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Microscopic Research of Spin, Charge and Orbital Ordering in A-Site Ordered Manganites

Research Project

Project/Area Number 16540324
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionThe University of Tokushima

Principal Investigator

OHNO Takashi  Univ., Tokushima, Engineering, Professor, 工学部, 教授 (70035640)

Co-Investigator(Kenkyū-buntansha) KISHIMOTO Yutaka  Univ., Tokushima, Faculty of Engineering, Professor, 工学部, 教授 (80201458)
KAWASAKI Yu  Univ., Tokushima, Faculty of Engineering, Lecturer, 工学部, 講師 (10346588)
Project Period (FY) 2004 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2005: ¥1,200,000 (Direct Cost: ¥1,200,000)
Fiscal Year 2004: ¥2,500,000 (Direct Cost: ¥2,500,000)
KeywordsStrongly Correlated Systems / Manganese Oxide / Phase Separation / Spin Ordering / Charge Ordering / Orbital Ordering / Nuclear Manetic Resonance / Relaxation Rate / 規則格子系 / スピン・電荷・軌道秩序 / スペクトル
Research Abstract

In these years various kind of and a lot of researches have been made concerning the well-known CMR manganites. Recently A-site ordered manganese oxides have been synthesized. We have been investigating the A-site ordered LaBaMn_2O_6 and YBaMn_2O_6 by measuring ^<139>La and ^<55>Mn NMR. We could observe the ^<55>Mn NMR signals from Mn nuclei both in ferromagnetic and antiferromagnetic regions as well as ^<139>La NMR signals from La nuclei both in ferromagnetic and antiferromagnetic regions at the ground state of LaBaMn_2O_6. Therefore it is evidenced that the ferromagnetic and antiferromagnetic regions are coexisting in LaBaMn_2O_6 from a microscopic point of view although LaO,BaO and MnO_2 layers are ordering crystallographically. The fact that the antiferromagnetic region appears and grows in the ferromagnetic region below 200 K and that it occupies about 50 % at the ground state has been shown by comparing the temperature dependence of Mn internal field with that of the neutron scattering intensity by the ferromagnetic region. It has been also evidenced that the ferromagnetic region is not nano-scale but mezzo-scale because ^<55>Mn NMR signals show a very big enhancement due to the domain walls. The ferromagnetic state coexistent with antiferromagnetic region in LaBaMn_2O_6 is proved to be the same as that in disordered La_<0.5>Ba_<0.5>MnO_3. from the same temperature dependence of spin-spin relaxation rate. We have been also measuring μSR at TRIUMF and KEK.

Report

(3 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • Research Products

    (27 results)

All 2006 2005 2004

All Journal Article (27 results)

  • [Journal Article] Ground State Properties of the A-site ordered/disordered manganites LaBaMn_2O_6/La_<0 : 5>MnO_3 probed by NMR2006

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Physica B (in press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Phase separation in A-site ordered Manganite LaBaMu_2O_6 proved by ^<139>La and ^<55>Mn NMR2006

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Physical Review Letters 69.3

      Pages: 37202-37205

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Ground State Properties of the A-site ordered/disordered manganites LaBaMn_2O_6/La_<0:5>Ba_<0:5>MnO_3 probed by NMR2006

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Physica B (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Phase separation in A-site ordered Manganite LaBaMu_2O_6 proved by ^<139>La and ^<55>Mn NMR2006

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Physical Review Letters 96,3

      Pages: 37202-37205

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Ground State Properties of the A-site ordered/disordered manganites LaBaMn_2O_6/La_<0:5>Ba_<0:5>MnO_3 probed by NMR2006

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Physica B (印刷中)

    • Related Report
      2005 Annual Research Report
  • [Journal Article] La-NQR study of superconductivity in La_3Ir_2Ge_22005

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Physica B 359, 360, 361

      Pages: 503-505

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<55>Mn NMR spectrum at the ground state in the A-site ordered RBaMn_2O_62005

    • Author(s)
      Takashi Ohno
    • Journal Title

      Physica B 359, 360, 362

      Pages: 1291-1293

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] La-NQR study of superconductivity in La_3Ir_2Ge_22005

