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Development of a process for the production of high bio-based content functional materials from un-utilized biomass

Research Project

Project/Area Number 16H01790
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental conscious materials and recycle
Research InstitutionThe University of Tokushima

Principal Investigator

NAKAMURA Yoshitoshi  徳島大学, 大学院社会産業理工学研究部(生物資源産業学域), 教授 (20172455)

Co-Investigator(Kenkyū-buntansha) 浅田 元子  徳島大学, 大学院社会産業理工学研究部(生物資源産業学域), 准教授 (10580954)
高木 均  徳島大学, 大学院社会産業理工学研究部(理工学域), 教授 (20171423)
佐々木 千鶴  徳島大学, 大学院社会産業理工学研究部(生物資源産業学域), 准教授 (50452652)
渡邊 隆司  京都大学, 生存圏研究所, 教授 (80201200)
Project Period (FY) 2016-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥41,210,000 (Direct Cost: ¥31,700,000、Indirect Cost: ¥9,510,000)
Fiscal Year 2019: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2018: ¥7,150,000 (Direct Cost: ¥5,500,000、Indirect Cost: ¥1,650,000)
Fiscal Year 2017: ¥15,990,000 (Direct Cost: ¥12,300,000、Indirect Cost: ¥3,690,000)
Fiscal Year 2016: ¥12,480,000 (Direct Cost: ¥9,600,000、Indirect Cost: ¥2,880,000)
Keywordsリグノセルロース廃棄物 / セルロースナノファイバー / リグニンエポキシ樹脂 / 水蒸気爆砕 / バイオリファイナリー / バイオマス / バイオマテリアル
Outline of Final Research Achievements

Lignocellulosic waste are used to produce biofuels and biomaterials. Increased use of these resources would lower environmental impacts such as the emission of greenhouse gases and fossil fuel depletion, helping to create a sustainable environment. This work proposed a new effective and environmentally friendly biorefinery process of lignocellulosic waste using a steam explosion followed by water and acetone extractions. The water extract, acetone extract, and the holocellulose component derived from steam-exploded lignocellulosic waste were converted into useful eco-materials. The water extract from steam-exploded product showed a high antioxidant activity. The acetone extract was converted into a cured lignin epoxy resin with high heat-resisting properties. The holocellulose component was used as the raw material for the CNF, and its reinforcement effect on the PLA resin was demonstrated.

Academic Significance and Societal Importance of the Research Achievements

本研究では,バイオマス構成成分の特性を損なわない程度の前処理と分離操作を用いて,分離構成成分を高収率,低コストおよび省エネルギーで高植物度機能性化成品に変換するための製造プロセスの開発を目指す。前処理として環境低負荷な高活性水蒸気爆砕,構成成分分離のための水・有機溶媒抽出および高植物度化成品の製造技術から成る一連のプロセスにより,バイオマス利用法の新しいステージ(バイオマス構成成分の物理・化学・生物的特性を十分に活かす化成品製造法)が開拓され,低炭素・循環型社会の実現に大きく寄与する。

Report

(5 results)
  • 2020 Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (25 results)

All 2021 2020 2019 2018 2017 2016

All Journal Article (11 results) (of which Peer Reviewed: 11 results) Presentation (14 results) (of which Int'l Joint Research: 6 results,  Invited: 3 results)

  • [Journal Article] Effect of Activated Cow Dung as Inoculum on Methane Production of Steam-Exploded Rice Husks2021

    • Author(s)
      Sholahuddin、Nakamura Yoshitoshi、Asada Chikako
    • Journal Title

      Waste and Biomass Valorization

      Volume: - Issue: 9 Pages: 5019-5028

    • DOI

      10.1007/s12649-021-01365-6

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Microwave-Assisted Hydrolysis of Cellulose in Towel and Wheat Straw Using Freeze-Thawing with NaOH2020

    • Author(s)
      Sasaki Chizuru、Sumitomo Yuka、Odashima Kai、Asada Chikako、Nakamura Yoshitoshi
    • Journal Title

      Waste and Biomass Valorization

      Volume: - Issue: 6 Pages: 3331-3339

    • DOI

      10.1007/s12649-020-01219-7

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ethanol Production from Sugarcane Bagasse Using Pressurized Microwave Treatment with Inorganic Salts and Salt-Tolerant Yeast2019

    • Author(s)
      Asada Chikako、Sasaki Chizuru、Oka Chihiro、Nakamura Yoshitoshi
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 5 Pages: 2001-2007

    • DOI

      10.1007/s12649-018-0527-z

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effects of Hydrothermal Methods such as Steam Explosion and Microwave Irradiation on Extraction of Water Soluble Antioxidant Materials from Garlic Husk2019

    • Author(s)
      Noda Yuko、Asada Chikako、Sasaki Chizuru、Nakamura Yoshitoshi
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 11 Pages: 3397-3402

    • DOI

      10.1007/s12649-018-0353-3

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Isolation and identification of an angiotensin I-converting enzyme inhibitory peptide from pearl oyster (Pinctada fucata) shell protein hydrolysate2019

    • Author(s)
      Sasaki Chizuru、Tamura Satoshi、Tohse Riho、Fujita Saki、Kikuchi Miyu、Asada Chikako、Nakamura Yoshitoshi
    • Journal Title

      Process Biochemistry

      Volume: 77 Pages: 137-142

    • DOI

      10.1016/j.procbio.2018.11.017

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Microwave-assisted glucose production from bode (Styrax tonkinensis) woody biomass for bioethanol production2018

    • Author(s)
      Sasaki Chizuru、Negoro Haruka、Asada Chikako、Nakamura Yoshitoshi
    • Journal Title

