakamura, in-Wook Hwang, N.Aratani, Tae Kyu Ahn, Dah Mee Ko, A.Takagi, T.Kawai, T.Matsumoto, Dongho Kim, A.Osuka
    • Journal Title

      J.Am.Chem.Soc. 127

      Pages: 236-246

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Conductance measurement of a DNA network in nanoscale by point contact current imaging atomic force microscopy.2005

    • Author(s)
      A.Terawaki, Y.Otsuka, Hea yeon Lee, T.Matsumoto, Hid.Tanaka, T.Kawai
    • Journal Title

      Appl.Phys.Lett. 86

      Pages: 113901-113903

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Printing Electrode for Top-Contact Molecular Junction2005

    • Author(s)
      K.Ojima, Y.Otsuka, T.Matsumoto, T.Kawai
    • Journal Title

      Appl.Phys.Lett. 87

    • Related Report
      2005 Annual Research Report
  • [Patent(Industrial Property Rights)] 探針装置2004

    • Inventor(s)
      松本卓也, 川合知二
    • Industrial Property Rights Holder
      独立行政法人科学技術振興機構
    • Industrial Property Number
      2004-188360
    • Filing Date
      2004-06-25
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2006 Final Research Report Summary 2004 Annual Research Report

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Published: 2004-04-01   Modified: 2016-04-21  

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