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Physica B 359-361

      Pages: 503-505

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] ^<55>Mn NMR spectrum at the ground state in the A-site ordered RBaMn_2O_62005

    • Author(s)
      Takashi Ohno
    • Journal Title

      Physica B 359-361

      Pages: 1291-1293

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] ^<139>La NQR Relaxation in Superconductor La_3Ir_2Ge_22004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan 73.12

      Pages: 3389-3393

    • NAID

      110001979310

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<11>B NMR Study of Magnetism in RRh_3B_2 (R=La, Ce, Nd, Sm, Eu and Gd)2004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan 73.7

      Pages: 1970-1981

    • NAID

      110001954917

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<139>La NQR Relaxation in Superconductor LaRu_3Si_22004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272, 273, 274, 275, 276

      Pages: 507-508

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spin fluctuation temperatures in mixed valence materials studied by magnetic susceptibility2004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272, 273, 274, 275, 277

      Pages: 509-510

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<209>Bi-NQR Investigation of the Non-magnetic Heavy-fermion compound CeRhBi2004

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Journal of the Physical Society of Japan 73.3

      Pages: 694-697

    • NAID

      110001954797

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] La NQR Probe of Strong-Coupling s-Wave Superconductivity in LaRu_3Si_22004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan 73.1

      Pages: 190-193

    • NAID

      110001954710

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<139>La NQR Relaxation in a Superconductor La_3Ir_2Ge_22004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan 73,12

      Pages: 3389-3393

    • NAID

      110001979310

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<11>B_NMR Study of Magnetism in_RRh_3B_2 (R=La,Ce,Nd,Sm,Eu and Gd)2004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan 73,7

      Pages: 1970-1981

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<139>La NQR Relaxation in Superconductor LaRu_3Si_22004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 507-508

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spin fluctuation temperatures in mixed valence materials studied by magnetic susceptibility2004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 509-510

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<209>Bi-NQR Investigation of the Non-magnetic Heavy-fermion Compound CeRhBi2004

    • Author(s)
      Yu Kawasaki
    • Journal Title

      Journal of the Physical Society of Japan 73,3

      Pages: 694-697

    • NAID

      110001954797

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] La-NQR Probe of Strong-Coupling s-Wave Superconductivity in LaRu_3Si_22004

    • Author(s)
      Yutaka Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan 73,1

      Pages: 190-193

    • NAID

      110001954710

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] La-NQR Probe of Strong-Coupling s-Wave Superconductivity in LaRu3Si22004

    • Author(s)
      Y.Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan Vol.73, No.1

      Pages: 190-193

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 209Bi-NQR Investigation of the Non-magnetic Heavy-fermion Compound CeRhBi2004

    • Author(s)
      Y.Kawasaki
    • Journal Title

      Journal of the Physical Society of Japan Vol.73, No.3

      Pages: 694-697

    • NAID

      110001954797

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Spin fluctuation temperatures in mixed valence materials studied by magnetic Susceptibility2004

    • Author(s)
      Y.Kishimoto
    • Journal Title

      Journal of Magnetism and Magnetic Materials Vol.272-276

      Pages: 509-510

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 139La NQR Relaxation in Superconductor LaRu3Si22004

    • Author(s)
      Y.Kishimoto
    • Journal Title

      Journal of Magnetism and Magnetic Materials Vol.272-276

      Pages: 507-508

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 11B NMR Study of Magnetism in RRh3B2 (R=La, Ce, Nd, Sm, Eu and Gd)2004

    • Author(s)
      Y.Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan Vol.73, No.7

      Pages: 1970-1981

    • NAID

      130004538858

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 139La NQR Relaxation in a Superconductor La3Ir2Ge22004

    • Author(s)
      Y.Kishimoto
    • Journal Title

      Journal of the Physical Society of Japan Vol.73, No.12

      Pages: 3389-3393

    • NAID

      210000105208

    • Related Report
      2004 Annual Research Report

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Published: 2004-04-01   Modified: 2020-05-15  

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