      Journal of Material Cycles and Waste Management

      Volume: 21 Issue: 1 Pages: 201-204

    • DOI

      10.1007/s10163-018-0783-9

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Production of cellulose nanofibers from Aspen and Bode chopsticks using a high temperature and high pressure steam treatment combined with milling2018

    • Author(s)
      A. Suzuki, C. Sasaki, C. Asada, Y. Nakamura
    • Journal Title

      Carbohydrate Polymers

      Volume: - Pages: 303-310

    • DOI

      10.1016/j.carbpol.2018.04.047

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Glucose and Valuable Chemicals Production from Cotton Waste Using Hydrothermal Method2018

    • Author(s)
      Chizuru Sasaki, Ami Kiyokawa, Chikako Asada and Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 3 Pages: 599-607

    • DOI

      10.1007/s12649-017-0084-x

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High concentration ethanol production from mixed softwood sawdust waste2018

    • Author(s)
      Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 2 Pages: 433-439

    • DOI

      10.1007/s12649-017-0073-0

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Total Biorefinery Process of Lignocellulosic Waste Using Steam Explosion Followed by Water and Acetone Extractions2018

    • Author(s)
      Asada C.、Sasaki C.、Suzuki A.、Nakamura Y.
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 12 Pages: 2423-2432

    • DOI

      10.1007/s12649-017-0157-x

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of cellulose nanofiber from steam exploded Japanese cedar2017

    • Author(s)
      Akihiro Suzuki, Chizuru Sasaki, Chikako Asada, Yoshitoshi Nakamura
    • Journal Title

      BioResources

      Volume: 12 Issue: 4 Pages: 7628-7641

    • DOI

      10.15376/biores.12.4.7628-7641

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] Renewable Resource-Based Material Synthesized from Lignocellulosic Biomass2018

    • Author(s)
      C. Asada, C. Sasaki, Y. Nakamura
    • Organizer
      12th World Congress on Biofuels and Bioenergy & 13th Global Summit and Expo on Biomass and Bioenergy、Zurich
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 木質バイオマスからの高植物度機能性化成品の製造2017

    • Author(s)
      淺田元子,佐々木千鶴,鈴木昭浩,中村嘉利
    • Organizer
      第12回バイオマス科学会議
    • Place of Presentation
      東京大学(東京都文京区)
    • Year and Date
      2017-01-18
    • Related Report
      2016 Annual Research Report
  • [Presentation] バイオマスへの応用を考慮した耐熱性セルラーゼ利用のための酵素カクテルの相乗効果検討,2017

    • Author(s)
      髙田弥生、淺田元子、佐々木千鶴、中村嘉利
    • Organizer
      第9回日本醸造学会 若手シンポジウム, 東京
    • Related Report
      2017 Annual Research Report
  • [Presentation] ファルカタを原料としたバイオエタノール製造のための水蒸気爆砕前処理の最適条件の検討2017

    • Author(s)
      妹尾政都、浅田元子、佐々木千鶴、中村嘉利
    • Organizer
      第9回日本醸造学会 若手シンポジウム, 東京
    • Related Report
      2017 Annual Research Report
  • [Presentation] バイオエタノール残渣となるモデルリグニンを用いたエポキシ樹脂合成の抽出溶媒検討2017

    • Author(s)
      藤井萌、浅田元子、佐々木千鶴、中村嘉利
    • Organizer
      第9回日本醸造学会 若手シンポジウム, 東京
    • Related Report
      2017 Annual Research Report
  • [Presentation] Glucose production from cotton-waste using hydrothermal methods2017

    • Author(s)
      Chizuru Sasaki, Chikako Asada, Yoshitoshi Nakamura
    • Organizer
      The 4th International Cellullose Conference (ICC 2017), Fukuoka
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Synthesis of ecomaterial from plant biomass and its physical properties2017

    • Author(s)
      Akihiro Suzuki, Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Organizer
      13th International Conference on Ecomaterials, Bangkok
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Comparison of steam explosion and steaming followed by milling treatment for bioethanol production from woody biomass2017

    • Author(s)
      Yuta Danura, Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Organizer
      13th International Conference on Ecomaterials, Bangkok
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Organosolv lignin extracted from hydrolyzed residue of steam exploded hardwood: a potential candidate for epoxy resin2017

    • Author(s)
      Takuya Yamamoto, Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Organizer
      13th International Conference on Ecomaterials, Bangkok
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 徳島県産間伐材を有効利用するための総合プロセス開発2017

    • Author(s)
      淺田元子
    • Organizer
      日本生物工学会生物資源を活用した地域創生研究部会シンポジウム(大阪大学吹田キャンパス)
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 木材構成成分の分離回収と有効利用2017

    • Author(s)
      淺田元子
    • Organizer
      化学工学会第82年会(芝浦工業大学豊洲キャンパス)
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] バイオマスの総合的有効利用プロセス2016

    • Author(s)
      中村嘉利
    • Organizer
      化学工学会第48回秋季大会
    • Place of Presentation
      徳島大学(徳島県徳島市)
    • Year and Date
      2016-09-06
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] 広葉樹アスペン廃材の総合利用プロセスの構築2016

    • Author(s)
      山本拓也,入江 翼,鈴木昭浩,佐々木千鶴,淺田元子,中村嘉利
    • Organizer
      第3回日本生物工学会西日本支部講演会
    • Place of Presentation
      徳島大学(徳島県徳島市)
    • Related Report
      2016 Annual Research Report
  • [Presentation] Fiber orientation control in cellulose nanofiber-reinforced green nanocomposites2016

    • Author(s)
      Hitoshi Takagi, Antonio Norio Nakagaito and Yuya Sakaguchi
    • Organizer
      Fiber Society 2016 Fall Meeting and Technical Conference
    • Place of Presentation
      Ithaca (U.S.A.)
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research

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Published: 2016-04-21   Modified: 2022-01-27  

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